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Quantum Computing, Communication, and Simulation

High bandwidth, low-spurious, and stable laser source architecture for optical quantum emitters manipulation and control

Sacha Welinski, Perrine Berger, Eduardo Beattie, Lothaire Ulrich, Soeren Wengerowski, Hugues de Riedmatten, Loïc Morvan

Published Mar 8, 2023• 0 citations
Publisher

Abstract

Manipulation of optically addressable quantum emitters need stable laser sources able to perform complex and high bandwidth waveforms from visible range to infrared. Such waveforms can be generated using an acoustic-optical modulator; however with a limited bandwidth. Here we present a laser source able to deliver high-bandwidth and low noise optical signals at multiple frequencies over a span of a few GHz (scalable to 100 GHz), with a high extinction ratio with respect to all other spurious optical signals. The central wavelengths can be tuned to match the resonance of different optical quantum emitters in the visible or IR.

DOI
10.1117/12.2648759

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The exploitation of quantum mechanics has the potential to solve important challenges and \nintroduce novel technologies enabling, among others, powerful computation (which can solve \ncertain problems exponentially faster than classical computers), perfectly secure communications, \nas well as sensing and imaging with precision and resolutions not achievable by classical means. \nIn order to make use of the unique properties of quantum physics, experimental platforms \nthat provide access to, and allow the control of quantum states, need to be developed. In \nparticular, quantum systems composed of multiple parties are required, where each party is in a \ncoherent superposition of states, and where multiples of such parties are in a coherent \nsuperposition with each other (e.g. being entangled). Additionally, in order to make use of such \nentangled quantum systems, it is required that each individual party can be coherently controlled \nand measured. The usability and available quantum resources of the entangled system is related \nto its size, which is proportional to the number of entangled parties, as well as the dimensionality \nof the superposition each party is in. For this reason, there is a imminent demand to achieve, \ninvestigate, and improve the generation and control of large quantum systems, comprised of as \nmany entangled parties as possible, where each party is in an ideally high-dimensional \nsuperposition. \nMany quantum platforms are currently subject to extensive research, such as trapped ions, \nsuperconducting circuits, defect centers in solid-state crystals, mechanical oscillators, and optical \nquantum states (i.e. photons). While all platforms provide distinct advantages (as well as \nchallenges), optical photon states are of particular interest, because they can interact with other \nquantum systems, and can be transmitted over long distances while preserving their quantum \ncoherence without the need for extensive shielding. A large variety of sources for optical \nquantum states has been demonstrated, however most such implementations suffer from high \ncomplexity, ultimately limiting their scalability. Integrated photonics has recently become a \nleading platform for the compact, cost-efficient, and stable generation and processing of optical \nquantum states. However, to date, integrated quantum sources have only been able to generate \nphoton pairs, which operated on single channels, and single polarization modes. Furthermore, in \nthe few realizations of on-chip entanglement, they were limited to two entangled parties, where \neach party was in a two-dimensional superposition. These limitations of current integrated photon sources arise in large part from the concepts currently exploited to generate and control these \nstates. In particular, path-entangled sources are the most commonly used, but increasing the \nquantum state complexity requires a significant, and very challenging, increase in device \ncomplexity. There is therefore an urgent need to develop new concepts that can achieve the onchip \ngeneration of large and complex photon states without increasing source complexity, while \nstill enabling coherent quantum state control and detection. \nIn this work, we aim to address these limitations by making use of multiple frequency and \ntemporal modes within a single spatial waveguide mode (therefore readily compatible with \nstandard optical fibers) of an on-chip microring resonator. This approach is in contrast to more \ncommonly used techniques relying on path entanglement, which exploits multiple spatial modes \nand generates entanglement by means of complex waveguide structures. Working within a single \nspatial mode, we achieve the first demonstration of pure heralded single photons and entangled \nphoton pairs, which are emitted on multiple frequency modes from a single source. We then \ndemonstrate the first generation of multi-photon entangled quantum states on a photonic chip. \nFinally, by making use of the spectral multi-mode nature of optical frequency combs, we achieve \nthe generation of photon pairs in a coherent superposition of multiple frequency modes, \nrepresenting the first generation of high-dimensional entangled states on a photonic chip. \nOur work represents a significant step forward in the generation of complex quantum \nstates on a photonic chip and in a single spatial mode compatible with standard optical fibers. In \naddition, we demonstrated coherent quantum state control and manipulation for all generated \nstates by means of standard telecommunications components, which could in the future be also \nintegrated on single, monolithic chip. Our results indicate that the exploitation of integrated \noptical frequency comb sources for the generation of optical quantum states can provide a \nscalable and practical platform for quantum technologies.

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Manipulation of optically addressable quantum emitters need stable laser sources able to perform complex and high bandwidth waveforms from visible range to infrared. Such waveforms can be generated using an acoustic-optical modulator; however with a limited bandwidth. Here we present a laser source able to deliver high-bandwidth and low noise optical signals at multiple frequencies over a span of a few GHz (scalable to 100 GHz), with a high extinction ratio with respect to all other spurious optical signals. The central wavelengths can be tuned to match the resonance of different optical quantum emitters in the visible or IR.
Optical manipulation of quantum systems requires stable laser sources able to produce complex waveforms over a large frequency range. In the visible region, such waveforms can be generated using an acousto-optic modulator driven by an arbitrary waveform generator, but these suffer from a limited tuning range typically of a few tens of MHz. Visible-range electro-optic modulators are an alternative option offering a larger modulation bandwidth, however they have limited output power which drastically restricts the scalability of quantum applications. There is currently no architecture able to perform phase-stabilized waveforms over several GHz in the visible or near infrared region while providing sufficient optical power for quantum applications. Here we propose and develop a modulation and frequency conversion set-up able to deliver optical waveforms over a large frequency range, with a high spurious extinction ratio, scalable to the entire visible/near infrared region with high optical power. The optical waveforms are first generated at telecom wavelength and then converted to the emitter wavelength through a sum frequency generation process. By adapting the pump laser frequency, the optical waveforms can be tuned to interact with a broad range of optical quantum emitters or qubits such as alkali atoms, trapped ions, rare earth ions, or fluorescent defects in solid-state matrices. Using this architecture, we were able to detect and study a single erbium ion in a nanoparticle. We also generated high bandwidth signals at 606 nm, which would enable frequency multiplexing of on-demand read-out Pr3+:Y2SiO5 quantum memories.
The method of quantum communication using sideband-modulated emission allows for efficient integration of devices constructed on this principle into optical fiber communication lines due to a number of advantages, including the absence of complex distributed interference schemes, simplification of the phase alignment task of the transmitter and receiver modules, and a significant increase in spectral efficiency of the use of the optical fiber communication line [1, 2]. The development of low-loss quantum communication methods using sideband frequencies, the efficiency of which does not depend on uncontrolled polarization change in the communication channel, and the development of methods for high-speed generation of quantum states are important theoretical and practical tasks. A semiconductor frequency-tunable laser with a central wavelength of 1550 nm, a bandwidth of 1.5 MHz, and a tuning step of 0.005 nm was used as the radiation source. The signal attenuation in the filter band is 43 dB, which allows to apply a modulation index of 0.05 with a contribution of the central wavelength to the quantum bit error rate of not more than 0.1%. The error rate when using the compensation scheme does not exceed 0.5%. The losses in the receiving module are 6.4 dB, which consist of losses of each modulator, on the polarization beam splitter, mixer, filter, and optical connectors.
Quantum repeaters—fundamental building blocks for long-distance quantum communication—are based on the interaction between photons and quantum memories. The photons must fulfil stringent requirements on central frequency, spectral bandwidth and purity in order for this interaction to be efficient. We present a design scheme for monolithically integrated resonant photon-pair sources based on parametric down-conversion in nonlinear waveguides, which facilitate the generation of such photons. We investigate the impact of different design parameters on the performance of our source. The generated photon spectral bandwidths can be varied between several tens of MHz up to around 1 GHz, facilitating an efficient coupling to different memories. The central frequency of the generated photons can be coarsely tuned by adjusting the pump frequency, poling period and sample temperature, and we identify stability requirements on the pump laser and sample temperature that can be readily fulfilled with off-the-shelf components. We find that our source is capable of generating high-purity photons over a wide range of photon bandwidths. Finally, the PDC emission can be frequency fine-tuned over several GHz by simultaneously adjusting the sample temperature and pump frequency. We conclude our study with demonstrating the adaptability of our source to different quantum memories.
The generation and application of squeezed light have long been central goals of quantum optics, enabling sensing below the standard quantum limit, optical quantum computing platforms, and more. Intensity noise squeezing of bright (coherent) states, in contrast to squeezed vacuum, is relatively underdeveloped. Bright squeezing has been generated directly through nonlinear optical processes or ``quietly pumped'' semiconductor lasers. However, these methods suffer from weak squeezing limits, narrow operating wavelength ranges, and have not been explored at large bandwidths. Here, we show how semiconductor lasers with sharp intensity-dependent dissipation can support highly broadband intensity noise squeezing from infrared (IR) to terahertz (THz) wavelengths, the latter of which has remained unexplored in quantum noise studies. Our protocol realizes strongly (>10>10>10 dB) intensity noise-squeezed intracavity quantum states, which could create a new regime for cavity quantum electrodynamics experiments, as well as strong output squeezing surpassing gigahertz bandwidths. Furthermore, we show how the same systems also create self-pulsing and bistable mean field behavior, enabling control of light in both the temporal and noise domains. The existence of these multiple functionalities in both the classical and quantum mechanical domains in a single semiconductor laser platform, from IR to THz wavelengths, could enable advances in on-chip quantum optical communication, computing, and sensing across the electromagnetic spectrum.
The exploitation of quantum mechanics has the potential to solve important challenges and \nintroduce novel technologies enabling, among others, powerful computation (which can solve \ncertain problems exponentially faster than classical computers), perfectly secure communications, \nas well as sensing and imaging with precision and resolutions not achievable by classical means. \nIn order to make use of the unique properties of quantum physics, experimental platforms \nthat provide access to, and allow the control of quantum states, need to be developed. In \nparticular, quantum systems composed of multiple parties are required, where each party is in a \ncoherent superposition of states, and where multiples of such parties are in a coherent \nsuperposition with each other (e.g. being entangled). Additionally, in order to make use of such \nentangled quantum systems, it is required that each individual party can be coherently controlled \nand measured. The usability and available quantum resources of the entangled system is related \nto its size, which is proportional to the number of entangled parties, as well as the dimensionality \nof the superposition each party is in. For this reason, there is a imminent demand to achieve, \ninvestigate, and improve the generation and control of large quantum systems, comprised of as \nmany entangled parties as possible, where each party is in an ideally high-dimensional \nsuperposition. \nMany quantum platforms are currently subject to extensive research, such as trapped ions, \nsuperconducting circuits, defect centers in solid-state crystals, mechanical oscillators, and optical \nquantum states (i.e. photons). While all platforms provide distinct advantages (as well as \nchallenges), optical photon states are of particular interest, because they can interact with other \nquantum systems, and can be transmitted over long distances while preserving their quantum \ncoherence without the need for extensive shielding. A large variety of sources for optical \nquantum states has been demonstrated, however most such implementations suffer from high \ncomplexity, ultimately limiting their scalability. Integrated photonics has recently become a \nleading platform for the compact, cost-efficient, and stable generation and processing of optical \nquantum states. However, to date, integrated quantum sources have only been able to generate \nphoton pairs, which operated on single channels, and single polarization modes. Furthermore, in \nthe few realizations of on-chip entanglement, they were limited to two entangled parties, where \neach party was in a two-dimensional superposition. These limitations of current integrated photon sources arise in large part from the concepts currently exploited to generate and control these \nstates. In particular, path-entangled sources are the most commonly used, but increasing the \nquantum state complexity requires a significant, and very challenging, increase in device \ncomplexity. There is therefore an urgent need to develop new concepts that can achieve the onchip \ngeneration of large and complex photon states without increasing source complexity, while \nstill enabling coherent quantum state control and detection. \nIn this work, we aim to address these limitations by making use of multiple frequency and \ntemporal modes within a single spatial waveguide mode (therefore readily compatible with \nstandard optical fibers) of an on-chip microring resonator. This approach is in contrast to more \ncommonly used techniques relying on path entanglement, which exploits multiple spatial modes \nand generates entanglement by means of complex waveguide structures. Working within a single \nspatial mode, we achieve the first demonstration of pure heralded single photons and entangled \nphoton pairs, which are emitted on multiple frequency modes from a single source. We then \ndemonstrate the first generation of multi-photon entangled quantum states on a photonic chip. \nFinally, by making use of the spectral multi-mode nature of optical frequency combs, we achieve \nthe generation of photon pairs in a coherent superposition of multiple frequency modes, \nrepresenting the first generation of high-dimensional entangled states on a photonic chip. \nOur work represents a significant step forward in the generation of complex quantum \nstates on a photonic chip and in a single spatial mode compatible with standard optical fibers. In \naddition, we demonstrated coherent quantum state control and manipulation for all generated \nstates by means of standard telecommunications components, which could in the future be also \nintegrated on single, monolithic chip. Our results indicate that the exploitation of integrated \noptical frequency comb sources for the generation of optical quantum states can provide a \nscalable and practical platform for quantum technologies.
Practical quantum networks will require multi-qubit quantum nodes. This in turn will increase the complexity of the photonic circuits needed to control each qubit and require strategies to multiplex memories. Integrated photonics operating at visible to near-infrared (VNIR) wavelength range can provide solutions to these needs. In this work, we realize a VNIR thin-film lithium niobate (TFLN) integrated photonics platform with the key components to meet these requirements, including low-loss couplers (<1 dB/facet), switches (>20 dB extinction), and high-bandwidth electro-optic modulators (>50 GHz). With these devices, we demonstrate high-efficiency and CW-compatible frequency shifting (>50% efficiency at 15 GHz), as well as simultaneous laser amplitude and frequency control. Finally, we highlight an architecture for multiplexing quantum memories and outline how this platform can enable a 2-order of magnitude improvement in entanglement rates over single memory nodes. Our results demonstrate that TFLN can meet the necessary performance and scalability benchmarks to enable large-scale quantum nodes.