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Optics Express

Enhancing the sensitivity of spin-exchange relaxation-free magnetometers using phase-modulated pump light with external Gaussian noise

Ning Ma, Xiujie Fang, Yaqi Zhang, Bozheng Xing, Lihong Duan, Jixi Lu, Bangcheng Han, Danyue Ma

Published Aug 8, 2024• 74 citations
Publisher

Abstract

An optical pumping scheme is proposed for reducing the gradient of electron spin polarization and suppressing light source noise in a spin-exchange relaxation-free magnetometer. This is achieved by modulating only the phase of a narrow-linewidth pump light field with external Gaussian noise. Compared to the absence of phase modulation, the uniformity of electron spin polarization was improved by over 40%, and the light-frequency noise suppression ratio of the magnetometer was enhanced by 4.3 times. Additionally, the response of the magnetometer was increased by 54%, resulting in a sensitivity of 0.34 fT/Hz 1/2 at 30 Hz. The applicability of this scheme can extend to other optical pumping experiments involving large atom ensembles requiring uniform electron spin polarization distribution, which is beneficial for developing ultra-high sensitivity and high stability magnetometers essential for magneto-cardiography and magneto-encephalography research applications.

DOI
10.1364/oe.530764

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An optical pumping scheme is proposed for reducing the gradient of electron spin polarization and suppressing light source noise in a spin-exchange relaxation-free magnetometer. This is achieved by modulating only the phase of a narrow-linewidth pump light field with external Gaussian noise. Compared to the absence of phase modulation, the uniformity of electron spin polarization was improved by over 40%, and the light-frequency noise suppression ratio of the magnetometer was enhanced by 4.3 times. Additionally, the response of the magnetometer was increased by 54%, resulting in a sensitivity of 0.34 fT/Hz 1/2 at 30 Hz. The applicability of this scheme can extend to other optical pumping experiments involving large atom ensembles requiring uniform electron spin polarization distribution, which is beneficial for developing ultra-high sensitivity and high stability magnetometers essential for magneto-cardiography and magneto-encephalography research applications.
A high-sensitivity atomic magnetometer based on broad linewidth laser pumping is demonstrated. The broad linewidth laser was obtained by broadening a narrow linewidth laser utilizing an external phase modulator driven by a pseudo-random-bit-sequence (PRBS) waveform. This ingenious optical pumping scheme can significantly enhance the signal response and suppress light shift noise, as well as can reduce the gradient of electron spin polarization and improve the stability of magnetometers. Compared with a narrow linewidth laser pumping scheme, the response of the magnetometer is increased by 56%, experimentally. The relative polarization gradient is reduced from 9.8%/cm to better than 4%/cm by setting PRBS with a bit rate of 16 GHz. This scheme can also be applied to many other fields such as noninvasive bio-magnetic imaging and atomic spin gyroscopes.
A hybrid optical pumping method employing a broad linewidth laser is proposed to enhance spin coherence and suppress virtual magnetic field noise in atomic magnetometers. The central frequency of broad linewidth laser is tuned to the resonance peak of the alkali-metal atoms D1 line. Its multiple frequency components suppress AC-Stark shift fluctuations caused by pumping laser frequency variations, thereby reducing virtual magnetic field noise. In addition, these components decrease the average optical absorption cross-section, improving the uniformity of atomic spin polarization, further enhancing spin coherence and extending transverse relaxation time. Experimental results show that, compared with narrow linewidth pumping, the proposed method suppresses virtual magnetic field noise by 17.95% to 34.50%, and increases the magnetometer response by 1.62% to 30.31% at 5 Hz. The average sensitivity within the frequency range of 1-20 Hz is improved to 0.158 fT/Hz 1/2 , representing a significant enhancement of 30.70% compared to narrow linewidth pumping.
Quantum manipulation technology and photoelectric detection technology have jointly facilitated the rapid development of ultra-sensitive atomic spin magnetometers. To improve the output signal and sensitivity of the spin-exchange-relaxation-free (SERF) atomic spin magnetometer, the noises influencing on the output signal and the sensitivity were analyzed, and the corresponding noise suppression methods were presented. The magnetic field noises, including the residual magnetic field noise and the light shift noise, were reduced to approximately zero by employing the magnetic field compensation method and by adjusting the frequency of the pump beam, respectively. With respect to the operation temperature, the simulation results showed that the temperature of the potassium atomic spin magnetometer realizing the spin-exchange relaxation-free regime was 180 °C. Moreover, the fluctuation noises of the frequency and the power were suppressed by using the frequency and the power stable systems. The experimental power stability results showed that the light intensity stability was enhanced 10%. Contrast experiments on the sensitivity were carried out to demonstrate the validity of the suppression methods. Finally, a sensitivity of 13 fT/Hz(1/2) was successfully achieved by suppressing noises and optimizing parameters.
This work proposes an optical pumping strategy based on a broadband laser to overcome the problem of atomic spin polarization gradients and sensitivity to optical frequency noise in NMR gyroscopes. A band-limited Gaussian white noise radiofrequency signal is applied to a lithium niobate electro-optic phase modulator to do this. A narrow linewidth laser maintains its frequency stability while uniformly broadening its spectrum to the hundreds of MHz range. Compared to unmodulated pumping, the proposed scheme enhances the uniformity of rubidium spin polarization by approximately 10%, reaching a measured value of 92.8%. Additionally, the sensitivity of the inert gas precession signal to optical frequency noise is reduced by half. This scheme can be extended to other atomic sensors requiring higher uniform spin polarization distributions and provides a promising way to achieve high-stability, low-noise NMR gyroscope systems.
Abstract Atomic spin comagnetometers based on the spin-exchange relaxation-free (SERF) effect offer significant potential for inertial sensing and support the development of long-endurance, high-precision navigation technologies. However, limited nuclear spin polarization constrains the long-term stability of these systems. Here, a flat-top optical pumping configuration is introduced for SERF comagnetometers, expanding the uniform-intensity region of the beam to approximately 62 % , which enhances atomic polarization by around 19 % and improves magnetic noise suppression by 32 % . Experimental results demonstrate notable improvements in both sensitivity and long-term stability, highlighting the effectiveness of flat-top beams in overcoming atomic polarization uniformity limitations and advancing SERF co-magnetometer performance.
We demonstrate the bandwidth enhancement of an all-optical spin-exchange relaxation-free (SERF) magnetometer based on amplitude-modulated (AM) light. Alkali metal atoms are modulated directly by the pump beam instead of the modulation field or radio frequency field. The first harmonic demodulation of an AM SERF magnetometer with a modulation intensity of 15 kHz results in a high bandwidth of over 11 kHz with a sensitivity of 20 fT/Hz1/2 at 30 Hz and 60 fT/Hz1/2 at 10 kHz. Meanwhile, the AM SERF magnetometer with DC demodulation presents the same sensitivity as a traditional DC SERF magnetometer (6 fT/Hz1/2 at 30 Hz). The presented technique for modulating the amplitude of the pump beam allows AM SERF magnetometers to enter the domain of high-bandwidth magnetometers and opens the door to many areas that are inaccessible to conventional magnetometers.