Excitons-polaritons of semiconductor microcavities are quasiparticles originating from the dressing of optical cavity photons by the interactions between quantum well electron-hole pairs. In planar geometry, their belonging to the family of quantum fluids has been many times demonstrated through the observation of macroscopic coherence phenomena, such as superfluidity and Bose-Einstein condensation. Like ultracold atoms, polaritons support on their surface a set of collective excitations, the Bogoliubov modes, whose spectrum encompasses the key information to describe the dynamics of quantum fluids. In this thesis, we present a wide variety of results concerning the detection and control of such modes in different configurations. Thanks to the development of a new high-resolution coherent spectroscopy method, we carried out a detailed study of the spectrum of polariton collective excitations. In particular, we highlighted the effects of the driven-dissipative nature of the system on the fundamental dynamics of the fluid, by investigating the interplay between the Bogoliubov modes and the polariton bistability under coherent pumping. This was the opportunity to reveal, in addition to the well-known phonon-type excitations, precursors of dynamical instability and the so-called ghost branch. Moreover, we studied the behavior of out-of-equilibrium phase transitions: first, via the effect of the system dimension on the bistability and, second, with the onset of a Goldstone mode, as a result of a spontaneous symmetry breaking in a parametric oscillation regime. Finally, we designed a pumping geometry that directly controls the instability modes between dark solitons of a pair guided by an intensity channel, leading to the formation of vortex-antivortex streets in the density.
Excitons-polaritons of semiconductor microcavities are quasiparticles originating from the dressing of optical cavity photons by the interactions between quantum well electron-hole pairs. In planar geometry, their belonging to the family of quantum fluids has been many times demonstrated through the observation of macroscopic coherence phenomena, such as superfluidity and Bose-Einstein condensation. Like ultracold atoms, polaritons support on their surface a set of collective excitations, the Bogoliubov modes, whose spectrum encompasses the key information to describe the dynamics of quantum fluids. In this thesis, we present a wide variety of results concerning the detection and control of such modes in different configurations. Thanks to the development of a new high-resolution coherent spectroscopy method, we carried out a detailed study of the spectrum of polariton collective excitations. In particular, we highlighted the effects of the driven-dissipative nature of the system on the fundamental dynamics of the fluid, by investigating the interplay between the Bogoliubov modes and the polariton bistability under coherent pumping. This was the opportunity to reveal, in addition to the well-known phonon-type excitations, precursors of dynamical instability and the so-called ghost branch. Moreover, we studied the behavior of out-of-equilibrium phase transitions: first, via the effect of the system dimension on the bistability and, second, with the onset of a Goldstone mode, as a result of a spontaneous symmetry breaking in a parametric oscillation regime. Finally, we designed a pumping geometry that directly controls the instability modes between dark solitons of a pair guided by an intensity channel, leading to the formation of vortex-antivortex streets in the density.
Spectroscopie cohérente haute résolution d'un fluide de polariton : modes de Bogoliubov, transitions de phase hors équilibre et turbulences Les exciton-polaritons de microcavités semiconductrices sont des quasiparticules résultant de l'habillement de photons de cavité optique par les paires d'électron-trou de puits quantique. En géométrie planaire, leur appartenance à la famille des fluides quantiques a été prouvée maintes fois à travers les observations de phénomènes de cohérence à l'échelle macroscopique, tels que la superfluidité et la condensation de Bose-Einstein. À l'instar des atomes ultrafroids, les polaritons supportent à leur surface un ensemble d'excitations collectives, les modes de Bogoliubov, dont les spectres incorporent les informations clés pour décrire les dynamiques des fluides quantiques. Dans cette thèse, nous présentons une large variété de résultats au sujet de la détection et le contrôle de tels modes dans différentes configurations. Grâce au développement d'une nouvelle méthode de spectroscopie cohérente haute-résolution, nous avons mené une étude détaillée du spectre des excitions collectives des polaritons. En particulier, nous avons révélé l'impact de la nature forcée-dissipative du système sur les dynamiques fondamentales du fluide, en examinant la relation entre les modes de Bogoliubov et la bistabilité polaritonique en pompage cohérent. Ceci nous a conduits à observer, en plus des excitations soniques bien connues des superfluides, des modes précurseurs d'instabilités et la branche fantôme. Qui plus est, nous avons étudié le comportement de transitions de phase hors-équilibres: d'abord, via les effets de la dimension du système sur la bistabilité; puis, avec la génération d'un mode de Goldstone, en conséquence d'une rupture spontanée de symétrie en régime d'oscillation paramétrique. Finalement, nous avons conçu une géométrie de pompage qui permet le contrôle direct des modes d'instabilités entre des solitons sombres d'une paire guidée par un canal d'intensité et menant à la formation d'une avenue de vortex-antivortex dans la densité du fluide.
The main scope of this thesis is the investigation of quantum properties of nonlinear, dissipative, optical and condensed matter systems. Compared with previous studies on this subjects, we reached several milestone of general interests for the theoretical and experimental community. \nThe main experimental platform we refer to in this thesis is microcavity polaritons: polaritons arise from the coupling of light with excitons in a quantum well, i.e., a 2D semiconductor material embedded in the microcavity. They have attracted the interest of the scientific community for their rich physics. Polaritons can form out-of-equilibrium Bose-Einstein condensates, they can experience superfluid phase transition and, due to their interaction via the excitonic component, they show a variety of phenomena which are typical of nonlinear physics, such as bistability and parametric scattering. \nIn particular, motivated by recent proposals about the generation of single photons from weakly nonlinear system, like the unconventional photon blockade, and by the production of squeezed states in polariton systems, we studied the possibility of obtaining antibunched light and other quantum states (like squeezed states and entangled states), when the nonlinear system shows some peculiar features: in particular we consider polariton soliton and cascade systems. \nFinally, when considering nonlinear incoherent processes, we investigate the effect of the PT-symmetry and the PT-symmetry breaking on the quantum state of the emitted light. \nHence, this research work has two main objectives: first, from the fundamental physics point of view, to understand the interplay between nonlinear phenomena and quantum optics, second to provide useful tools for future technological applications. Specifically, for the latter case, we demonstrate a theorem that links the measurement of intensity correlations with the occurrence of certain phase transitions, and we propose a setup to maximize the non-classicality of the light emitted by weakly non-linear systems via a cascade configuration. \n \n \n
Motivated by recent experiments on light-matter interacting systems, we investigate a dilute Bose gas and self-bound quantum droplets in a one-dimensional optical lattice coupled to a lossy cavity mode. Using a classical-field approach, we determine the stationary states and collective excitations of this non-equilibrium system. Apart from the usual Bogoliubov modes, we identify a polariton-like gapped excitation, the frequency of which softens as a precursor of the density ordering transition. Moreover, its relaxation time diverges as the critical point is approached, signaling the non-equilibrium nature of this transition. Dynamically, this polariton-like mode can be probed by inducing cavity field fluctuations, which in turn generates spatio-temporal oscillations of both the condensate and droplet states. In the droplet regime, we also analyze the bound modes which bear the characteristics of such non-equilibrium self-bound state. In addition, we uncover solitonic non-equilibrium states, including condensate with kink-like configuration and double-droplet state, and investigate their robustness following a sudden quench. Remarkably, although these states become unstable beyond a critical coupling, they continue to manifest in the dynamics, akin to the scarring phenomena. Our results demonstrate that dissipative cavity coupling provides a versatile route for exploring rich non-equilibrium dynamics of condensates and quantum droplets within experimentally accessible settings.
A transient spectroscopy technique for studying near-condensate modes of exciton polaritons in high-quality-factor planar semiconductor microcavities is proposed. It is demonstrated that, under the conditions of coherent external pumping, the transition to the upper steady state of an optically bistable condensate is accompanied by the excitation of near-condensate modes. They manifest themselves in the appearance of transient oscillations of the polariton intensity as the system switches to the upper branch of the S-shaped bistable pump dependence of the intensity. Analysis of the time-resolved spectra of these oscillations provides information on interactions in the system and the evolution of the exciton-polariton condensate density.
A quantum fluid passing an obstacle behaves differently from a classical one. When the flow is slow enough, the quantum gas enters a superfluid regime, and neither whirlpools nor waves form around the obstacle. For higher flow velocities, it has been predicted that the perturbation induced by the defect gives rise to the turbulent emission of quantized vortices and to the nucleation of solitons. Using an interacting Bose gas of exciton-polaritons in a semiconductor microcavity, we report the transition from superfluidity to the hydrodynamic formation of oblique dark solitons and vortex streets in the wake of a potential barrier. The direct observation of these topological excitations provides key information on the mechanisms of superflow and shows the potential of polariton condensates for quantum turbulence studies.
Abstract Superfluidity, first discovered in liquid 4He, is closely related to Bose–Einstein condensation (BEC) phenomenon. However, even at zero temperature, a fraction of the quantum liquid is excited out of the condensate into higher momentum states via interaction-induced fluctuations—the phenomenon of quantum depletion. Quantum depletion of atomic BECs in thermal equilibrium is well understood theoretically but is difficult to measure. This measurement is even more challenging in driven-dissipative exciton–polariton condensates, since their non-equilibrium nature is predicted to suppress quantum depletion. Here, we observe quantum depletion of a high-density exciton–polariton condensate by detecting the spectral branch of elementary excitations populated by this process. Analysis of this excitation branch shows that quantum depletion of exciton–polariton condensates can closely follow or strongly deviate from the equilibrium Bogoliubov theory, depending on the exciton fraction in an exciton polariton. Our results reveal beyond mean-field effects of exciton–polariton interactions and call for a deeper understanding of the relationship between equilibrium and non-equilibrium BECs.