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iScience

Ultrafast observation of the abnormal time delay of femtosecond laser pulses in a quartz crystal

Baoshan Guo, Tianyong Zhang, Lan Jiang

Published Jun 19, 2024• 1 citation
Publisher

Abstract

Light with different frequencies has different propagation speeds when propagating in a medium. Nonlinear optics indicates that the refractive index of the medium also varies with the intensity of light. In this article, we have discovered an anomalous slow light phenomenon that is independent of light intensity through multi-frame ultrafast imaging. The experimental results show that when coaxial 800-nm and 400-nm pulses simultaneously enter the quartz crystal, the time delay between the 800-nm and 400-nm laser pulses is up to 5 times the normal value calculated by the dispersion theory. Moreover, this delay is independent of the laser intensity, indicating that the anomalous slow light phenomenon does not originate from refractive index changes in nonlinear optics. This abnormal time delay effect may find more applications in different fields, and its physical mechanism still needs further exploration.

DOI
10.1016/j.isci.2024.110316

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Light with different frequencies has different propagation speeds when propagating in a medium. Nonlinear optics indicates that the refractive index of the medium also varies with the intensity of light. In this article, we have discovered an anomalous slow light phenomenon that is independent of light intensity through multi-frame ultrafast imaging. The experimental results show that when coaxial 800-nm and 400-nm pulses simultaneously enter the quartz crystal, the time delay between the 800-nm and 400-nm laser pulses is up to 5 times the normal value calculated by the dispersion theory. Moreover, this delay is independent of the laser intensity, indicating that the anomalous slow light phenomenon does not originate from refractive index changes in nonlinear optics. This abnormal time delay effect may find more applications in different fields, and its physical mechanism still needs further exploration.
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We demonstrate the slow group-velocity propagation of electromagnetic pulses through a narrow transmission band of a simple coaxial photonic crystal. The narrow transmission band was formed by creating a defect in a periodic coaxial cable filter which resulted in a narrow-frequency passband within an otherwise forbidden band stop region. Strong normal dispersion within this region causes the group velocity of the pulse to be slowed well below the speed of light and below the expected propagation speed in a coaxial cable. This phenomenon is essentially similar to the much-studied slow light propagation observed in atomic vapors through regions of strong dispersion. The simplicity with which this phenomenon can be observed in a one-dimensional coaxial photonic crystal makes this a versatile experiment for such studies. Group velocities of 0.30c, where c is the speed of light in a vacuum, were observed.
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Paradoxically, slow light promises to increase the speed of telecommunications in novel photonic structures, such as coupled resonators [1] and photonic crystals [2,3]. Apart from signal delays, the key consequence of slowing light down is the enhancement of light-matter interactions. Linear effects such as refractive index modulation scale linearly with slowdown in photonic crystals [3], and nonlinear effects are expected to scale with its square [4]. By directly observing the spatial compression of an optical pulse, by factor 25, we confirm the mechanism underlying this square scaling law. The key advantage of photonic structures over other slow light concepts is the potentially large bandwidth, which is crucial for telecommunications [5]. Nevertheless, the slow light previously observed in photonic crystals [2,3,6,7] has been very dispersive and featured narrow bandwidth. We demonstrate slow light with a bandwidth of 2.5 THz and a delay-bandwidth product of 30, which is an order of magnitude larger than any reported so far.
Subluminal and superluminal propagation of a light pulse in Kerr materials has been investigated. Group velocities as slow as much less than 1 mm per second to as fast as negative several thousands meters per second can easily be obtained in the Kerr medium, which possesses a large nonlinear refractive index and long relaxation time, such as Cr3+-doped alexandrite, ruby, and GdAlO3. The physical mechanism is the strong highly dispersive coupling between different frequency components of the pulse.
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