Abstract Atomic spin comagnetometers based on the spin-exchange relaxation-free (SERF) effect offer significant potential for inertial sensing and support the development of long-endurance, high-precision navigation technologies. However, limited nuclear spin polarization constrains the long-term stability of these systems. Here, a flat-top optical pumping configuration is introduced for SERF comagnetometers, expanding the uniform-intensity region of the beam to approximately 62 % , which enhances atomic polarization by around 19 % and improves magnetic noise suppression by 32 % . Experimental results demonstrate notable improvements in both sensitivity and long-term stability, highlighting the effectiveness of flat-top beams in overcoming atomic polarization uniformity limitations and advancing SERF co-magnetometer performance.
Abstract Atomic spin comagnetometers based on the spin-exchange relaxation-free (SERF) effect offer significant potential for inertial sensing and support the development of long-endurance, high-precision navigation technologies. However, limited nuclear spin polarization constrains the long-term stability of these systems. Here, a flat-top optical pumping configuration is introduced for SERF comagnetometers, expanding the uniform-intensity region of the beam to approximately 62 % , which enhances atomic polarization by around 19 % and improves magnetic noise suppression by 32 % . Experimental results demonstrate notable improvements in both sensitivity and long-term stability, highlighting the effectiveness of flat-top beams in overcoming atomic polarization uniformity limitations and advancing SERF co-magnetometer performance.
Ultrasensitive spin exchange relaxation-free (SERF) comagnetometers have been widely applied in various new physics experiments and show great potential for inertial navigation. However, the spatially nonuniform spin polarization of alkali metal (AM) and noble gas (NG) atoms results in an effective magnetic field gradient on the order of 100 nT/cm which is much larger than that is produced by the coils and remanence on the magnitude of 1 nT/cm, thereby reducing the suppression ability of the magnetic noise and limiting the scale factor and noise floor of the comagnetometers. In this study, we establish a model of the effective magnetic field gradient caused by uneven spin polarization and analyze the influencing factors. Our results indicate that optimizing the density ratio of hybrid AM atoms can suppress the effective magnetic field gradient. Nevertheless, the available pump light power imposes a limitation on the density ratio. To further address this issue, we propose a balanced light-assisted hybrid spin exchange optical pumping (HSEOP) method. Our experimental results confirm the effectiveness of the mentioned approach, with 67% suppression of the nuclear transverse relaxation rate and a nearly threefold increase in the scale factor. Furthermore, the optimal density ratio in experimental applications can be reduced from 200 to below 80, thereby overcoming the limitation of laser power in SERF comagnetometers and providing the possibility for wider applications. Finally, the suppression factor of magnetic noise is enhanced by 89% by optimizing the density ratio and the balanced light-assisted HSEOP method. This research sheds light on the fundamental physics experiments and potential for inertial navigation.
Spin exchange relaxation free (SERF) comagnetometers, which use coupled alkali metal and noble gas spins, are promising for precision measurements due to their potential for miniaturization and high sensitivity. In these systems, alkali atoms are optically pumped with circularly polarized light, and their polarization is transferred to noble gas nuclei via spin-exchange collisions. However, spatial inhomogeneities in alkali polarization induced by factors such as optical absorption, gas diffusion, and temperature gradients generate effective magnetic field gradients for the noble gas spins. These gradients accelerate spin relaxation and degrade overall sensor performance. This work introduces a pump beam reflection compensation scheme to improve alkali polarization uniformity in a SERF comagnetometer. By retro reflecting the pump beam back along its original optical path with reversed helicity, alkali atoms are repolarized from the opposite direction. This counter propagating beam compensates polarization gradients through reverse optical pumping, thereby homogenizing the effective field experienced by the noble gas spins. The modified pumping configuration enhances spatial uniformity while maintaining a simple and compact sensor architecture. A revised polarization rate model incorporating the retro reflected beam is presented. Simulations comparing single beam, 90% reflection, and total reflection configurations confirm a marked reduction in alkali polarization gradients for reflection based designs. Experimentally, the transverse relaxation time of the noble gas spins is extended by 77.66%, indicating significantly suppressed gradient induced decoherence. The proposed method supports the development of miniaturized, high performance SERF comagnetometers.
Atomic spin sensors are essential for beyond-the-standard-model exploration, biomagnetic measurement, and quantum navigation. While the traditional DC mode spin-exchange relaxation-free (SERF) comagnetometer achieves ultrahigh sensitivity, further improvements require suppressing technical noise and surpassing standard quantum limit. In this work, we develop a K-Rb-21Ne SERF atomic comagnetometer that dynamically polarizes the electron and nuclear spins, shielding signals from direct interference by pump light. We establish a three-phase evolutionary model for hybrid spin ensemble dynamics, yielding a complete analytical solution, and analyze the responses to various spin perturbations. Additionally, we achieve an averaged 38.5 % suppression of the polarization noise and identify the key factors that limit sensitivity improvements. The dynamically polarized comagnetometer exhibits effective suppression of technical noise and holds the potential to overcome quantum noise limit, while offering promising applications in exploring new physics and precise magnetic field measurements.
In recent years, developments in quantum sensing, laser, and atomic sensor technologies have also enabled advancement in the field of quantum navigation. Atomic-based gyroscopes have emerged as one of the most critical atomic sensors in this respect. In this review, a brief technology statement of spin exchange relaxation free (SERF) and nuclear magnetic resonance (NMR) type atomic comagnetometer gyroscope (CG) is presented. Related studies in the literature have been gathered, and the fundamental compositions of CGs with technical basics are presented. A comparison of SERF and NMR CGs is provided. A basic simulation of SERF CG was carried out because of its high theoretic bias stability limit. Besides, some highly critical challenges for CGs were examined and reported with compensation methods. The objective of this review is to offer a guide for researchers to develop high-precision atomic gyroscopes and to encourage further research.
Atomic spin sensors are essential for beyond-the-standard-model exploration, biomagnetic measurement, and quantum navigation. While the traditional DC mode spin-exchange relaxation-free (SERF) comagnetometer achieves ultrahigh sensitivity, further improvements require suppressing technical noise and surpassing standard quantum limit. In this work, we develop a K-Rb- 21 Ne SERF atomic comagnetometer that dynamically polarizes the electron and nuclear spins, shielding signals from direct interference by pump light. We establish a three-phase evolutionary model for hybrid spin ensemble dynamics, yielding a complete analytical solution, and analyze the responses to various spin perturbations. Additionally, we achieve an average 39% suppression of the polarization noise and identify the key factors that limit sensitivity improvements. The dynamically polarized comagnetometer exhibits effective suppression of technical noise and holds the potential to overcome quantum noise limit while offering promising applications in exploring new physics and precise magnetic field measurements.
We explore the impact of pumping beams with different transverse intensity profiles on the performance of the spin-exchange relaxation-free (SERF) atomic magnetometers (AMs). We conduct experiments comparing the traditional Gaussian optically-pumped AM with that utilizing the flat-top optically-pumped (FTOP) method. Our findings reveal that the FTOP-based approach outperforms the conventional method, exhibiting a larger response, a narrower magnetic resonance linewidth, and a superior low-frequency noise performance. Specifically, the use of FTOP method leads to a 16% enhancement in average sensitivity within 1 Hz–30 Hz frequency range. Our research emphasizes the significance of achieving transverse polarization uniformity in AMs, providing insights for future optimization efforts and sensitivity improvements in miniaturized magnetometers.