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Quantum Nanophotonic Materials, Devices, and Systems

Integrated lithium niobite photonic circuits for nonlinear photon-pair generation and linear photonic state manipulation

Hyounghan Kwon

Published Oct 4, 2024• 0 citations
Publisher

Abstract

Integrated quantum photonic system has become a promising candidate for next-generation quantum optical system. Thanks to the scalability and strong light-matter interactions, such nanophotonic systems can realize compactness, large-scale integration, stability, and novel optical functionalities simultaneously. In this talk, I will introduce our experimental works in the fields of the integrated lithium niobate photonics. First, we demonstrate a set of nonlinear photon-pair generations for the nonlinear quantum photonic sources. Next, I will show our works on lithium-niobate integrated quantum photonic circuits for the application in quantum communications and variational quantum simulations.

DOI
10.1117/12.3029243

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Integrated quantum photonic system has become a promising candidate for next-generation quantum optical system. Thanks to the scalability and strong light-matter interactions, such nanophotonic systems can realize compactness, large-scale integration, stability, and novel optical functionalities simultaneously. In this talk, I will introduce our experimental works in the fields of the integrated lithium niobate photonics. First, we demonstrate a set of nonlinear photon-pair generations for the nonlinear quantum photonic sources. Next, I will show our works on lithium-niobate integrated quantum photonic circuits for the application in quantum communications and variational quantum simulations.
Quantum technologies have surpassed classical systems by leveraging the unique properties of superposition and entanglement in photons and matter. Recent advancements in integrated quantum photonics, especially in silicon-based and lithium niobate platforms, are pushing the technology toward greater scalability and functionality. Silicon circuits have progressed from centimeter-scale, dual-photon systems to millimeter-scale, high-density devices that integrate thousands of components, enabling sophisticated programmable manipulation of multi-photon states. Meanwhile, lithium niobate, thanks to its wide optical transmission window, outstanding nonlinear and electro-optic coefficients, and chemical stability, has emerged as an optimal substrate for fully integrated photonic quantum chips. Devices made from this material exhibit high efficiency in in generating, manipulating, converting, storing, and detecting photon states, thereby establishing a basis for deterministic multi-photon generation and single-photon quantum interactions, as well as comprehensive frequency-state control. This review explores the development of integrated photonic quantum technologies based on both silicon and lithium niobate, highlighting invaluable insights gained from silicon-based systems that can assist the scaling of lithium niobate technologies. It examines the functional integration mechanisms of lithium niobate in electro-optic tuning and nonlinear energy conversion, showcasing its transformative impact throughout the photonic quantum computing process. Looking ahead, we speculate on the developmental pathways for lithium niobate platforms and their potential to revolutionize areas such as quantum communication, complex system simulation, quantum sampling, and optical quantum computing paradigms.
Quantum photonics has advanced rapidly and become a leading approach for developing a broad range of quantum technologies, including quantum communications, quantum information processing, quantum computing, and quantum sensing. Besides, the emerging photonic integrated circuits (PIC) technology has been widely used to implement versatile optical elements advantageous for different quantum applications. For example, PIC-based devices have functioned as building blocks, such as photonic qubit sources, linear optical circuits, modulators, and even single-photon detectors, for realizing highly integrated, large-scale quantum computing schemes. In such a powerful quantum photonic integrated circuits (QPIC) scheme, the creation, manipulation, and testing of quantum entanglement states from the generated qubits via a reconfigurable photonic circuitry are essential. Though the state-of-the-art PIC technology is established based on Si photonics due to its widely mature nanophotonic circuit (waveguide) fabrication technology supported by the existing immense semiconductor industry, Si-based PIC has limitations in implementing efficient and fast active elements that usually demand a quadratic nonlinearity. Lithium niobate (LN), renowned as “the silicon of photonics”, has long been a popular material widely used in integrated-optical and nonlinear-optical applications. A great variety of passive and active photonic elements have been realized in the LN platform. Recently, a novel material based on high-quality single-crystalline films of LN, known as thin-film LN on insulator (LNOI), has been developed and has soon drawn enormous attention for its greatly promising ability to realize nanoscale PIC/QPIC in this iconic optical material platform. In this presentation, we report our recent studies on several key LN PIC building blocks for developing novel quantum photonic sources and circuits, including highly integrated photonic-circuit periodically poled lithium niobate (PPLN) chips for photon-pair generation and manipulation, for high-dimensional frequency-entangled qudit production, for time-frequency grid-state generation, for continuous-variable squeezed vacuum state generation, and their potential applications to quantum computing/communication/sensing technology. Besides, a PP-LNOI electro-optic (EO) polarization mode converter (PMC) useful for demonstrating fast control of quantum polarization states and other LNOI circuit elements as QPIC building blocks will also be presented.
Entangled photons generation is an interesting field of research, since progress in this area will directly affect the development of photonic quantum technologies, including quantum computing, simulation and sensing. Several methods have been sifted to increase the performances of entangled photon sources and the integrated optics approach represents a promising strategy. In particular, integrated waveguide sources represent a robust tool, thanks to their stability and the enhancement of nonlinear light-crystal interaction provided by waveguide field confinement. Here, we show the versatility of a hybrid approach, realizing an integrated optical source for the generation of entangled photon-pairs at telecom wavelength. The nonlinear active medium used is lithium niobate, while the routing and manipulation of the generated signal is performed in aluminum-borosilicate glass photonic circuits. The system is composed of three cascaded devices. First, a balanced directional coupler at the fundamental wavelength equally splits the pump in the lithium niobate waveguides, which generate single-photon pairs through type 0 spontaneous parametric down-conversion process. A third chip, encompassing directional couplers and waveplates, closes the interferometer and recombines the generated photons, thus giving access to different quantum states of light: path-entangled or polarization-entangled states. A thermal phase shifter, which controls the relative phase between the interferometer arms, gives an additional degree of freedom for engineering the output state of the presented photon pairs source. All these components are entirely fabricated by femtosecond laser micromachining, a direct and very versatile technique that allows to process different kind of materials and realize high quality optical circuits.
Generating and interfering nonclassical states of light is fundamental to optical quantum information science and technology. Quantum photonic integrated circuits provide one pathway towards scalability by combining nonlinear sources of nonclassical light and programmable circuits in centimeter-scale devices. The key requirements for quantum applications include efficient generation of indistinguishable photon-pairs and high-visibility programmable quantum interference. Here, we demonstrate a lithium niobate-on-insulator (LNOI) integrated photonic circuit that generates a two-photon path-entangled state, and a programmable interferometer for quantum interference. We generate entangled photons with ∼2.3×10^{8} pairs/s/mW brightness and perform quantum interference experiments on the chip with 96.8±3.6% visibility. LNOI is an emerging photonics technology that has revolutionized high-speed modulators and efficient frequency conversion. Our results provide a path towards large-scale integrated quantum photonics including efficient photon-pair generation and programmable circuits for applications such as boson sampling and quantum communications.
Integrated thin-film lithium niobate (TFLN) photonics has emerged as a powerful platform for quantum information science, offering its outstanding nonlinear, electro-optic (EO), and integration capabilities. In this review, we present the latest advances in TFLN-based integrated photonics tailored to quantum technologies. We first explore state-of-the-art quantum light sources realized in both straight waveguide and resonator configuration, including high-brightness photon pair generations, squeezed light, and versatile entanglement schemes. Next, we detail progress in integrated photonic processors, with a focus on programmable interferometric networks, ultrafast EO modulators, and essential passive components for photonic qubit processing. We then address critical challenges in optical interfacing and detection technologies, discussing recent innovations in low-loss fiber-to-chip and grating coupler designs, as well as the integration of on-chip single photon detectors. This review provides a forward-looking perspective on scalable quantum photonic systems that could underpin future advances in quantum communication, computing, and sensing.
The aim of this thesis is to explore nonlinear nanostructures – photonic systems with one or more dimension with nanoscale feature size – as new platforms for parametric photon-pair generation. This is motivated by the need for photon-pair sources in many technological applications of quantum optics, such as quantum communication, imaging and computing. The initial hypothesis is that nonlinear nanostructures are a promising platform to complement established photon-pair source schemes based on bulk crystals or photonic integrated circuits in terms of quantum state-engineering, footprint, functional density etc. However, nonlinear pair generation, e.g. via spontaneous parametric down-conversion (SPDC), is a new subfield in nanophotonics with a very limited number of studies existing. This constitutes the knowledge-gap addressed in this thesis. Therefore, the objective is to provide first experimental demonstrations of SPDC in subwavelength-scale and nonlinear nanostructures. We investigate the ability of such systems to control the properties of two-photon quantum states such as frequency and angular spectrum or polarization entanglement. To this end we analyze nanostructures with different degrees of complexity, starting with an unstructured thin crystal with one nanoscale dimension, leading up to a 3D nano-scale resonator with subwavelength-sized features in all dimensions. Furthermore, we test different types of nonlinear materials such as lithium niobate, group III-V semiconductors and emerging, highly nonlinear materials such as molybdenum disulfide. Additionally, we also advance the theoretical understanding by developing a comprehensive model of the quantum process of nonlinear parametric pair-generation in photonic nanostructures.