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arXiv:2602.18269

Higher-order spatial photon interference versus dipole blockade effect

Arthur Rotari, Mihai A. Macovei

quant-phcond-mat.stat-mechSubmitted Feb 20, 2026• Announced Feb 23, 2026• 0 citations
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Abstract

The steady-state quantum dynamics of three dipole-dipole coupled two-level emitters, fixed at the vertices of an equilateral triangle, and interacting via the environmental thermostat is investigated. We have analytically obtained the populations of the involved three-atom cooperative states as well as of the second- and third-order spatial photon correlation functions of the light scattered by the few-qubit sample. As a consequence, we have demonstrated that this incoherently excited system spontaneously generates streams of single photons possessing sub-Poissonian photon statistics. In analogy to the dipole-dipole blockade, one may expect that at smaller inter particle distances, compared to the photon emission wavelength, the reported phenomenon has the same origin. However, we have shown that the quantum photon features are due to the interaction's nature of the few symmetrically arranged two-level emitters with the surrounding thermal reservoir. Respectively, at larger atomic intervals the effect occurs because of high-order spatial interference phenomena. Sub-wavelength interference fringes can be observed too, via measurements of spatial higher-order photon correlation functions.

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10 pages, 3 figures

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The steady-state quantum dynamics of three dipole-dipole coupled two-level emitters, fixed at the vertices of an equilateral triangle, and interacting via the environmental thermostat is investigated. We have analytically obtained the populations of the involved three-atom cooperative states as well as of the second- and third-order spatial photon correlation functions of the light scattered by the few-qubit sample. As a consequence, we have demonstrated that this incoherently excited system spontaneously generates streams of single photons possessing sub-Poissonian photon statistics. In analogy to the dipole-dipole blockade, one may expect that at smaller inter particle distances, compared to the photon emission wavelength, the reported phenomenon has the same origin. However, we have shown that the quantum photon features are due to the interaction's nature of the few symmetrically arranged two-level emitters with the surrounding thermal reservoir. Respectively, at larger atomic intervals the effect occurs because of high-order spatial interference phenomena. Sub-wavelength interference fringes can be observed too, via measurements of spatial higher-order photon correlation functions.
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Second-order interference effects in the spontaneous emission by two identical two-level atoms, separated a distance apart and both initially excited, are considered. On the basis of the analysis in our previous paper published in 2004, within fourth-order perturbation, detailed analysis of the second-order quantum interference in the emitted field is made. The interference arises both from single-photon states and two-photon states owing to interferences between different decaying sequences. By detailed analysis we have found some cancellations between single-photon and two-photon interference terms, and an interpretation of this is given. The contributions from the single- and the two-photon states as well as the total interference are analysed numerically for various interatomic distances and times. The contribution from a two-photon state is mostly larger than that from a single-photon state except when the atomic electric dipole is large, in which case the two contributions can be comparable. It is shown that the emission patterns from the two interacting atoms provide more information on atom–atom correlations than the decay time evolution of the atomic states population does. The number of interference fringes and the distance between them depend on the interatomic distance in a similar fashion to Young's interference fringes.
We investigate the collective interaction of a multi-atom three-level ladder system with an environmental incoherent reservoir. The exact solution of the master equation that describes such a system of atoms emitting distinguishable or indistinguishable photons on interaction with an incoherent reservoir is obtained. The quantum decay interference effects have no influences over steady-state distribution of population among the energy levels. However, the photon statistics of the collectively emitted photons are different in this case. In particular, the normalized second-order photon correlation function shows a minimum in its value for the photons generated on lower atomic transition in a system with orthogonal dipoles. The minimum is due to the steady-state amplified spontaneous emission by the incoherent applied fields.
We investigate the collective interaction of a multi-atom three-level ladder system with an environmental incoherent reservoir. The exact solution of the master equation that describes such a system of atoms emitting distinguishable or indistinguishable photons on interaction with an incoherent reservoir is obtained. The quantum decay interference effects have no influences over steady-state distribution of population among the energy levels. However, the photon statistics of the collectively emitted photons are different in this case. In particular, the normalized second-order photon correlation function shows a minimum in its value for the photons generated on lower atomic transition in a system with orthogonal dipoles. The minimum is due to the steady-state amplified spontaneous emission by the incoherent applied fields.
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Sub- and superradiant dynamics of spontaneously decaying atoms are manifestations of collective many-body systems. We study the internal dynamics and the radiation properties of two atoms in free space. Interesting results are obtained when the atoms are separated by less than half a wavelength of the atomic transition, where the dipole-dipole interaction gives rise to new coherent effects, such as (a) coherence between two intermediate collective states, (b) oscillations in the two-photon correlation G(2){G}^{(2)}G(2), (c) emission of two photons by one atom, and (d) the loss of directional correlation. We compare the population dynamics during the two-photon emission process with the dynamics of single-photon emission in the cases of a $\ensuremath{\Lambda}$ and a V scheme. We compute the temporal correlation and angular correlation of two successively emitted photons using the G(2){G}^{(2)}G(2) for different values of atomic separation. We find antibunching when the atomic separation is a quarter wavelength $\ensuremath{\lambda}∕4$. Oscillations in the temporal correlation provide a useful feature for measuring subwavelength atomic separation. Strong directional correlation between two emitted photons is found for atomic separation larger than a wavelength. We also compare the directionality of a photon spontaneously emitted by the two atoms prepared in phased-symmetric and phased-antisymmetric entangled states ${\ensuremath{\mid}\ifmmode\pm\else\textpm\fi{}⟩}_{{\mathbf{k}}_{0}}={e}^{i{\mathbf{k}}_{0}∙{\mathbf{r}}_{1}}\ensuremath{\mid}{a}_{1},{b}_{2}⟩\ifmmode\pm\else\textpm\fi{}{e}^{i{\mathbf{k}}_{0}∙{\mathbf{r}}_{2}}\ensuremath{\mid}{b}_{1},{a}_{2}⟩$ by a laser pulse with wave vector k0{\mathbf{k}}_{0}k0​. Photon emission is directionally suppressed along k0{\mathbf{k}}_{0}k0​ for the phased-antisymmetric state. The directionality ceases for interatomic distances less than $\ensuremath{\lambda}∕2$.