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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Entanglement-Enhanced Frequency Comparison of Two Optical Atomic Clocks

B. C. Nichol, R. Srinivas, D. P. Nadlinger, P. Drmota, D. Main, G. Araneda, Christopher J. Ballance, D. M. Lucas

Published Jun 26, 2023• 1 citation
Publisher

Abstract

Optical atomic clocks are our most precise tools to measure time and frequency [1]–[3]. They enable precision frequency comparisons between atoms in separate locations to probe the space-time variation of fundamental constants [4] and the properties of dark matter [5], [6], to perform geodesy [4], [7], [8] and to evaluate systematic clock shifts. Measurements on independent systems are limited by the standard quantum limit (SQL); measurements on entangled systems, in contrast, can surpass the SQL to reach the ultimate precision allowed by quantum theory - the so-called Heisenberg limit. While local entangling operations have been used to demonstrate this enhancement at microscopic distances [9]–[14], frequency comparisons between remote atomic clocks require rapid high-fidelity entanglement between separate systems that have no intrinsic interactions.

DOI
10.1109/cleo/europe-eqec57999.2023.10232118

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Optical atomic clocks are our most precise tools to measure time and frequency [1]–[3]. They enable precision frequency comparisons between atoms in separate locations to probe the space-time variation of fundamental constants [4] and the properties of dark matter [5], [6], to perform geodesy [4], [7], [8] and to evaluate systematic clock shifts. Measurements on independent systems are limited by the standard quantum limit (SQL); measurements on entangled systems, in contrast, can surpass the SQL to reach the ultimate precision allowed by quantum theory - the so-called Heisenberg limit. While local entangling operations have been used to demonstrate this enhancement at microscopic distances [9]–[14], frequency comparisons between remote atomic clocks require rapid high-fidelity entanglement between separate systems that have no intrinsic interactions.
Optical atomic clocks with unrivaled precision and accuracy have advanced the frontier of precision measurement science and opened new avenues for exploring fundamental physics. A fundamental limitation on clock precision is the standard quantum limit (SQL), which stems from the uncorrelated projection noise of each atom. State-of-the-art optical lattice clocks interrogate large ensembles to minimize the SQL, but density-dependent frequency shifts pose challenges to scaling the atom number. The SQL can be surpassed, however, by leveraging entanglement, though it remains an open problem to achieve quantum advantage from spin squeezing at state-of-the-art stability levels. Here, we demonstrate clock performance beyond the SQL, achieving a fractional frequency precision of 1.1×10^{-18} for a single spin-squeezed clock. With cavity-based quantum nondemolition measurements, we prepare two spin-squeezed ensembles of ∼30 000 strontium atoms confined in a two-dimensional optical lattice. A synchronous clock comparison with an interrogation time of 61 ms achieves a metrological improvement of 2.0(2) dB beyond the SQL, after correcting for state preparation and measurement errors. These results establish the most precise entanglement-enhanced clock to date and offer a powerful platform for exploring the interplay of gravity and quantum entanglement.
Recent developments in atomic physics have enabled the experimental generation of many-body entangled states to boost the performance of quantum sensors beyond the Standard Quantum Limit (SQL). This limit is imposed by the inherent projection noise of a quantum measurement. In this Perspective article, we describe the commonly used experimental methods to create many-body entangled states to operate quantum sensors beyond the SQL. In particular, we focus on the potential of applying quantum entanglement to state-of-the-art optical atomic clocks. In addition, we present recently developed time-reversal protocols that make use of complex states with high quantum Fisher information without requiring sub-SQL measurement resolution. We discuss the prospects for reaching near-Heisenberg limited quantum metrology based on such protocols.
Optical atomic clocks that operate at frequencies up to 100,000 times higher than their microwave counterparts permit better resolutions and accuracies, while also providing more leeway in environmental control for out of lab applications. Many of the precision applications of these clocks, including relativistic geodesy and tests of fundamental physics rely on the intercomparison of at least two optical clocks. Relative comparisons that include single ion clocks, however, can require close to one month of continuous averaging to achieve measurement instabilities near 1 part in 1018. The long averaging times result from limits imposed on the quantum project noise as a result of signal detection from a single ion, as well as atom probe time limitations due to laser-atom decoherence. In this talk I will describe how the phase coherent properties of an optical frequency comb can be used to enable correlated and synchronous measurement of atomic clocks as a means to improve their relative measurement instability by close to a factor of 10, and nearly 100 times speed up in averaging time over conventional measurement techniques.
Precision navigation and timing, very-long-baseline interferometry, next-generation communication, sensing, and tests of fundamental physics all require a highly synchronized network of clocks. With the advance of highly-accurate optical atomic clocks, the precision requirements for synchronization are reaching the limits of classical physics (i.e. the standard quantum limit, SQL). Efficiently overcoming the SQL to reach the fundamental Heisenberg limit can be achieved via the use of squeezed or entangled light. Although approaches to the Heisenberg limit are well understood in theory, a practical implementation, such as in space-based platforms, requires that the advantage outweighs the added costs and complexity. Here, we focus on the question: can entanglement yield a quantum advantage in clock synchronization over lossy satellite-to-satellite channels? We answer in the affirmative, showing that the redundancy afforded by the two-mode nature of entanglement allows recoverability even over asymmetrically lossy channels. We further show this recoverability is an improvement over single-mode squeezing sensing, thereby illustrating a new complexity-performance trade-off for space-based sensing applications.
Atomic projection noise limits the ultimate precision of all atomic sensors, including clocks, inertial sensors, magnetometers, etc. The independent quantum collapse of N atoms into a definite state (for example spin up or down) leads to an uncertainty ΔθSQL= 1/√N in the estimate of the quantum phase accumulated during a Ramsey sequence or its many generalizations. This phase uncertainty is referred to as the standard quantum limit. Creating quantum entanglement between the N atoms can allow the atoms to partially cancel each other's quantum noise, leading to reduced noise in the phase estimate below the standard quantum limit. Recent experiments have demonstrated up to 10 dB of phase noise reduction relative to the SQL by making collective spin measurements. This is achieved by trapping laser-cooled Rb atoms in an optical cavity and precisely measuring the shift of the cavity resonance frequency by an amount that depends on the number of atoms in spin up. Detecting the probe light with high total efficiency reduces excess classical and quantum back-action of the probe. Here we discuss recent progress and a technique for reducing the relative frequency noise between the probe light and the optical cavity, a key requirement for further advances.
Rapid progress in the precision and accuracy of optical atomic clocks over the last decade has advanced the frontiers of timekeeping, metrology, and quantum science. However, the stabilities of most optical clocks remain limited by the local oscillator rather than the atoms themselves, leaving room for further progress. Here we implement a "multiplexed" one-dimensional optical lattice clock, in which spatially-resolved, movable ensembles of ultra-cold strontium atoms are trapped in the same optical lattice, interrogated simultaneously by a shared clock laser, and read-out in parallel. By performing synchronized Ramsey interrogations of ensemble pairs we observe atom-atom coherence times up to 26 seconds, a 270-fold improvement over the atom-laser coherence time, demonstrate a relative stability of 9.7(4)×10−18/τ9.7(4)\times10^{-18}/\sqrtτ9.7(4)×10−18/τ​ (where τττ is the averaging time in seconds), and reach a fractional uncertainty of 8.9(3)×10−208.9(3)\times 10^{-20}8.9(3)×10−20 after 3.3 hours of averaging. These results demonstrate that applications requiring ultra-high-precision comparisons between optical atomic clocks need not be limited by the stability of the local oscillator. With multiple ensemble pairs, we realize a miniaturized clock network consisting of 6 atom ensembles, resulting in 15 unique pairwise clock comparisons with relative stabilities below 3×10−17/τ3\times10^{-17}/\sqrtτ3×10−17/τ​. Finally, we demonstrate the capability to simultaneously load spatially-resolved, heterogeneous ensemble pairs of all four stable isotopes of strontium in a lattice. The unique capabilities offered by this platform pave the way for future studies of precision isotope shift measurements, spatially resolved characterization of limiting clock systematics, development of clock-based gravitational wave and dark matter detectors, and novel tests of relativity including measurements of the gravitational redshift at sub-centimeter scales.