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Observation of quantum depletion in a non-equilibrium exciton–polariton condensate

Maciej Pieczarka, Eliezer Estrecho, Maryam Boozarjmehr, O. Bleu, Mark Steger, Kenneth West, Loren N. Pfeiffer, David W. Snoke, Jesper Levinsen, Meera M. Parish, Andrew G. Truscott, Elena A. Ostrovskaya

Published Jan 1, 2020• 52 citations
OpenAlex

Abstract

Abstract Superfluidity, first discovered in liquid 4He, is closely related to Bose–Einstein condensation (BEC) phenomenon. However, even at zero temperature, a fraction of the quantum liquid is excited out of the condensate into higher momentum states via interaction-induced fluctuations—the phenomenon of quantum depletion. Quantum depletion of atomic BECs in thermal equilibrium is well understood theoretically but is difficult to measure. This measurement is even more challenging in driven-dissipative exciton–polariton condensates, since their non-equilibrium nature is predicted to suppress quantum depletion. Here, we observe quantum depletion of a high-density exciton–polariton condensate by detecting the spectral branch of elementary excitations populated by this process. Analysis of this excitation branch shows that quantum depletion of exciton–polariton condensates can closely follow or strongly deviate from the equilibrium Bogoliubov theory, depending on the exciton fraction in an exciton polariton. Our results reveal beyond mean-field effects of exciton–polariton interactions and call for a deeper understanding of the relationship between equilibrium and non-equilibrium BECs.

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Observation of quantum depletion in a non-equilibrium exciton–polariton condensate

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He, is closely related to Bose-Einstein condensation (BEC) phenomenon. However, even at zero temperature, a fraction of the quantum liquid is excited out of the condensate into higher momentum states via interaction-induced fluctuations-the phenomenon of quantum depletion. Quantum depletion of atomic BECs in thermal equilibrium is well understood theoretically but is difficult to measure. This measurement is even more challenging in driven-dissipative exciton-polariton condensates, since their non-equilibrium nature is predicted to suppress quantum depletion. Here, we observe quantum depletion of a high-density exciton-polariton condensate by detecting the spectral branch of elementary excitations populated by this process. Analysis of this excitation branch shows that quantum depletion of exciton-polariton condensates can closely follow or strongly deviate from the equilibrium Bogoliubov theory, depending on the exciton fraction in an exciton polariton. Our results reveal beyond mean-field effects of exciton-polariton interactions and call for a deeper understanding of the relationship between equilibrium and non-equilibrium BECs.

arXiv:1905.10511•Nature Communications•Jan 22, 2020•57 citations

Stimulated cooling in non-equilibrium Bose-Einstein condensate

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We report on the experimental observation of stimulated cooling in the non-equilibrium Bose-Einstein condensate (BEC) of weakly interacting exciton-polaritons from approximately room temperature down to 20K. By resolving the condensate in energy-momentum space and performing interferometric measurements, we distinguish the condensate from thermalized particles yet occupying excited states macroscopically. In contrast to the analytical quantum theories of non-equilibrium BEC [Shishkov et al., Phys. Rev. Lett. 128, 065301 (2022)], we observe segmentation of the particle density along the excited states into two fractions both following Bose-Einstein distribution, albeit with different effective temperatures and chemical potentials. Our results indicate that the temperature of the weakly interacting Bose gas is universally set by the density-dependent chemical potential, revealing a defining property of non-equilibrium BECs. Finally, we demonstrate that the stimulated nature of the cooling process directly governs the emergence of quantum coherence of the condensate and shapes the dissipative properties of the excited states.

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From polariton condensates to highly photonic quantum degenerate states of bosonic matter

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Bose-Einstein condensation (BEC) is a thermodynamic phase transition of an interacting Bose gas. Its key signatures are remarkable quantum effects like superfluidity and a phonon-like Bogoliubov excitation spectrum, which have been verified for atomic BECs. In the solid state, BEC of exciton-polaritons has been reported. Polaritons are strongly coupled light-matter quasiparticles in semiconductor microcavities and composite bosons. However, they are subject to dephasing and decay and need external pumping to reach a steady state. Accordingly the polariton BEC is a nonequilibrium process of a degenerate polariton gas in self-equilibrium, but out of equilibrium with the baths it is coupled to and therefore deviates from the thermodynamic phase transition seen in atomic BECs. Here we show that key signatures of BEC can even be observed without fulfilling the self-equilibrium condition in a highly photonic quantum degenerate nonequilibrium system.

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Abstract We report on the experimental observation of stimulated cooling in the non-equilibrium Bose--Einstein condensate (BEC) of weakly interacting exciton-polaritons from approximately room temperature down to 20K. Our results indicate that the temperature of the weakly interacting Bose gas is universally set by the density-dependent chemical potential, revealing a defining property of non-equilibrium BECs. We demonstrate that the stimulated nature of the cooling process directly governs the emergence of quantum coherence of the condensate and shapes the dissipative properties of the excited states.

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The experimental realization of Bose-Einstein condensation (BEC) with atoms and quasiparticles has triggered wide exploration of macroscopic quantum effects.Microcavity polaritons are of particular interest because quantum phenomena such as BEC and superfluidity can be observed at elevated temperatures.However, polariton lifetimes are typically too short to permit thermal equilibration.This has led to debate about whether polariton condensation is intrinsically a nonequilibrium effect.Here we report the first unambiguous observation of BEC of optically trapped polaritons in thermal equilibrium in a high-Q microcavity, evidenced by equilibrium Bose-Einstein distributions over broad ranges of polariton densities and bath temperatures.With thermal equilibrium established, we verify that polariton condensation is a phase transition with a well-defined density-temperature phase diagram.The measured phase boundary agrees well with the predictions of basic quantum gas theory.

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Excitons-polaritons of semiconductor microcavities are quasiparticles originating from the dressing of optical cavity photons by the interactions between quantum well electron-hole pairs. In planar geometry, their belonging to the family of quantum fluids has been many times demonstrated through the observation of macroscopic coherence phenomena, such as superfluidity and Bose-Einstein condensation. Like ultracold atoms, polaritons support on their surface a set of collective excitations, the Bogoliubov modes, whose spectrum encompasses the key information to describe the dynamics of quantum fluids. In this thesis, we present a wide variety of results concerning the detection and control of such modes in different configurations. Thanks to the development of a new high-resolution coherent spectroscopy method, we carried out a detailed study of the spectrum of polariton collective excitations. In particular, we highlighted the effects of the driven-dissipative nature of the system on the fundamental dynamics of the fluid, by investigating the interplay between the Bogoliubov modes and the polariton bistability under coherent pumping. This was the opportunity to reveal, in addition to the well-known phonon-type excitations, precursors of dynamical instability and the so-called ghost branch. Moreover, we studied the behavior of out-of-equilibrium phase transitions: first, via the effect of the system dimension on the bistability and, second, with the onset of a Goldstone mode, as a result of a spontaneous symmetry breaking in a parametric oscillation regime. Finally, we designed a pumping geometry that directly controls the instability modes between dark solitons of a pair guided by an intensity channel, leading to the formation of vortex-antivortex streets in the density.

•Nov 28, 2022•1 citation
Abstract Superfluidity, first discovered in liquid 4He, is closely related to Bose–Einstein condensation (BEC) phenomenon. However, even at zero temperature, a fraction of the quantum liquid is excited out of the condensate into higher momentum states via interaction-induced fluctuations—the phenomenon of quantum depletion. Quantum depletion of atomic BECs in thermal equilibrium is well understood theoretically but is difficult to measure. This measurement is even more challenging in driven-dissipative exciton–polariton condensates, since their non-equilibrium nature is predicted to suppress quantum depletion. Here, we observe quantum depletion of a high-density exciton–polariton condensate by detecting the spectral branch of elementary excitations populated by this process. Analysis of this excitation branch shows that quantum depletion of exciton–polariton condensates can closely follow or strongly deviate from the equilibrium Bogoliubov theory, depending on the exciton fraction in an exciton polariton. Our results reveal beyond mean-field effects of exciton–polariton interactions and call for a deeper understanding of the relationship between equilibrium and non-equilibrium BECs.
He, is closely related to Bose-Einstein condensation (BEC) phenomenon. However, even at zero temperature, a fraction of the quantum liquid is excited out of the condensate into higher momentum states via interaction-induced fluctuations-the phenomenon of quantum depletion. Quantum depletion of atomic BECs in thermal equilibrium is well understood theoretically but is difficult to measure. This measurement is even more challenging in driven-dissipative exciton-polariton condensates, since their non-equilibrium nature is predicted to suppress quantum depletion. Here, we observe quantum depletion of a high-density exciton-polariton condensate by detecting the spectral branch of elementary excitations populated by this process. Analysis of this excitation branch shows that quantum depletion of exciton-polariton condensates can closely follow or strongly deviate from the equilibrium Bogoliubov theory, depending on the exciton fraction in an exciton polariton. Our results reveal beyond mean-field effects of exciton-polariton interactions and call for a deeper understanding of the relationship between equilibrium and non-equilibrium BECs.
We report on the experimental observation of stimulated cooling in the non-equilibrium Bose-Einstein condensate (BEC) of weakly interacting exciton-polaritons from approximately room temperature down to 20K. By resolving the condensate in energy-momentum space and performing interferometric measurements, we distinguish the condensate from thermalized particles yet occupying excited states macroscopically. In contrast to the analytical quantum theories of non-equilibrium BEC [Shishkov et al., Phys. Rev. Lett. 128, 065301 (2022)], we observe segmentation of the particle density along the excited states into two fractions both following Bose-Einstein distribution, albeit with different effective temperatures and chemical potentials. Our results indicate that the temperature of the weakly interacting Bose gas is universally set by the density-dependent chemical potential, revealing a defining property of non-equilibrium BECs. Finally, we demonstrate that the stimulated nature of the cooling process directly governs the emergence of quantum coherence of the condensate and shapes the dissipative properties of the excited states.
Bose-Einstein condensation (BEC) is a thermodynamic phase transition of an interacting Bose gas. Its key signatures are remarkable quantum effects like superfluidity and a phonon-like Bogoliubov excitation spectrum, which have been verified for atomic BECs. In the solid state, BEC of exciton-polaritons has been reported. Polaritons are strongly coupled light-matter quasiparticles in semiconductor microcavities and composite bosons. However, they are subject to dephasing and decay and need external pumping to reach a steady state. Accordingly the polariton BEC is a nonequilibrium process of a degenerate polariton gas in self-equilibrium, but out of equilibrium with the baths it is coupled to and therefore deviates from the thermodynamic phase transition seen in atomic BECs. Here we show that key signatures of BEC can even be observed without fulfilling the self-equilibrium condition in a highly photonic quantum degenerate nonequilibrium system.
Abstract We report on the experimental observation of stimulated cooling in the non-equilibrium Bose--Einstein condensate (BEC) of weakly interacting exciton-polaritons from approximately room temperature down to 20K. Our results indicate that the temperature of the weakly interacting Bose gas is universally set by the density-dependent chemical potential, revealing a defining property of non-equilibrium BECs. We demonstrate that the stimulated nature of the cooling process directly governs the emergence of quantum coherence of the condensate and shapes the dissipative properties of the excited states.
The experimental realization of Bose-Einstein condensation (BEC) with atoms and quasiparticles has triggered wide exploration of macroscopic quantum effects.Microcavity polaritons are of particular interest because quantum phenomena such as BEC and superfluidity can be observed at elevated temperatures.However, polariton lifetimes are typically too short to permit thermal equilibration.This has led to debate about whether polariton condensation is intrinsically a nonequilibrium effect.Here we report the first unambiguous observation of BEC of optically trapped polaritons in thermal equilibrium in a high-Q microcavity, evidenced by equilibrium Bose-Einstein distributions over broad ranges of polariton densities and bath temperatures.With thermal equilibrium established, we verify that polariton condensation is a phase transition with a well-defined density-temperature phase diagram.The measured phase boundary agrees well with the predictions of basic quantum gas theory.
Excitons-polaritons of semiconductor microcavities are quasiparticles originating from the dressing of optical cavity photons by the interactions between quantum well electron-hole pairs. In planar geometry, their belonging to the family of quantum fluids has been many times demonstrated through the observation of macroscopic coherence phenomena, such as superfluidity and Bose-Einstein condensation. Like ultracold atoms, polaritons support on their surface a set of collective excitations, the Bogoliubov modes, whose spectrum encompasses the key information to describe the dynamics of quantum fluids. In this thesis, we present a wide variety of results concerning the detection and control of such modes in different configurations. Thanks to the development of a new high-resolution coherent spectroscopy method, we carried out a detailed study of the spectrum of polariton collective excitations. In particular, we highlighted the effects of the driven-dissipative nature of the system on the fundamental dynamics of the fluid, by investigating the interplay between the Bogoliubov modes and the polariton bistability under coherent pumping. This was the opportunity to reveal, in addition to the well-known phonon-type excitations, precursors of dynamical instability and the so-called ghost branch. Moreover, we studied the behavior of out-of-equilibrium phase transitions: first, via the effect of the system dimension on the bistability and, second, with the onset of a Goldstone mode, as a result of a spontaneous symmetry breaking in a parametric oscillation regime. Finally, we designed a pumping geometry that directly controls the instability modes between dark solitons of a pair guided by an intensity channel, leading to the formation of vortex-antivortex streets in the density.