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EPJ Quantum Technology

Polychromatic atom optics for atom interferometry

Samuel Lellouch, Oliver Ennis, Ramiz Haditalab, Mehdi Langlois, Michael Holynski

Published Mar 8, 2023• 4 citations
Publisher

Abstract

Abstract Coherent manipulation of atoms with atom-optic light pulses is central to atom interferometry. Achieving high pulse efficiency is essential for enhancing fringe contrast and sensitivity, in particular for large-momentum transfer interferometers which use an increased number of pulses. We perform an investigation of optimizing the frequency domain of pulses by using tailored polychromatic light fields, and demonstrate the possibility to deliver high-efficiency and resilient atom-optic pulses even in the situation of inhomogeneous atomic clouds and laser beams. We find that this approach is able to operate over long interrogation times despite spontaneous emission and to achieve experimentally relevant pulse efficiencies for clouds up to $100~\mu \text{K}$ 100 μ K . This overcomes some of the most stringent barriers for large-momentum transfer and has the potential to reduce the complexity of atom interferometers. We show that polychromatic light pulses could enhance single-photon-based large-momentum transfer atom interferometry—achieving $850\,\hbar k$ 850 ħ k of momentum splitting with experimentally accessible parameters, which represents a significant improvement over the state-of-the art. The benefits of the method extend beyond atom interferometry and could enable groundbreaking advances in quantum state manipulation.

DOI
10.1140/epjqt/s40507-023-00165-2

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Abstract Coherent manipulation of atoms with atom-optic light pulses is central to atom interferometry. Achieving high pulse efficiency is essential for enhancing fringe contrast and sensitivity, in particular for large-momentum transfer interferometers which use an increased number of pulses. We perform an investigation of optimizing the frequency domain of pulses by using tailored polychromatic light fields, and demonstrate the possibility to deliver high-efficiency and resilient atom-optic pulses even in the situation of inhomogeneous atomic clouds and laser beams. We find that this approach is able to operate over long interrogation times despite spontaneous emission and to achieve experimentally relevant pulse efficiencies for clouds up to 100 μK100~\mu \text{K}100 μK 100 μ K . This overcomes some of the most stringent barriers for large-momentum transfer and has the potential to reduce the complexity of atom interferometers. We show that polychromatic light pulses could enhance single-photon-based large-momentum transfer atom interferometry—achieving 850 ℏk850\,\hbar k850ℏk 850 ħ k of momentum splitting with experimentally accessible parameters, which represents a significant improvement over the state-of-the art. The benefits of the method extend beyond atom interferometry and could enable groundbreaking advances in quantum state manipulation.
Atom interferometric sensors can enable extremely precise measurements of inertial motion and external fields by manipulating and interfering atomic states using pulses of laser light. However, like many experiments that require the coherent control of a quantum system, the interaction fidelity is limited by inhomogeneities in the control fields. Variations in atomic velocity and laser intensity lead different atoms to experience different interactions under the same pulse, reducing the interference fringe contrast, introducing bias, and limiting the sensitivity. We present the theoretical design and experimental demonstration of pulses for atom interferometry which compensate inhomogeneities in atomic velocity and laser intensity. By varying the laser phase throughout a pulse and choosing an appropriate fidelity measure to be maximised, pulses are optimised by adapting optimal control techniques originally designed for nuclear magnetic resonance applications. We show using simulations that optimised pulses significantly improve the fidelity of interferometer operations and verify this experimentally using Raman transitions within a cold sample of 85Rb atoms. We demonstrate a robust state-transfer pulse that achieves a fidelity of 99.8(3)% in a ∼ 35 µK sample and obtain a threefold increase in the fringe contrast using a full sequence of optimised pulses. Many of the pulse shapes found by optimal control are simple and symmetrical, and we show that certain symmetries are integral to error compensation. By systematically exploring the dependence of these solutions on the model and optimisation parameters, we demonstrate a stability which underlines the general applicability of optimised pulses to a range of interferometer configurations. Finally, we introduce and computationally analyse a novel theoretical approach to improve the sensitivity of large-momentum-transfer (LMT) interferometers, whereby “biselective” pulses are optimised to track the changing resonance conditions encountered in extended pulse sequences that are designed to increase the measurement sensitivity. When conventional pulses of steady phase are used, the interference contrast decays rapidly as extra pulses are added because of the change in resonance. Using numerical simulations, we show that bi-selective pulses maintain interaction fidelity throughout extended pulse sequences, allowing significant increases in the sensitivity that may be obtained using LMT.
We present designs for the augmentation ``mirror'' pulses of large-momentum-transfer atom interferometers that maintain their fidelity as the wave-packet momentum difference is increased. These biselective pulses, tailored using optimal control methods to the evolving bimodal momentum distribution, should allow greater interferometer areas and hence increased inertial measurement sensitivity, without requiring elevated Rabi frequencies or extended frequency chirps. Using an experimentally validated model, we have simulated the application of our pulse designs to large-momentum-transfer atom interferometry using stimulated Raman transitions in a laser-cooled atomic sample of 85Rb^{85}\mathrm{Rb}85Rb at 1 $\ensuremath{\mu}\mathrm{K}$. After the wave packets have separated by 42 photon recoil momenta, our pulses maintain a fringe contrast of 90%, whereas, for adiabatic rapid passage and conventional $\ensuremath{\pi}$ pulses, the contrast is less than 10%. Furthermore, we show how these pulses may be adapted to be robust to laser intensity variations between pulses and to suppress the detrimental off-resonant excitation that limits other broadband pulse schemes.
Abstract Multi-photon Bragg diffraction is a powerful method for fast, coherent momentum transfer of atom waves. However, laser noise, Doppler detunings, and cloud expansion limit its efficiency in large momentum transfer (LMT) pulse sequences. We present simulation studies of robust Bragg pulses developed through numerical quantum optimal control. Optimized pulse performance under noise and cloud inhomogeneities is analyzed and compared to analogous Gaussian and adiabatic rapid passage pulses in simulated LMT Mach–Zehnder interferometry sequences. The optimized pulses maintain robust population transfer and phase response over a broader range of noise, resulting in superior contrast in LMT sequences with thermal atom clouds and intensity inhomogeneities. Large optimized LMT sequences use lower pulse area than Gaussian pulses, making them less susceptible to spontaneous emission loss. The optimized sequences maintain over five times better contrast with tens of ℏ k momentum separation and offer more improvement with greater LMT. Such pulses could allow operation of Bragg atom interferometers with unprecedented sensitivity, improved contrast, and hotter atom sources.
Atom interferometry is a highly versatile experimental technique for precision measurement, with applications in inertial sensing and tests of fundamental physics. Such interferometers rely on high fidelity transfer of atoms between internal states, which can be challenging when working with thermal atom clouds, where a range of resonance frequencies exists. Inhomogeneities in the spatial intensity distribution of the manipulation lasers can also give rise to a range of coupling strengths; both of these effects serve to reduce the fidelity of coherent manipulation operations. Composite pulses offer one route to high fidelity coherent manipulations. In this thesis we investigate the performance of composite pulses in a thermal cloud of Rubidium 85. We find remarkable agreement between theory and experimental investigation of composite inversion pulses, and build on this to model the performance of such pulses in atom interferometers. We also find excellent agreement between our model and the first experimental demonstration of an application of interferometry in the cooling of atoms; this is the first step towards implementing this cooling method in complex structures like molecules.
Abstract Large-scale atom interferometers promise unrivaled strain sensitivity to mid-band gravitational waves, and will probe a new parameter space in the search for ultra-light scalar dark matter. These proposals require gradiometry with kilometer-scale baselines, a momentum separation above 104ℏk between interferometer arms, and optical transitions to long-lived clock states to reach the target sensitivities. Prohibitively high optical power and wavefront flatness requirements have thus far limited the maximum achievable momentum splitting. Here we propose a scheme for optical cavity enhanced atom interferometry, using circulating, spatially resolved pulses, and intracavity frequency modulation to meet these requirements. We present parameters for the realization of 20 kW circulating pulses in a 1 km interferometer enabling 104ℏk splitting on the 698 nm clock transition in 87Sr. This scheme addresses the presently insurmountable laser power requirements and is feasible in the context of a kilometer-scale atom interferometer facility.
We report here on the realization of light-pulse atom interferometers with large-momentum-transfer atom optics based on a sequence of Bragg transitions. We demonstrate momentum splitting up to 200 photon recoils in an ultracold atom interferometer. We highlight a new mechanism of destructive interference of the losses leading to a sizable efficiency enhancement of the beam splitters. We perform a comprehensive study of parasitic interferometers due to the inherent multiport feature of the quasi-Bragg pulses. Finally, we experimentally verify the phase shift enhancement and characterize the interferometer visibility loss.