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Journal of Modern Optics

Photon bunching from an equilateral triangle of atoms

Qurrat-ul-Ain Gulfam

Published Feb 23, 2023• 2 citations
Publisher

Abstract

Fluorescent photon emission probability from a system of three atoms has been studied as a function of detection angles. The system under investigation consists of identical bi-level atoms forming an equilateral triangle. Only a single atom in the triangle is resonantly excited by a weak laser. The interaction mechanism among the atoms is the vacuum-mediated dipole–dipole interaction and the collective decay process. The focus is to analyse the photon pairs simultaneously radiated by the system in the far-field domain. The analysis has been done for various interatomic separations. It is seen that the interference between the photon emitters can lead to strong emission in certain directions. An intuitive understanding of the interesting directions for strong photon bunching is given. It is found that a reduction in the intensity of radiation leads to superradiance along specific directions.

DOI
10.1080/09500340.2023.2220162

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Fluorescent photon emission probability from a system of three atoms has been studied as a function of detection angles. The system under investigation consists of identical bi-level atoms forming an equilateral triangle. Only a single atom in the triangle is resonantly excited by a weak laser. The interaction mechanism among the atoms is the vacuum-mediated dipole–dipole interaction and the collective decay process. The focus is to analyse the photon pairs simultaneously radiated by the system in the far-field domain. The analysis has been done for various interatomic separations. It is seen that the interference between the photon emitters can lead to strong emission in certain directions. An intuitive understanding of the interesting directions for strong photon bunching is given. It is found that a reduction in the intensity of radiation leads to superradiance along specific directions.
The probability of correlated emission of fluorescent photons as a function of detection directions has been investigated. The model system comprises identical two-level atoms arranged in the form of a line. A weak laser field resonantly excites only one of the atoms in the line. Two interaction mechanisms, namely, the vacuum-induced dipole–dipole interaction and the collective spontaneous emission couple the system of atoms. The aim is to observe the emission of a set of photon twins synchronized in time. It is seen that strongly directional emission of pairs of photons can take place due to the interference between the emitters. These highly correlated pairs of photons can be observed in very precise geometric directions. The observation is made based on two different detection procedures. It is found that the superradiant photons always tend to be bunched along the same direction.
We examine angular distribution of the probability of correlated fluorescence photon emission from a linear chain of identical equidistant two-level atoms. We selectively excite one of the atoms by a resonant laser field. The atoms are coupled to each other via the dipole-dipole interaction and collective spontaneous emission. Our attention is focused on the simultaneous observation of correlated pairs of photons. It is found that the interference between the emitting atoms can result in a highly directional emission of photon pairs. These pairs of photons exhibit strong correlations and their emission is highly concentrated into specific directions. We demonstrate the crucial role of the selective coherent excitation in such a geometrical configuration. Shifting the driving field from an atom located at one end of the chain to the other causes the radiation pattern to flip to the opposite half of the detection plane. Furthermore, we find that atomic systems in which only an atom situated at a particular position within the linear chain is driven by a laser field can radiate correlated twin photons in directions along which the radiation of single photons is significantly reduced. Alternatively, superbunching in the emitted photon statistics preferentially occurs in directions of negligible or vanishing single-photon emission. The effect of superbunching strengthens as more emitters are added to the chain. Depending on the number of atoms and the position of the driven atom within the chain, the strongly correlated pairs of photons can be emitted into few well-defined directions.
The steady-state quantum dynamics of three dipole-dipole coupled two-level emitters, fixed at the vertices of an equilateral triangle, and interacting via the environmental thermostat is investigated. We have analytically obtained the populations of the involved three-atom cooperative states as well as of the second- and third-order spatial photon correlation functions of the light scattered by the few-qubit sample. As a consequence, we have demonstrated that this incoherently excited system spontaneously generates streams of single photons possessing sub-Poissonian photon statistics. In analogy to the dipole-dipole blockade, one may expect that at smaller inter particle distances, compared to the photon emission wavelength, the reported phenomenon has the same origin. However, we have shown that the quantum photon features are due to the interaction's nature of the few symmetrically arranged two-level emitters with the surrounding thermal reservoir. Respectively, at larger atomic intervals the effect occurs because of high-order spatial interference phenomena. Sub-wavelength interference fringes can be observed too, via measurements of spatial higher-order photon correlation functions.
The ignition of two-quantum collective emission of inverted sub-ensemble of radiators due to mutual interaction of this sub-ensemble with other two dipole active atomic subsystems in process of two-photon exchanges between the atoms through the vacuum field is proposed. The three particle resonances between two-photon and single quantum transitions of inverted radiators from the ensemble are proposed for acceleration of collective decay rate of bi-photons, obtained relatively dipole-forbidden transitions of excited atomic sub-ensemble. This mutual interaction between three super-fluorescent processes in subatomic ensembles take place relatively dipole-forbidden transitions in one of radiator subsystem. The collective resonance emission and absorption of two-quanta have nontraditional behavior, accompanied with acceleration and inhibition of collective emission processes of photons.
The coherent photon scattering of atoms in an atomic array is studied. It is found that due to cooperative photon exchanges, the excitation probability of an atom in an array parallel to the direction of laser propagation ($\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\mathbit{k}}$) will either grow or decay along $\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\mathbit{k}}$, depending on the detuning of the laser. The symmetry of the system for atomic separations of $a=j\ensuremath{\lambda}/2$ causes the excitation distribution and scattered radiation to abruptly become symmetric about the center of the array, where jjj is an integer and $\ensuremath{\lambda}$ is the transition wavelength. For atomic separations of $a<\ensuremath{\lambda}/2$, a collection of nonradiating states ($\mathrm{\ensuremath{\Gamma}}\ensuremath{\sim}0$) disrupts the described trend. In order to interpret this surprising result, a band-structure calculation in the $N\ensuremath{\rightarrow}\ensuremath{\infty}$ limit is conducted, where the decay rates and the collective Lamb shifts of the eigenmodes versus quasimomentum are obtained. This calculation shows that the collective exchange of photons in an array strongly affects its scattered radiation, allowing one to easily manipulate the collective Lamb shift and directly excite either superradiant or subradiant eigenmodes by correctly choosing the angle of the driving laser.
Sub- and superradiant dynamics of spontaneously decaying atoms are manifestations of collective many-body systems. We study the internal dynamics and the radiation properties of two atoms in free space. Interesting results are obtained when the atoms are separated by less than half a wavelength of the atomic transition, where the dipole-dipole interaction gives rise to new coherent effects, such as (a) coherence between two intermediate collective states, (b) oscillations in the two-photon correlation G(2){G}^{(2)}G(2), (c) emission of two photons by one atom, and (d) the loss of directional correlation. We compare the population dynamics during the two-photon emission process with the dynamics of single-photon emission in the cases of a $\ensuremath{\Lambda}$ and a V scheme. We compute the temporal correlation and angular correlation of two successively emitted photons using the G(2){G}^{(2)}G(2) for different values of atomic separation. We find antibunching when the atomic separation is a quarter wavelength $\ensuremath{\lambda}∕4$. Oscillations in the temporal correlation provide a useful feature for measuring subwavelength atomic separation. Strong directional correlation between two emitted photons is found for atomic separation larger than a wavelength. We also compare the directionality of a photon spontaneously emitted by the two atoms prepared in phased-symmetric and phased-antisymmetric entangled states ${\ensuremath{\mid}\ifmmode\pm\else\textpm\fi{}⟩}_{{\mathbf{k}}_{0}}={e}^{i{\mathbf{k}}_{0}∙{\mathbf{r}}_{1}}\ensuremath{\mid}{a}_{1},{b}_{2}⟩\ifmmode\pm\else\textpm\fi{}{e}^{i{\mathbf{k}}_{0}∙{\mathbf{r}}_{2}}\ensuremath{\mid}{b}_{1},{a}_{2}⟩$ by a laser pulse with wave vector k0{\mathbf{k}}_{0}k0​. Photon emission is directionally suppressed along k0{\mathbf{k}}_{0}k0​ for the phased-antisymmetric state. The directionality ceases for interatomic distances less than $\ensuremath{\lambda}∕2$.