Quantum entanglement is a vital resource in quantum information processing. High-dimensional quantum entanglement offers advantages that classical systems cannot surpass, particularly in enhancing channel capacity, improving system noise resilience, and increasing sensitivity to external environments. The construction of multimode entanglement in the spectral domain is well-suited for fiber-optic systems. Here, we present a straightforward scheme for generating multimode frequency-bin entanglement using a semiconductor chip through a simple mode conversion. A general model for Hong–Ou–Mandel (HOM) interference with a multimode frequency-bin entangled state is presented and applied to the experiments. The multimode entangled photons we produced exhibit HOM interference with a high-visibility beating pattern, demonstrating a strong relationship with the mode number, mode spacing, and the profile of the single mode. Building on the Fisher information analysis, we explore the relationship between the features in multimode entangled state interference traces and the precision of interferometric measurements even in the presence of experimental nonidealities. This work may deepen the understanding of multimode frequency-bin entanglement and advance the application of multimode HOM interference in quantum sensing.
Quantum entanglement is a vital resource in quantum information processing. High-dimensional quantum entanglement offers advantages that classical systems cannot surpass, particularly in enhancing channel capacity, improving system noise resilience, and increasing sensitivity to external environments. The construction of multimode entanglement in the spectral domain is well-suited for fiber-optic systems. Here, we present a straightforward scheme for generating multimode frequency-bin entanglement using a semiconductor chip through a simple mode conversion. A general model for Hong–Ou–Mandel (HOM) interference with a multimode frequency-bin entangled state is presented and applied to the experiments. The multimode entangled photons we produced exhibit HOM interference with a high-visibility beating pattern, demonstrating a strong relationship with the mode number, mode spacing, and the profile of the single mode. Building on the Fisher information analysis, we explore the relationship between the features in multimode entangled state interference traces and the precision of interferometric measurements even in the presence of experimental nonidealities. This work may deepen the understanding of multimode frequency-bin entanglement and advance the application of multimode HOM interference in quantum sensing.
The Hong-Ou-Mandel (HOM) interference in the multimode frequency domain has been explored for precision metrology, with several experimental demonstrations exploiting its robustness against dispersion and phase noise, as well as its large dynamic range and compatibility with fragile samples. Conventional multimode HOM metrology exploits frequency-entangled states, which naturally satisfy bosonic exchange symmetry under any centered symmetric joint spectral distribution, to provide these advantages. However, these entangled states are typically generated via spontaneous parametric down-conversion (SPDC), requiring strong pump lasers that hinder practical implementation. In this paper, we employ frequency product states, which do not possess entanglement or path-mode exchange symmetry, as the probe state and post-select measurement outcomes exhibiting frequency anti-correlation. Our results demonstrate that these advantages,peak narrowing, dispersion cancellation, phase-noise immunity, a large dynamic range, and compatibility with fragile samples, arise neither from entanglement nor from bosonic exchange symmetry, but rather from spectral anti-correlation. We further show that entanglement is not the source of the measurement precision: the entanglement-free approach attains the same quantum Fisher information as the entangled-state scheme, indicating that the fundamental precision limit does not originate from entanglement.
Hong–Ou–Mandel (HOM) interferometry with entangled photons exhibits distinctive quantum features. By introducing frequency entanglement (discrete-color entangled states) into HOM interference, the characteristic HOM dip is modulated by sinusoidal fringes, which significantly enhances the sensitivity of HOM sensors. The frequency-entangled photon sources demonstrated to date rely on non-resonant parametric down-conversion (PDC), which limits the photon coherence length and, consequently, restricts the sensing dynamic range to the millimeter scale. In this work, we demonstrate narrowband frequency-entangled photon source based on resonant PDC in a crystalline whispering gallery mode resonator. The MHz-level spectral bandwidth of photons enables a meter-scale dynamic range. With highly nondegenerate frequency-entangled photon pairs featuring a 96 THz frequency detuning, we observe high-contrast quantum beating with sub-picosecond resolution in the HOM experiment. Our WGMR-based frequency-entangled photon source has potential applications in quantum metrology and quantum information processing.
Hong-Ou-Mandel (HOM) interferometry with entangled photons exhibits distinctive quantum features. By introducing frequency entanglement (discrete-color entangled states) into HOM interference, the characteristic HOM dip is modulated by sinusoidal fringes, which significantly enhance the sensitivity of HOM sensors. The frequency-entangled photon sources demonstrated to date rely on non-resonant parametric down-conversion (PDC), which limits the photon coherence length and, consequently, restricts the sensing dynamic range to the sub-millimeter scale. In this work, we demonstrate narrowband frequency-entangled photon source based on resonant PDC in a crystalline whispering gallery mode resonator. The MHz-level spectral bandwidth of photons enables a meter-scale dynamic range. With highly nondegenerate frequency-entangled photon pairs featuring a 96 THz frequency detuning, we observe high-contrast quantum beating with sub-picosecond resolution in the HOM experiment. Our WGMR-based frequency-entangled photon source has potential applications in quantum metrology and quantum information processing.
The Hong-Ou-Mandel interferometer is a versatile tool for analyzing the joint properties of photon pairs, relying on a truly quantum interference effect between two-photon probability amplitudes. While the theory behind this form of two-photon interferometry is well established, the development of advanced photon sources and exotic two-photon states has highlighted the importance of quantifying precisely what information can and cannot be inferred from features in a Hong-Ou-Mandel interference trace. Here we examine Hong-Ou-Mandel interference with regard to a particular class of states, so-called quantum frequency combs, and place special emphasis on the role spectral phase plays in these measurements. We find that this form of two-photon interferometry is insensitive to the relative phase between different comb line pairs. This is true even when different comb line pairs are mutually coherent at the input of a Hong-Ou-Mandel interferometer and the fringe patterns display sharp temporal features. Consequently, Hong-Ou-Mandel interference cannot speak to the presence of high-dimensional frequency-bin entanglement in two-photon quantum frequency combs.
High-dimensional, frequency-entangled photonic quantum bits (qudits for d -dimension) are promising resources for quantum information processing in an optical fiber network and can also be used to improve channel capacity and security for quantum communication. However, up to now, it is still challenging to prepare high-dimensional frequency-entangled qudits in experiments, due to technical limitations. Here we propose and experimentally implement a novel method for a simple generation of frequency-entangled qudts with without the use of any spectral filters or cavities. The generated state is distributed over 15 km in total length. This scheme combines the technique of spectral engineering of biphotons generated by spontaneous parametric down-conversion and the technique of spectrally resolved Hong-Ou-Mandel interference. Our frequency-entangled qudits will enable quantum cryptographic experiments with enhanced performances. This distribution of distinct entangled frequency modes may also be useful for improved metrology, quantum remote synchronization, as well as for fundamental test of stronger violation of local realism.
High-dimensional (HD) quantum entanglement expands the Hilbert space, offering a robust framework for quantum information processing with enhanced capacity and error resilience. In this work, we present an HD frequency-domain entangled state, the hybrid frequency-entangled qudit (HFEQ), generated via Hong-Ou-Mandel (HOM) interference, exhibiting both discrete-variable (DV) and continuous-variable (CV) characteristics in the frequency domain. By tuning HOM interference, we generate and control HFEQs with dimensions D = 5 , 7 , 9 , and 11, confirming their DV nature. Franson interferometry verifies global frequency correlations with a visibility of 97.6 ± 0.6 % and CV entanglement within individual frequency modes with a visibility exceeding 95 % . Furthermore, based on the developed theoretical model, the generated HFEQs exhibit a Schmidt number that exceeds the upper bound D of conventional frequency-entangled qudits, certifying additional entanglement inherent to the hybrid structure. Our findings provide deeper insight into the physical nature of frequency-entangled qudits generated by quantum interference and introduce a resource for HD time-frequency quantum information processing.