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Japanese Journal of Applied Physics

Demonstrating long-term stable optical coupling between single-mode optical fibers and well-defined energy photons emitted from nitrogen impurity centers in GaAs flakes

Takayuki Ishida, Yoshiki Sakuma, Michio Ikezawa

Published Oct 13, 2023• 1 citation
Publisher

Abstract

Abstract A key challenge in realizing scalable optical quantum information technology is not only to obtain stable single photons coupled to single-mode fibers but also to match the emission energy between remote emitters. We have fabricated an energy-matching favorable and long-term stable structure by coupling a nitrogen impurity center with a well-defined emission energy to a single-mode optical fiber core. The nitrogen-doped GaAs microflakes sandwiched between the two FC (acronym for "ferrule connector" or "fiber channel") connectors yielded sharp emission peaks due to nitrogen isoelectronic traps. Although some emitters showed spectral diffusion, the unaffected emitters showed stable emission and were able to generate photons stably for over 20 h continuously without photodegradation. In addition, the photoluminescence spectrum does not change in shape and intensity after more than 3 years, indicating that the photon source with this structure is resistant to thermal cycling and positional drift and has excellent long-term stability.

DOI
10.35848/1347-4065/ad034e

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Abstract A key challenge in realizing scalable optical quantum information technology is not only to obtain stable single photons coupled to single-mode fibers but also to match the emission energy between remote emitters. We have fabricated an energy-matching favorable and long-term stable structure by coupling a nitrogen impurity center with a well-defined emission energy to a single-mode optical fiber core. The nitrogen-doped GaAs microflakes sandwiched between the two FC (acronym for "ferrule connector" or "fiber channel") connectors yielded sharp emission peaks due to nitrogen isoelectronic traps. Although some emitters showed spectral diffusion, the unaffected emitters showed stable emission and were able to generate photons stably for over 20 h continuously without photodegradation. In addition, the photoluminescence spectrum does not change in shape and intensity after more than 3 years, indicating that the photon source with this structure is resistant to thermal cycling and positional drift and has excellent long-term stability.
We studied optical properties of isoelectronic traps in nitrogen δ-doped GaAs by micro-photoluminescence (µ-PL) spectroscopy. We found that these nitrogen impurity centers (NNA) emit photons with nearly identical emission energy at 1475 meV and polarization direction. Furthermore, single photon generation from a single impurity center was confirmed by a strong photon antibunching under the continuous optical excitation at 5 K. Our results suggest that the nitrogen impurity center in GaAs might be well suited for the energetically-defined single photon source for the quantum information application.
We studied optical properties of isoelectronic traps in nitrogen δ-doped GaAs by micro-photoluminescence (µ-PL) spectroscopy. We found that these nitrogen impurity centers (NNA) emit photons with nearly identical emission energy at 1475 meV and polarization direction. Furthermore, single photon generation from a single impurity center was confirmed by a strong photon antibunching under the continuous optical excitation at 5 K. Our results suggest that the nitrogen impurity center in GaAs might be well suited for the energetically-defined single photon source for the quantum information application.
Abstract In this work, we present a stand-alone and fiber-coupled quantum-light source. The plug-and-play device is based on an optically driven quantum dot delivering single photons via an optical fiber. The quantum dot is deterministically integrated in a monolithic microlens which is precisely coupled to the core of an optical fiber via active optical alignment and epoxide adhesive bonding. The rigidly coupled fiber-emitter assembly is integrated in a compact Stirling cryocooler with a base temperature of 35 K. We benchmark our practical quantum device via photon auto-correlation measurements revealing g(2)(0) = 0.07 ± 0.05 under continuous-wave excitation and we demonstrate triggered non-classical light at a repetition rate of 80 MHz. The long-term stability of our quantum light source is evaluated by endurance tests showing that the fiber-coupled quantum dot emission is stable within 4% over several successive cool-down/warm-up cycles. Additionally, we demonstrate non-classical photon emission for a user-intervention-free 100-hour test run and stable single-photon count rates up to 11.7 kHz with a standard deviation of 4%.
Nitrogen-Vacancy (NV) centers in diamond are promising solid-state quantum emitters that can be utilized for photonic quantum applications. Various diamond nanophotonic devices have been fabricated for efficient extraction of single photons emitted from NV centers to a single guided mode. However, for constructing scalable quantum networks, further efficient coupling of single photons to a guided mode of a single-mode fiber (SMF) is indispensable and a difficult challenge. Here, we propose a novel efficient hybrid system between an optical nanofiber and a cylindrical-structured diamond nanowire. The maximum coupling efficiency as high as 75% for the sum of both fiber ends is obtained by numerical simulations. The proposed hybrid system will provide a simple and efficient interface between solid-state quantum emitters and a SMF suitable for constructing scalable quantum networks.
Miniaturization of quantum optical devices down to μm-dimensions and integration into fibre optical networks is a major prerequisite for future implementations of quantum information communication and processing applications. Also scalability, long-term stability and room-temperature operation are important properties of such devices. Lately there have been major improvements in down-sizing logical structures and functionalizing optical fibers. Here we present an alignment free, μm-scale single photon source consisting of a single quantum emitter on an optical fiber operating at room temperature. It easily integrates into fiber optic networks for quantum cryptography or quantum metrology applications. Near-field coupling of a single nitrogen-vacancy center is achieved in a bottom-up approach by placing a pre-selected nanodiamond directly on the fiber facet. Its high photon collection efficiency is equivalent to a far-field collection via an objective with a numerical aperture of 0.82. Furthermore, simultaneous excitation and recollection through the fiber is possible introducing a fiber-connected single emitter sensor that allows near-field probing with quantum mechanical properties.
Luminescence from single isoelectronic traps in nitrogen δ-doped gallium phosphide was studied by micro-photoluminescence spectroscopy. These single traps were found to emit photons that were nearly identical in both emission energy and brightness. Furthermore, single photon emission from a single nitrogen pair is confirmed by a strong antibunching under continuous optical excitation at 30 K. These results imply that single nitrogen pairs in GaP might be useful for realizing unique sources of energetically-defined single photons, and even indistinguishable photons.