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arXiv:2503.00362 · Physical Review Research

Harnessing hybrid frequency-entangled qudits through quantum interference

Sheng-Hung Wang, Po-Han Chen, Chengyu Yang, Yen-Hung Chen, Pin-Ju Tsai

Published Nov 12, 2025• 3 citations
arXivHTMLPDF

Abstract

High-dimensional (HD) quantum entanglement expands the Hilbert space, offering a robust framework for quantum information processing with enhanced capacity and error resilience. In this work, we present an HD frequency-domain entangled state, the hybrid frequency-entangled qudit (HFEQ), generated via Hong-Ou-Mandel (HOM) interference, exhibiting both discrete-variable (DV) and continuous-variable (CV) characteristics in the frequency domain. By tuning HOM interference, we generate and control HFEQs with dimensions D = 5 , 7 , 9 , and 11, confirming their DV nature. Franson interferometry verifies global frequency correlations with a visibility of 97.6 ± 0.6 % and CV entanglement within individual frequency modes with a visibility exceeding 95 % . Furthermore, based on the developed theoretical model, the generated HFEQs exhibit a Schmidt number that exceeds the upper bound D of conventional frequency-entangled qudits, certifying additional entanglement inherent to the hybrid structure. Our findings provide deeper insight into the physical nature of frequency-entangled qudits generated by quantum interference and introduce a resource for HD time-frequency quantum information processing.

DOI
10.1103/99qy-y833

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High-dimensional (HD) quantum entanglement expands the Hilbert space, offering a robust framework for quantum information processing with enhanced capacity and error resilience. In this work, we present an HD frequency-domain entangled state, the hybrid frequency-entangled qudit (HFEQ), generated via Hong-Ou-Mandel (HOM) interference, exhibiting both discrete-variable (DV) and continuous-variable (CV) characteristics in the frequency domain. By tuning HOM interference, we generate and control HFEQs with dimensions D = 5 , 7 , 9 , and 11, confirming their DV nature. Franson interferometry verifies global frequency correlations with a visibility of 97.6 ± 0.6 % and CV entanglement within individual frequency modes with a visibility exceeding 95 % . Furthermore, based on the developed theoretical model, the generated HFEQs exhibit a Schmidt number that exceeds the upper bound D of conventional frequency-entangled qudits, certifying additional entanglement inherent to the hybrid structure. Our findings provide deeper insight into the physical nature of frequency-entangled qudits generated by quantum interference and introduce a resource for HD time-frequency quantum information processing.
Abstract High-dimensional quantum entanglement is currently one of the most prolific fields in quantum information processing due to its high information capacity and error resilience. A versatile method for harnessing high-dimensional entanglement has long been hailed as an absolute necessity in the exploration of quantum science and technologies. Here we exploit Hong-Ou-Mandel interference to manipulate discrete frequency entanglement in arbitrary-dimensional Hilbert space. The generation and characterization of two-, four- and six-dimensional frequency entangled qudits are theoretically and experimentally investigated, allowing for the estimation of entanglement dimensionality in the whole state space. Additionally, our strategy can be generalized to engineer higher-dimensional entanglement in other photonic degrees of freedom. Our results may provide a more comprehensive understanding of frequency shaping and interference phenomena, and pave the way to more complex high-dimensional quantum information processing protocols.
Quantum entanglement is a fundamental resource for secure information processing and communications. The canonical optical quantum information processing encodes a single qubit per photon, with remarkable demonstrations of secure quantum communications, linear optical quantum computing amongst others. Often the polarization qubit, a discrete variable with entangled Bell states, is used. Continuous variables such as energy-time modes and spatial modes, however, present a dramatically larger Hilbert space for quantum information processing. The high-dimensional entanglement capture more qubits per photon, enabling dramatically higher secure key rates over longer distances and with better error resilience. Here I will describe our results on high-dimensional entanglement in quantum frequency combs for dense quantum communications. We first demonstrate revival of the Hong-Ou-Mandel interferences, long postulated by theorists more than a decade ago, up to 19-dimensions and with visibilities up to 96.5%. The mode-locked two-photon state in high-dimensions is further witnessed through a stabilized Franson interferometer, as a generalized Bell’s inequality test and hyperentangled through multiple degrees-of-freedom. Entanglement revivals of the non-local interference at discrete time-bins are uncovered, up to 97.8% visibility, as a fundamental resource for dense secure information processing.
Quantum entanglement is a vital resource in quantum information processing. High-dimensional quantum entanglement offers advantages that classical systems cannot surpass, particularly in enhancing channel capacity, improving system noise resilience, and increasing sensitivity to external environments. The construction of multimode entanglement in the spectral domain is well-suited for fiber-optic systems. Here, we present a straightforward scheme for generating multimode frequency-bin entanglement using a semiconductor chip through a simple mode conversion. A general model for Hong–Ou–Mandel (HOM) interference with a multimode frequency-bin entangled state is presented and applied to the experiments. The multimode entangled photons we produced exhibit HOM interference with a high-visibility beating pattern, demonstrating a strong relationship with the mode number, mode spacing, and the profile of the single mode. Building on the Fisher information analysis, we explore the relationship between the features in multimode entangled state interference traces and the precision of interferometric measurements even in the presence of experimental nonidealities. This work may deepen the understanding of multimode frequency-bin entanglement and advance the application of multimode HOM interference in quantum sensing.
Abstract Qudit entanglement is an indispensable resource for quantum information processing since increasing dimensionality provides a pathway to higher capacity and increased noise resilience in quantum communications, and cluster-state quantum computations. In continuous-variable time–frequency entanglement, encoding multiple qubits per photon is only limited by the frequency correlation bandwidth and detection timing jitter. Here, we focus on the discrete-variable time–frequency entanglement in a biphoton frequency comb (BFC), generating by filtering the signal and idler outputs with a fiber Fabry–Pérot cavity with 45.32 GHz free-spectral range (FSR) and 1.56 GHz full-width-at-half-maximum (FWHM) from a continuous-wave (cw)-pumped type-II spontaneous parametric downconverter (SPDC). We generate a BFC whose time-binned/frequency-binned Hilbert space dimensionality is at least 324, based on the assumption of a pure state. Such BFC’s dimensionality doubles up to 648, after combining with its post-selected polarization entanglement, indicating a potential 6.28 bits/photon classical-information capacity. The BFC exhibits recurring Hong–Ou–Mandel (HOM) dips over 61 time bins with a maximum visibility of 98.4% without correction for accidental coincidences. In a post-selected measurement, it violates the Clauser–Horne–Shimony–Holt (CHSH) inequality for polarization entanglement by up to 18.5 standard deviations with an S-parameter of up to 2.771. It has Franson interference recurrences in 16 time bins with a maximum visibility of 96.1% without correction for accidental coincidences. From the zeroth- to the third-order Franson interference, we infer an entanglement of formation (Eof) up to 1.89 ± 0.03 ebits—where 2 ebits is the maximal entanglement for a 4 × 4 dimensional biphoton—as a lower bound on the 61 time-bin BFC’s high-dimensional entanglement. To further characterize time-binned/frequency-binned BFCs we obtain Schmidt mode decompositions of BFCs generated using cavities with 45.32, 15.15, and 5.03 GHz FSRs. These decompositions confirm the time–frequency scaling from Fourier-transform duality. Moreover, we present the theory of conjugate Franson interferometry—because it is characterized by the state’s joint-temporal intensity (JTI)—which can further help to distinguish between pure-state BFC and mixed state entangled frequency pairs, although the experimental implementation is challenging and not yet available. In summary, our BFC serves as a platform for high-dimensional quantum information processing and high-dimensional quantum key distribution (QKD).
Frequency modes of light are one of the most promising platforms that provide access to high-dimensional quantum states amongst different photonic degrees of freedom capable of high-dimensionality, enabling robust, error-tolerant, and scalable quantum optical information systems. We demonstrate engineering of precisely controlled two-photon high-dimensional states entangled in frequency through time-domain Fourier optical synthesis. We generate and convert a continuous broadband frequency-entangled state into a large range of discrete frequency bins suitable for ITU standards, with spacings ranging from 12.5 GHz to 750 GHz, and observe spectral anticorrelations over 38 frequency bins, including intra-bin pure states at a 100 GHz bin spacing. We characterize the full quantum state dimensionality via Schmidt decomposition and observe lower bounds on the frequency-binned Hilbert-space dimensionalities of at least 289, formed by two entangled qudits with dimension 17. Furthermore, we demonstrate quantum nonlocality via frequency correlations in a transmission experiment over a campus-scale two-node fiber network. This work represents a crucial step towards building a versatile and relatively simple way of generating precisely controlled high-dimensional spectral qudits, with the potential of harnessing in wavelength-multiplexed quantum networks, high-dimensional information processing, and communication of quantum states specifically, and fiber-optic quantum remote sensing.
Abstract High‐dimensional frequency entanglement is an enabling resource in quantum technology due to its high information capacity and error resilience. A concise yet efficient method for precisely quantifying its dimensionality remains an open challenge, owing to the difficulties for performing required superposition measurements in energy‐time domains, and the complexity associated with full quantum state tomography that scales unfavorably with dimensions. With the assistance of Hong–Ou–Mandel experiment that performs a Fourier transform between the entangled photons in terms of joint spectral intensities and the quantum interference in terms of biphoton temporal coincidences, the concept of Shannon dimensionality as a fast quantifier of bipartite continuous frequency entanglement is unlocked. This quantitative technique reveals the complete distribution of frequency entanglement but without suffering from any limitation of modal capacity of the detection geometry. These results may significantly facilitate the use of quantum interference for characterizing the high‐dimensional entanglement nature by avoiding some stringent conditions.