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arXiv:2410.16841 · Optics Express

Quantum metrology timing limits of biphoton frequency comb

Baihong Li, Qi-qi Li, Xiao-Fei Zhang, Rui‐Bo Jin

Published Jun 25, 2025• 2 citations
arXivHTMLPDF

Abstract

Biphoton frequency comb (BFC), which encompasses multiple discrete frequency modes and represents high-dimensional frequency entanglement, is crucial in quantum information processing due to its high information capacity and error resilience. It also holds significant potential for enhancing timing precision in quantum metrology. Here, we examine quantum metrology timing limits using the BFC as a probe state and derive a quantum Cramér-Rao bound (QCRB) that depends on the mode number, mode spacing, frequency detuning, and single-mode bandwidth. Our results coincide with previous findings that considered only the latter two factors. Under ideal conditions (zero loss and perfect visibility), this bound can be saturated by both spectrally non-resolved Hong-Ou-Mandel (HOM) interferometry at zero delay and spectrally resolved HOM interferometry at arbitrary delays. In practical scenarios, the Fisher information is below the QCRB but can approach its maximum by increasing the mode number and mode spacing for a fixed delay point, suggesting an optimal strategy for improving the precision of HOM-based sensing in practice. Furthermore, compared to spectrally non-resolved measurement, spectrally resolved measurement is a superior strategy due to its higher Fisher information, shorter measurement times, and ambiguity-free dynamic range.

DOI
10.1364/oe.562859

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Biphoton frequency comb (BFC), which encompasses multiple discrete frequency modes and represents high-dimensional frequency entanglement, is crucial in quantum information processing due to its high information capacity and error resilience. It also holds significant potential for enhancing timing precision in quantum metrology. Here, we examine quantum metrology timing limits using the BFC as a probe state and derive a quantum Cramér-Rao bound (QCRB) that depends on the mode number, mode spacing, frequency detuning, and single-mode bandwidth. Our results coincide with previous findings that considered only the latter two factors. Under ideal conditions (zero loss and perfect visibility), this bound can be saturated by both spectrally non-resolved Hong-Ou-Mandel (HOM) interferometry at zero delay and spectrally resolved HOM interferometry at arbitrary delays. In practical scenarios, the Fisher information is below the QCRB but can approach its maximum by increasing the mode number and mode spacing for a fixed delay point, suggesting an optimal strategy for improving the precision of HOM-based sensing in practice. Furthermore, compared to spectrally non-resolved measurement, spectrally resolved measurement is a superior strategy due to its higher Fisher information, shorter measurement times, and ambiguity-free dynamic range.
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Quantum entanglement is a vital resource in quantum information processing. High-dimensional quantum entanglement offers advantages that classical systems cannot surpass, particularly in enhancing channel capacity, improving system noise resilience, and increasing sensitivity to external environments. The construction of multimode entanglement in the spectral domain is well-suited for fiber-optic systems. Here, we present a straightforward scheme for generating multimode frequency-bin entanglement using a semiconductor chip through a simple mode conversion. A general model for Hong–Ou–Mandel (HOM) interference with a multimode frequency-bin entangled state is presented and applied to the experiments. The multimode entangled photons we produced exhibit HOM interference with a high-visibility beating pattern, demonstrating a strong relationship with the mode number, mode spacing, and the profile of the single mode. Building on the Fisher information analysis, we explore the relationship between the features in multimode entangled state interference traces and the precision of interferometric measurements even in the presence of experimental nonidealities. This work may deepen the understanding of multimode frequency-bin entanglement and advance the application of multimode HOM interference in quantum sensing.
Hong-Ou-Mandel (HOM) interferometry is a powerful quantum metrology technique to reconstruct the surface-depth profile of transparent samples with complementary benefits of measurement precision and experimental robustness. It is generally assumed that a trade-off exists between the standard HOM interferometry sensitivity and its ambiguity-free dynamic range. Here we challenge this ``well-known'' assumption through the implementation of spectrally resolved HOM interferometry with discrete color entanglement, and show that the well-separated frequencies embedded in a quantum state suffices to achieve great advantages in enhancing the temporal resolution but without limiting its ambiguity-free dynamic range. Backed by the Fisher-information analysis, spectrally resolved coincidence detection is an optimal measurement strategy as it enables us to recover the quantum Cram\'er-Rao bound. These results may significantly facilitate the use of spectrally resolved quantum interference for real-time quantum information processing, such as ultrafast phase transition and spectral-temporal photography.
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Hong-Ou-Mandel (HOM) interferometry enables delay estimation at the quantum precision limit but is traditionally constrained to path differences within the coherence time of the interfering photons. Here, we demonstrate single-measurement path-delay sensing at the measurement Cramer-Rao bound using spectrally resolved HOM interference, thereby removing the conventional dynamic-range limitation imposed by the photon coherence window, with no scanning required for calibration. By extracting delay information from the spectral interference fringes of spectrally entangled photon pairs, we retain near-optimal sensitivity over an operational range exceeding the photon coherence time by over two orders of magnitude. Using one million detected photon pairs, we achieve a time-delay precision of 20 attosecond (6 nm), while real-time operation (at 1 Hz) yields 330 attosecond (100 nm) precision. Because the estimator relies on fringe periodicity rather than absolute coincidence rates, the method is intrinsically robust to photon losses and variations in interference visibility, eliminating the need for recalibration. As a practical demonstration, we measure the thickness of a 300 um transmissive target with nanometer-scale precision. These results mark a significant step towards deploying quantum-limited measurements in real-world sensing applications using HOM interferometry.