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Chinese Optics Letters

High-precision alkali-atom density measurement and control methods using light absorption for dual-beam SERF magnetometers

Ziao Liu, Jixi Lu, Zhaohui Hu, Xiaoyu Li, Yifan Yan, Di Zhan, Jianli Li

Published Jan 1, 2024• 9 citations
Publisher

Abstract

The alkali-atom density measurement method based on light absorption is highly suitable for a spin-exchange relaxationfree (SERF) atomic magnetometer because of its high-precision measurement and complete nonmagnetic interference.In this study, the optical rotation angle detection system based on polarization balance detection is utilized to realize the alkali-atom density real-time measurement without affecting magnetic field measurement.We discovered that there exists an optimal frequency detuning of the probe light, which offers the highest sensitivity in alkali-atom density measurement and the lowest susceptibility to temperature fluctuations in terms of the scale factor.In contrast to conventional light absorption measurements based on pump light, this method demonstrated a threefold improvement in alkali-atom density measurement sensitivity while remaining immune to ambient magnetic fields and incident light intensity fluctuations.Furthermore, we utilized this method to achieve closed-loop temperature control with an accuracy of 0.04°C.

DOI
10.3788/col202422.051201

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The alkali-atom density measurement method based on light absorption is highly suitable for a spin-exchange relaxationfree (SERF) atomic magnetometer because of its high-precision measurement and complete nonmagnetic interference.In this study, the optical rotation angle detection system based on polarization balance detection is utilized to realize the alkali-atom density real-time measurement without affecting magnetic field measurement.We discovered that there exists an optimal frequency detuning of the probe light, which offers the highest sensitivity in alkali-atom density measurement and the lowest susceptibility to temperature fluctuations in terms of the scale factor.In contrast to conventional light absorption measurements based on pump light, this method demonstrated a threefold improvement in alkali-atom density measurement sensitivity while remaining immune to ambient magnetic fields and incident light intensity fluctuations.Furthermore, we utilized this method to achieve closed-loop temperature control with an accuracy of 0.04°C.
The atomic density of an alkali vapor cell is a critical factor in determining the performance of atomic magnetometers. This paper presents a novel method to detect the density of an alkali atomic ensemble under arbitrary polarization states. By establishing a comprehensive model that correlates the absorption spectrum with the incident light’s polarization, our approach enables real-time and flexible measurements across varying temperatures and polarization angles. Experimental validations are conducted by systematically rotating a quarter-wave plate and controlling the vapor cell temperature, thereby collecting transmission spectra at multiple polarizations. The results demonstrate that the proposed method simplifies density measurements while preserving high accuracy, laying a solid foundation for further research on Spin-Exchange Relaxation-Free (SERF) atomic magnetometers. This technique serves as a versatile and effective tool for in-situ monitoring of alkali metal vapor density in various sensor applications.
High sensitivity measurements of inertia and magnetic field could be achieved by utilizing a category of devices, which manipulate the atomic spins in the spin-exchange-relaxation-free regime. The alkali cell which contains the alkali metal vapor is used to sense magnetic field and inertia. The atomic number density of alkali vapor and the polarization of alkali metal vapor are two of the most important parameters of the cell. They play an important role in the research on atomic spins in the spin-exchange-relaxation-free regime. Besides, optical polarization plays an important role in quantum computing and atomic physics. We propose a measurement of alkali vapor polarization and alkali number density by detecting the optical rotation in one system. This method simplifies existing experimental equipment and processes. A constant bias magnetic field is applied and the Faraday rotation angle is detected by a bunch of the probe beam to deduce alkali-metal density. Then the magnetic field is closed and a bunch of the pump laser is utilized to polarize alkali-metal. Again, the probe beam is utilized to obtain the polarization of alkali metal. The alkali density obtained at first is used to deduce the polarization. This paper applies a numerical method to analyze the Faraday rotation and the polarization rotation. According to the numerical method, the optimal wavelength for the experiment is given. Finally, the fluctuation of magnetic field and wavelength on signal analysis are analyzed.
The number density of alkali atoms in vaper cell is an important parameter for atomic magnetometer. The vapor cell is usually heated to a high temperature for the number density exceed to 1018m−3to achieve the spin-exchange-relaxation-free (SERF) process. The optical rotation of multichannel atomic magnetometers is affected by the number density distribution. We present an effective method for monitoring and analyzing the spatial distribution homogeneity of the atomic number density in the alkali metal cell within the SERF magnetometer. The numerical results from researching the model of electric heating films and ovens show that the temperature gradient increases with an increase in the cell temperature. This causes an nonuniform number density distribution based on the saturated vapor pressure curve. We present a laser absorption spectroscopy method by using the high-resolution beam profiling camera to record the power of the beam before and after the cell. An optimized optical system of the atomic magnetometer has been established by measuring the the number density variation in the spatial distribution in mm scale. The number density variation coefficient, which is introduced to evaluate the distribution homogeneity, increases from 0.0257 to 0.0333 when the temperature of the oven wall rises from 140°C to 190 °C, showing the same trend as the simulation results. The optical rotation distribution is calculated according to the magnetometer output signal formula. This study is of great interest for optimizing the oven structure and improving the stability of atomic spin polarization and sensitivity of the multichannel magnetometer.
Abstract A single-beam spin-exchange relaxation-free (SERF) atomic magnetometer can extract vector magnetic field information by detecting the transmission intensity of a resonant circularly polarized pumping beam, which depends sensitively on the atomic density of the alkali metal. We present a novel scheme to determine atomic density based on zero-field magnetic resonance. The resonance linewidth under different transverse DC magnetic fields is fitted by means of a quadratic function. The atomic density can be extracted from the quadratic coefficients of the fitted function. The experimental results indicate that the deviation of measured density is less than two times compared with the theoretical values between 378 K and 403 K. Furthermore, the influence of modulation field on resonance linewidth is investigated experimentally and theoretically. A miniature single-beam SERF atomic magnetometer with a sensor head volume of only 16.2 cm 3 and the measuring sensitivity of 40 fT/ Hz 1/2 has been achieved. These results should be beneficial for guiding the development of a chip-scale atomic magnetometer with high sensitivity and spatial resolution for bio-magnetic field imaging applications.
Abstract For optically pumped atomic magnetometers, the attenuation of the pumping light through the alkali-metal vapor due to light absorption is related to the number density of alkali-metal atoms. In this study, we propose an in-situ measurement and control method of atomic number density based on light absorption in the temperature range of 60 °C–160 °C, which is a much wider temperature range than considered in previous reports. A light absorption-density model is proposed to accurately describe the relationship between the light transmittance and the atomic number density. The influence of static and oscillating magnetic fields on the atomic number density measurement is also analyzed. Based on this model, a close-loop system is constructed to control the atomic number density using an electric heater. The experimental results exhibit that the proposed method can limit the fluctuation of the atomic number density in the range of 1.4%.
The light shift in a spin-exchange relaxation-free (SERF) atomic magnetometer (AM) generated by detuning of circularly polarized pump light, results in deviations of orthogonality measurement and attenuation of magnetometer response. In this paper, we propose and systematically investigate a dual-axis method to suppress light shift based on a self-developed single-beam compact SERF AM capable of measuring magnetic field components along two orthogonal sensitive axes. By sequentially observing the non-sensitive axis response and applying a magnetic field along the pump light direction, the virtual magnetic field induced by light shift is compensated and is rigorously demonstrated as a dominant component in this direction. Experimental results show a significant reduction in crosstalk between the dual sensitive axes, improving accuracy in resonant frequency determination of87Rb atoms and orthogonality evaluation of triaxial coils. Furthermore, the performance of dual-axis measurement in the SERF AM is tested, showing a more notable enhancement than that of single-axis measurement.