Abstract Multi-photon Bragg diffraction is a powerful method for fast, coherent momentum transfer of atom waves. However, laser noise, Doppler detunings, and cloud expansion limit its efficiency in large momentum transfer (LMT) pulse sequences. We present simulation studies of robust Bragg pulses developed through numerical quantum optimal control. Optimized pulse performance under noise and cloud inhomogeneities is analyzed and compared to analogous Gaussian and adiabatic rapid passage pulses in simulated LMT Mach–Zehnder interferometry sequences. The optimized pulses maintain robust population transfer and phase response over a broader range of noise, resulting in superior contrast in LMT sequences with thermal atom clouds and intensity inhomogeneities. Large optimized LMT sequences use lower pulse area than Gaussian pulses, making them less susceptible to spontaneous emission loss. The optimized sequences maintain over five times better contrast with tens of ℏ k momentum separation and offer more improvement with greater LMT. Such pulses could allow operation of Bragg atom interferometers with unprecedented sensitivity, improved contrast, and hotter atom sources.
Abstract Multi-photon Bragg diffraction is a powerful method for fast, coherent momentum transfer of atom waves. However, laser noise, Doppler detunings, and cloud expansion limit its efficiency in large momentum transfer (LMT) pulse sequences. We present simulation studies of robust Bragg pulses developed through numerical quantum optimal control. Optimized pulse performance under noise and cloud inhomogeneities is analyzed and compared to analogous Gaussian and adiabatic rapid passage pulses in simulated LMT Mach–Zehnder interferometry sequences. The optimized pulses maintain robust population transfer and phase response over a broader range of noise, resulting in superior contrast in LMT sequences with thermal atom clouds and intensity inhomogeneities. Large optimized LMT sequences use lower pulse area than Gaussian pulses, making them less susceptible to spontaneous emission loss. The optimized sequences maintain over five times better contrast with tens of ℏ k momentum separation and offer more improvement with greater LMT. Such pulses could allow operation of Bragg atom interferometers with unprecedented sensitivity, improved contrast, and hotter atom sources.
The combination of adiabatic rapid passage and multiphoton Bragg diffraction (ARPMB pulses) to efficiently transfer many photon recoils of momentum ($\ensuremath{\hbar}k$) to cold-atom clouds is theoretically and experimentally investigated. This method is insensitive to perturbations of the pulse intensity or detuning. In particular, the theoretically calculated velocity acceptance can be up to 80 of one recoil velocity vr, the theoretical maximum in Bragg diffraction. We experimentally demonstrate ARPMB pulses with transfer efficiency of 99.7 per $\ensuremath{\hbar}k$ using $10\ensuremath{\hbar}k$ pulses, limited by spontaneous emission losses, and Mach-Zehnder interferometers with 80 contrast.
This thesis contributes to the debate over the viability of using Bose-condensed sources to improve the sensitivity of atom interferometers. Specifically, we present theoretical investigations into (1) the effect of source momentum width on large momentum transfer (LMT) atom interferometry with Bragg pulses, and (2) the prospect of stabilising a high flux, narrow linewidth, continuously pumped atom laser via measurement-based feedback control of the BEC that forms the lasing mode of the atom laser. To begin, this thesis considers the effect of the atomic source's momentum width on the phase sensitivity of Bragg pulse atom interferometers in the Mach-Zehnder configuration. We show that an atomic cloud's momentum width places a fundamental upper bound on the maximum transfer efficiency of a Bragg mirror pulse, and furthermore limits the phase sensitivity of a Bragg pulse atom interferometer. We quantify these momentum width effects and precisely compute how mirror efficiencies and interferometer phase sensitivities vary as functions of Bragg order and source type. In particular, we show that narrow momentum width Bose-condensed sources give comparable sensitivities to broad momentum width thermal sources, even after incorporating the lower atom flux of Bose-condensed sources. Coupled with other favourable properties of Bose-condensed sources, such as their high tolerance to classical noise due to optical wavefront aberrations and the Coriolis effect, this suggests that LMT Bragg atom interferometry with Bose-condensed sources should yield improved sensitivities over current inertial sensors. Furthermore, our results and methodology allow for the efficient optimisation of Bragg pulses, which will help in the design of LMT Bragg mirrors and beamsplitters for atom-interferometer-based inertial sensors, irrespective of source type. In the second part of this thesis, we investigate the prospect of measurement-based feedback control of a BEC, with the aim of reducing density fluctuations by cooling the condensate to a stable spatial mode. Firstly, we consider the effects of experimental imperfections on the estimation-based feedback control of a weakly-interacting BEC undergoing continuous position measurement. These limitations violate the assumption that the estimator (i.e., filter) accurately models the underlying system, thus requiring a separate analysis of the system and filter dynamics. We show that the control scheme is robust to detector inefficiency, time delay, technical noise and miscalibrated parameters. These results imply that reasonable experimental imperfections do not limit the feasibility of cooling a BEC by continuous measurement and feedback. Secondly, we designed a feedback-control scheme for a trapped condensate, with interatomic interactions of any strength, based on a phase-contrast imaging setup. We derive the filtering equation for the system, and show that it gives a continuous measurement of the condensate's density. A semiclassical analysis of this control scheme shows that feedback-cooling of an interacting BEC is also possible, and that the interatomic interactions actually increase the effectiveness of the control. Therefore, measurement-based feedback control can stabilise the spatial mode of a BEC, which is a requirement for the high flux, narrow linewidth, continuously pumped atom laser sources that could potentially give inertial measurement sensitivities orders of magnitude beyond current state-of-the-art devices.
Bragg diffraction of matter waves is an established technique used in the most accurate quantum sensors. It is also the method of choice to operate large-momentum-transfer, high-sensitivity atom interferometers. It suffers, however, from an intrinsic multi-path character. Optimal control theory (OCT) has recently led to an improved robustness of atom interferometers to a range of challenging environmental effects such as vibrations or platform accelerations. In this theoretical work, we apply OCT protocols to control the Bragg diffraction phase shifts, thereby enhancing the metrological accuracy of the interferometer. We show a minimization of the diffraction phase for realistic conditions of finite temperature of the incoming wavepacket in a multi-path, high-order Bragg interferometer in a Mach–Zehnder configuration. We study input states with different momentum widths and find that our approach mitigates diffraction phases below the microradian level in the case of 1% of the photon recoil, thereby eliminating one of the leading systematic effects in atom interferometry.
Atom interferometric sensors can enable extremely precise measurements of inertial motion and external fields by manipulating and interfering atomic states using pulses of laser light. However, like many experiments that require the coherent control of a quantum system, the interaction fidelity is limited by inhomogeneities in the control fields. Variations in atomic velocity and laser intensity lead different atoms to experience different interactions under the same pulse, reducing the interference fringe contrast, introducing bias, and limiting the sensitivity. We present the theoretical design and experimental demonstration of pulses for atom interferometry which compensate inhomogeneities in atomic velocity and laser intensity. By varying the laser phase throughout a pulse and choosing an appropriate fidelity measure to be maximised, pulses are optimised by adapting optimal control techniques originally designed for nuclear magnetic resonance applications. We show using simulations that optimised pulses significantly improve the fidelity of interferometer operations and verify this experimentally using Raman transitions within a cold sample of 85Rb atoms. We demonstrate a robust state-transfer pulse that achieves a fidelity of 99.8(3)% in a ∼ 35 µK sample and obtain a threefold increase in the fringe contrast using a full sequence of optimised pulses. Many of the pulse shapes found by optimal control are simple and symmetrical, and we show that certain symmetries are integral to error compensation. By systematically exploring the dependence of these solutions on the model and optimisation parameters, we demonstrate a stability which underlines the general applicability of optimised pulses to a range of interferometer configurations. Finally, we introduce and computationally analyse a novel theoretical approach to improve the sensitivity of large-momentum-transfer (LMT) interferometers, whereby “biselective” pulses are optimised to track the changing resonance conditions encountered in extended pulse sequences that are designed to increase the measurement sensitivity. When conventional pulses of steady phase are used, the interference contrast decays rapidly as extra pulses are added because of the change in resonance. Using numerical simulations, we show that bi-selective pulses maintain interaction fidelity throughout extended pulse sequences, allowing significant increases in the sensitivity that may be obtained using LMT.
We formulate a robust optimal control algorithm to synthesize minimum energy pulses that can transfer a cold atom system into various momentum states. The algorithm uses adaptive linearization of the evolution operator and sequential quadratic programming to iterate the control towards a minimum energy pulse that achieves optimal target state fidelity. Robustness to parameter variation is achieved using Legendre polynomial approximation over the domain of variation. The method is applied to optimize the Bragg beamsplitting operation in ultra-cold atom interferometry. Even in the presence of 10-40% variability in the initial momentum dispersion of the atomic cloud and the intensity of the optical pulse, the algorithm reliably converges to a control protocol that robustly achieves unprecedented momentum levels with high fidelity for a single-frequency multi-photon Bragg diffraction scheme (e.g. ∣±40ℏk⟩). We show the advantages of our method by comparison to stochastic optimization using sampled parameter values, provide detailed sensitivity analyses, and performance of the designed pulses is verified in laboratory experiments.
Large-momentum-transfer (LMT) atom interferometers using elastic Bragg scattering on light waves are among the most precise quantum sensors to date. To advance their accuracy from the mrad to the μrad regime, it is necessary to understand the rich phenomenology of the Bragg interferometer, which differs significantly from that of a standard two-mode interferometer. We develop an analytic model for the interferometer signal and demonstrate its accuracy using comprehensive numerical simulations. Our analytic treatment allows the determination of the atomic projection noise limit of a LMT Bragg interferometer and provides the means to saturate this limit. It affords accurate knowledge of the systematic phase errors as well as their suppression by 2 orders of magnitude down to a few μrad using appropriate light-pulse parameters.