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arXiv:1605.00292 · Physical Review A

Collective dipole-dipole interactions in an atomic array

R. T. Sutherland, F. Robicheaux

Published Jul 27, 2016• 85 citations
arXivHTMLPDF

Abstract

The coherent photon scattering of atoms in an atomic array is studied. It is found that due to cooperative photon exchanges, the excitation probability of an atom in an array parallel to the direction of laser propagation ($\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\mathbit{k}}$) will either grow or decay along $\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\mathbit{k}}$, depending on the detuning of the laser. The symmetry of the system for atomic separations of $a=j\ensuremath{\lambda}/2$ causes the excitation distribution and scattered radiation to abruptly become symmetric about the center of the array, where $j$ is an integer and $\ensuremath{\lambda}$ is the transition wavelength. For atomic separations of $a<\ensuremath{\lambda}/2$, a collection of nonradiating states ($\mathrm{\ensuremath{\Gamma}}\ensuremath{\sim}0$) disrupts the described trend. In order to interpret this surprising result, a band-structure calculation in the $N\ensuremath{\rightarrow}\ensuremath{\infty}$ limit is conducted, where the decay rates and the collective Lamb shifts of the eigenmodes versus quasimomentum are obtained. This calculation shows that the collective exchange of photons in an array strongly affects its scattered radiation, allowing one to easily manipulate the collective Lamb shift and directly excite either superradiant or subradiant eigenmodes by correctly choosing the angle of the driving laser.

DOI
10.1103/physreva.94.013847

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The coherent photon scattering of atoms in an atomic array is studied. It is found that due to cooperative photon exchanges, the excitation probability of an atom in an array parallel to the direction of laser propagation (\mathbitk\ifmmode^\elseˆ\fi\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\mathbit{k}}\mathbitk\ifmmode^\elseˆ\fi​) will either grow or decay along \mathbitk\ifmmode^\elseˆ\fi\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\mathbit{k}}\mathbitk\ifmmode^\elseˆ\fi​, depending on the detuning of the laser. The symmetry of the system for atomic separations of a=j\ensuremathλ/2a=j\ensuremath{\lambda}/2a=j\ensuremathλ/2 causes the excitation distribution and scattered radiation to abruptly become symmetric about the center of the array, where jjj is an integer and \ensuremathλ\ensuremath{\lambda}\ensuremathλ is the transition wavelength. For atomic separations of a<\ensuremathλ/2a<\ensuremath{\lambda}/2a<\ensuremathλ/2, a collection of nonradiating states (\ensuremathΓ\ensuremath∼0\mathrm{\ensuremath{\Gamma}}\ensuremath{\sim}0\ensuremathΓ\ensuremath∼0) disrupts the described trend. In order to interpret this surprising result, a band-structure calculation in the N\ensuremath→\ensuremath∞N\ensuremath{\rightarrow}\ensuremath{\infty}N\ensuremath→\ensuremath∞ limit is conducted, where the decay rates and the collective Lamb shifts of the eigenmodes versus quasimomentum are obtained. This calculation shows that the collective exchange of photons in an array strongly affects its scattered radiation, allowing one to easily manipulate the collective Lamb shift and directly excite either superradiant or subradiant eigenmodes by correctly choosing the angle of the driving laser.
Collective coupling between dipoles can dramatically modify the optical response of a medium. Such effects depend strongly on the geometry of the medium and the polarization of the light. Using a classical coupled dipole model, here we investigate the simplest case of one-dimensional arrays of interacting atomic dipoles driven by a weak laser field. Changing the polarization and direction of the driving field allows us to separately address superradiant, subradiant, redshifted, and blueshifted eigenmodes, as well as observe strong Fano-like interferences between different modes. The cooperative eigenvectors can be characterized by the phase difference between nearest-neighbor dipoles, ranging from all oscillating in phase to all oscillating out of phase with their nearest neighbors. Investigating the eigenvalue behavior as a function of atom number and lattice spacing, we find that certain eigenmodes of an infinite atomic chain have the same decay rate as a single atom between two mirrors. The effects we observe provide a framework for collective control of the optical response of a medium, giving insight into the behavior of more complicated geometries, as well as providing further evidence for the dipolar analog of cavity QED.
The recoil of atoms in arrays due to the emission or absorption of photons is studied for subwavelength interatomic spacing. The atoms in the array interact with each other through collective dipole-dipole interactions and with the incident laser field in the low-intensity limit. Shining uniform light on the array gives rise to patterns of excitation and recoil in the array. They arise due to the interference of different eigenmodes of excitation. The relation between the recoil and the decay dynamics is studied when the array is in its excitation eigenstates. The recoil experienced by a subradiant collective decay is substantially larger than that from independent atom decay. A method to calculate the rate of recoil when steady state has been achieved with a constant influx of photons is also described.
Abstract We investigate the spectral shift known as the collective Lamb shift in forward scattering for a cold dense atomic cloud. The shift results from resonant dipole–dipole interaction mediated by real and virtual photon exchange, forming many-body states displaying various super- and subradiant behaviour. However, the scattering spectrum reflects the overall contributions from these states but also averages out the radiative details associated with the underlying spin orders, causing ambiguity in determination and raising controversy on the scaling property of this shift. We employ a Monte–Carlo simulation to study how the collective states contribute to emission. We thus distinguish two kinds of collective shift that follow different scaling laws. One results from dominant occupation of the near-resonant collective states. This shift is usually small and insensitive to the density or the number of participating atoms. The other comes from large spatial correlation of dipoles, associated with the states of higher degree of emission. This corresponds to larger collective shift that is approximately linearly dependent on the optical depth. We further demonstrate that the spatial spin order plays an essential role in superradiant emission. Our analysis provides a novel perspective for understanding collective scattering and cooperative effects.
The interaction of light with an atomic sample containing a large number of particles gives rise to many collective (or cooperative) effects, such as multiple scattering, superradiance, and subradiance, even if the atomic density is low and the incident optical intensity weak (linear optics regime). Tracing over the degrees of freedom of the light field, the system can be well described by an effective atomic Hamiltonian, which contains the light-mediated dipole-dipole interaction between atoms. This long-range interaction is at the origin of the various collective effects, or of collective excitation modes of the system. Even though an analysis of the eigenvalues and eigenfunctions of these collective modes does allow distinguishing superradiant modes, for instance, from other collective modes, this is not sufficient to understand the dynamics of a driven system, as not all collective modes are significantly populated. Here, we study how the excitation parameters, i.e., the driving field, determines the population of the collective modes. We investigate in particular the role of the laser detuning from the atomic transition, and demonstrate a simple relation between the detuning and the steady-state population of the modes. This relation allows understanding several properties of cooperative scattering, such as why superradiance and subradiance become independent of the detuning at large enough detuning without vanishing, and why superradiance, but not subradiance, is suppressed near resonance. We also show that the spatial properties of the collective modes allow distinguishing diffusive modes, responsible for radiation trapping, from subradiant modes.
The recoil momentum and energy of ultracold atoms is studied for situations where collective scattering or emission of photons is important. Effects due to the dipole-dipole interaction are emphasized. For two and many atoms confined in optical traps, calculations of the energy and momentum with respect to atomic separation are performed. When the atomic separation is comparable to or larger than the transition wavelength, the ultracold atoms' recoil energy depends mainly on collective spontaneous decay rather than forces from the cooperative frequency shift. Calculations for a laser pulse reflecting from an atomic array suggest that the recoil energy of atoms can be substantially larger than might be expected from an independent atom picture.
Superradiance is one of the many fascinating phenomena predicted by quantum electrodynamics that have first been experimentally demonstrated in atomic systems and more recently in condensed matter systems like quantum dots, superconducting q-bits, cyclotron transitions and plasma oscillations in quantum wells (QWs). It occurs when a dense collection of N identical two-level emitters are phased via the exchange of photons, giving rise to enhanced light-matter interaction, hence to a faster emission rate. Of great interest is the regime where the ensemble interacts with one photon only and therefore all of the atoms, but one, are in the ground state. In this case the quantum superposition of all possible configurations produces a symmetric state that decays radiatively with a rate N times larger than that of the individual oscillators. This phenomenon, called single photon superradiance, results from the exchange of real photons among the N emitters. Yet, to single photon superradiance is also associated another collective effect that renormalizes the emission frequency, known as cooperative Lamb shift. In this work, we show that single photon superradiance and cooperative Lamb shift can be engineered in a semiconductor device by coupling spatially separated plasma resonances arising from the collective motion of confined electrons in QWs. These resonances hold a giant dipole along the growth direction z and have no mutual Coulomb coupling. They thus behave as a collection of macro-atoms on different positions along the z axis. Our device is therefore a test bench to simulate the low excitation regime of quantum electrodynamics.