Hong-Ou-Mandel (HOM) interferometry is a powerful quantum metrology technique to reconstruct the surface-depth profile of transparent samples with complementary benefits of measurement precision and experimental robustness. It is generally assumed that a trade-off exists between the standard HOM interferometry sensitivity and its ambiguity-free dynamic range. Here we challenge this ``well-known'' assumption through the implementation of spectrally resolved HOM interferometry with discrete color entanglement, and show that the well-separated frequencies embedded in a quantum state suffices to achieve great advantages in enhancing the temporal resolution but without limiting its ambiguity-free dynamic range. Backed by the Fisher-information analysis, spectrally resolved coincidence detection is an optimal measurement strategy as it enables us to recover the quantum Cram\'er-Rao bound. These results may significantly facilitate the use of spectrally resolved quantum interference for real-time quantum information processing, such as ultrafast phase transition and spectral-temporal photography.
Hong-Ou-Mandel (HOM) interferometry is a powerful quantum metrology technique to reconstruct the surface-depth profile of transparent samples with complementary benefits of measurement precision and experimental robustness. It is generally assumed that a trade-off exists between the standard HOM interferometry sensitivity and its ambiguity-free dynamic range. Here we challenge this ``well-known'' assumption through the implementation of spectrally resolved HOM interferometry with discrete color entanglement, and show that the well-separated frequencies embedded in a quantum state suffices to achieve great advantages in enhancing the temporal resolution but without limiting its ambiguity-free dynamic range. Backed by the Fisher-information analysis, spectrally resolved coincidence detection is an optimal measurement strategy as it enables us to recover the quantum Cram'er-Rao bound. These results may significantly facilitate the use of spectrally resolved quantum interference for real-time quantum information processing, such as ultrafast phase transition and spectral-temporal photography.
Extracting information from a fast-moving object plays a crucial role in better understanding natural phenomena and exploring the unknown world. The conventional Hong-Ou-Mandel (HOM) sensor can acquire temporal information of an object using the single-shot method. However, this method is strictly limited by the temporal resolution of coincidence detection. On the other hand, implementing a suitable quantum interferometer for tracking fast-moving objects with relatively little technological effort has long been sought after, particularly for photon-sensitive biological and chemical dynamic processes. Here, we present a fast HOM interferometer based on quantum interference on a biphoton beat note and spectrally resolved detection. To verify the feasibility of our method, we demonstrate a proof-of-principle experiment that implements a fast HOM sensor for observing the track of a moving translation stage. These results may facilitate the use of quantum interference for enhancing the temporal resolution and processing speed in a fast HOM-based sensor, which has an important scientific significance in both fundamental research and applied science.
Hong-Ou-Mandel (HOM) interferometry enables delay estimation at the quantum precision limit but is traditionally constrained to path differences within the coherence time of the interfering photons. Here, we demonstrate single-measurement path-delay sensing at the measurement Cramer-Rao bound using spectrally resolved HOM interference, thereby removing the conventional dynamic-range limitation imposed by the photon coherence window, with no scanning required for calibration. By extracting delay information from the spectral interference fringes of spectrally entangled photon pairs, we retain near-optimal sensitivity over an operational range exceeding the photon coherence time by over two orders of magnitude. Using one million detected photon pairs, we achieve a time-delay precision of 20 attosecond (6 nm), while real-time operation (at 1 Hz) yields 330 attosecond (100 nm) precision. Because the estimator relies on fringe periodicity rather than absolute coincidence rates, the method is intrinsically robust to photon losses and variations in interference visibility, eliminating the need for recalibration. As a practical demonstration, we measure the thickness of a 300 um transmissive target with nanometer-scale precision. These results mark a significant step towards deploying quantum-limited measurements in real-world sensing applications using HOM interferometry.
The Hong-Ou-Mandel (HOM) interference in the multimode frequency domain has been explored for precision metrology, with several experimental demonstrations exploiting its robustness against dispersion and phase noise, as well as its large dynamic range and compatibility with fragile samples. Conventional multimode HOM metrology exploits frequency-entangled states, which naturally satisfy bosonic exchange symmetry under any centered symmetric joint spectral distribution, to provide these advantages. However, these entangled states are typically generated via spontaneous parametric down-conversion (SPDC), requiring strong pump lasers that hinder practical implementation. In this paper, we employ frequency product states, which do not possess entanglement or path-mode exchange symmetry, as the probe state and post-select measurement outcomes exhibiting frequency anti-correlation. Our results demonstrate that these advantages,peak narrowing, dispersion cancellation, phase-noise immunity, a large dynamic range, and compatibility with fragile samples, arise neither from entanglement nor from bosonic exchange symmetry, but rather from spectral anti-correlation. We further show that entanglement is not the source of the measurement precision: the entanglement-free approach attains the same quantum Fisher information as the entangled-state scheme, indicating that the fundamental precision limit does not originate from entanglement.
We demonstrate real-time displacement measurement using spectrally resolved Hong–Ou–Mandel (HOM) interference that saturates the quantum Cram´er-Rao bound. Unlike conventional HOM-based methods, our approach does not require the displacement to be confined within the HOM dip width, typically a few tens of microns. By analyzing the periodicity of spectral interference fringes, we can maintain sensitivity at the quantum limit over displacement ranges extending to hundreds of microns. In principle, the measurable range can be extended up to the coherence length of the pump laser, limited only by the spectral resolution of the detector. We further demonstrate that real-time displacement tracking is feasible with current technology, establishing this technique as a practical and powerful tool for quantum-enhanced sensing and metrology.
Hong-Ou-Mandel (HOM) interferometry with entangled photons exhibits distinctive quantum features. By introducing frequency entanglement (discrete-color entangled states) into HOM interference, the characteristic HOM dip is modulated by sinusoidal fringes, which significantly enhance the sensitivity of HOM sensors. The frequency-entangled photon sources demonstrated to date rely on non-resonant parametric down-conversion (PDC), which limits the photon coherence length and, consequently, restricts the sensing dynamic range to the sub-millimeter scale. In this work, we demonstrate narrowband frequency-entangled photon source based on resonant PDC in a crystalline whispering gallery mode resonator. The MHz-level spectral bandwidth of photons enables a meter-scale dynamic range. With highly nondegenerate frequency-entangled photon pairs featuring a 96 THz frequency detuning, we observe high-contrast quantum beating with sub-picosecond resolution in the HOM experiment. Our WGMR-based frequency-entangled photon source has potential applications in quantum metrology and quantum information processing.
Biphoton frequency comb (BFC), which encompasses multiple discrete frequency modes and represents high-dimensional frequency entanglement, is crucial in quantum information processing due to its high information capacity and error resilience. It also holds significant potential for enhancing timing precision in quantum metrology. Here, we examine quantum metrology timing limits using the BFC as a probe state and derive a quantum Cramér-Rao bound (QCRB) that depends on the mode number, mode spacing, frequency detuning, and single-mode bandwidth. Our results coincide with previous findings that considered only the latter two factors. Under ideal conditions (zero loss and perfect visibility), this bound can be saturated by both spectrally non-resolved Hong-Ou-Mandel (HOM) interferometry at zero delay and spectrally resolved HOM interferometry at arbitrary delays. In practical scenarios, the Fisher information is below the QCRB but can approach its maximum by increasing the mode number and mode spacing for a fixed delay point, suggesting an optimal strategy for improving the precision of HOM-based sensing in practice. Furthermore, compared to spectrally non-resolved measurement, spectrally resolved measurement is a superior strategy due to its higher Fisher information, shorter measurement times, and ambiguity-free dynamic range.