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Optica Quantum

Low-noise short-wavelength pumped frequency downconversion for quantum frequency converters

Jan Fabian Geus, Florian Elsen, Sebastian Nyga, Arian Stolk, Kian L. van der Enden, E.J. van Zwet, C. Haefner, Ronald Hanson, Bernd Jungbluth

Published May 13, 2024• 16 citations
Publisher

Abstract

In this paper, we present a novel single stage quantum frequency conversion (QFC) scheme based on an enhancement cavity, which allows for high conversion efficiencies with record low noise levels, 100 times smaller than in previous systems and close to the thermal background. Our approach represents a significant improvement over traditional QFC methods that rely on periodically poled waveguide crystals, which typically produce high levels of noise with input wavelengths in the visible spectrum. One of the key challenges in QFC is the generation of noise photons - photons that are not part of the desired output state. Those noise photons are one of the major limitations of today’s quantum network experiments. It has been widely believed that single stage QFC of qubit photons in the visible range would result in too many noise photons in the telecom band, because of SPDC induced by the short wavelength driver laser. However, using the enhancement cavity design, we are able to overcome this challenge and demonstrate high-fidelity QFC from the visible to telecom band. Our results have important implications for the development of practical QFC devices for a range of applications, including quantum communication and quantum networks, where low noise levels are critical.

DOI
10.1364/opticaq.515769

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In this paper, we present a novel single stage quantum frequency conversion (QFC) scheme based on an enhancement cavity, which allows for high conversion efficiencies with record low noise levels, 100 times smaller than in previous systems and close to the thermal background. Our approach represents a significant improvement over traditional QFC methods that rely on periodically poled waveguide crystals, which typically produce high levels of noise with input wavelengths in the visible spectrum. One of the key challenges in QFC is the generation of noise photons - photons that are not part of the desired output state. Those noise photons are one of the major limitations of today’s quantum network experiments. It has been widely believed that single stage QFC of qubit photons in the visible range would result in too many noise photons in the telecom band, because of SPDC induced by the short wavelength driver laser. However, using the enhancement cavity design, we are able to overcome this challenge and demonstrate high-fidelity QFC from the visible to telecom band. Our results have important implications for the development of practical QFC devices for a range of applications, including quantum communication and quantum networks, where low noise levels are critical.
Quantum frequency conversion (QFC) is essential for bridging the spectral gap between stationary qubits and low-loss optical communication channels. Practicable QFC interfaces connecting ultraviolet and telecommunication bands are of great significance but have remained elusive, constrained by the dual challenges of a high-performance frequency converter and effective noise suppression in short-wavelength pumping configurations. We address this by demonstrating the phase-matching mechanism with domain defects and differential-tuning behavior of the spontaneous parametric down-conversion noises. Based on a quantitative analysis of performance degradation induced by domain defects, we propose specific fabrication guidelines and experimentally achieve an ultrahigh normalized conversion efficiency of 839%/(W cm^{2}) for the fundamental guided mode in thin-film lithium niobate waveguides. Meanwhile, we reveal a new noise control mechanism for short-wavelength pumping by utilizing the differential-tuning behaviors of difference-frequency generation and spontaneous parametric down-conversion processes. Then a single-stage QFC from 393 nm to the telecom C band with a record-high external efficiency of 28.8% and an ultralow noise level of 35 counts per second is achieved experimentally. The proposed mechanisms would enable other QFCs with higher efficiency and lower noise, advancing the development of scalable quantum networks. Furthermore, it holds significant potential for driving progress in both classical and integrated nonlinear photonics.
Quantum frequency conversion (QFC) which converts the frequencies of photons while preserving the quantum state is an essential technology for realizing the quantum internet and quantum interconnect. For the QFC based on the frequency downconversion from visible to the telecom wavelengths around 1500 nm, it is widely known that noise photons produced by the strong pump light used for QFC contaminate the frequency-converted photon, which degrades the quality of the quantum property of the photon after QFC. In conventional QFC experiments, noise photons are removed using external narrowband frequency filter systems. In contrast, in this study, we implement a compact QFC device integrating the cavity structure only for the converted mode. While the cavity structure can enhance not only the desired QFC efficiency but also the noise photon generation rate, we show that the cavity-enhanced QFC followed by a relatively wide bandpass filter achieves the signal-to-noise ratio comparable to the QFCs with external narrowband filters. We experimentally demonstrate the cavity-enhanced QFC using a single photon at 780 nm to 1540 nm, in which the non-classical photon statistics is clearly observed after QFC.
In this work we experimentally and theoretically characterize the converted signal and the noise level of a quantum frequency conversion (QFC) device implemented for frequency down conversion from the visible to telecommunication wavelengths. This frequency converter is a useful device able to interface quantum memories operating at different wavelengths. We observe that the main noise source is directly induced by the pump via spontaneous parametric down-conversion (SPDC), enhanced by imperfections in the periodic poling structure of the waveguide. We also measure conversion with high signal to noise ratio for microsecond long weak coherent states at the single photon level. Finally, we show theoretically that the converted Stokes/Anti-Stokes non-classical correlations of photon pairs emitted by quantum memories could be largely preserved for pulse durations lower than 4µs.
Quantum frequency conversion (QFC) is essential for bridging the spectral gap between stationary qubits and low-loss optical communication channels. In this work, we demonstrate a short-wavelength-pumping QFC with the first-order quasi-phase matching period of 3.07 um on thin-film lithium niobate, converting ultraviolet photons to the telecom C-band. By constructing a theoretical model that correlates the normalized conversion efficiency with domain defects in the short-period phase-matched waveguide, we found the critical tolerance of domain defects along the waveguide should be ≤2\le 2≤2 (excluding the ends). Based on this, we achieved a theoretical limit normalized conversion efficiency of 839%/(W*cm^2) for the fundamental guided mode through fabrication optimization. Furthermore, we propose a robust noise suppression strategy for short-wavelength pumping by utilizing the counter-tuning behaviors of difference-frequency generation and spontaneous parametric down-conversion. By combining these advances with ultra-narrowband filtering, we achieve a record-high external efficiency of 28.8% and an ultra-low noise of 35 counts per second. This high-performance QFC connecting ultraviolet and telecom bands satisfies the stringent requirements for long-lived remote ion-ion entanglement in scalable quantum networks [W.-Z. Liu et al., Nature (2026)].
The silicon-vacancy center in diamond holds great promise as a qubit for quantum communication networks. However, since the optical transitions are located within the visible red spectral region, quantum frequency conversion to low-loss telecommunication wavelengths becomes a necessity for its use in long-range, fiber-linked networks. This work presents a highly efficient, low-noise quantum frequency conversion device for photons emitted by a silicon-vacancy (SiV) center in diamond to the telecom C-band. By using a two-stage difference-frequency mixing scheme SPDC noise is circumvented and Raman noise is minimized, resulting in a very low noise rate of 10.4±0.710.4 \pm 0.710.4±0.7 photons per second as well as an overall device efficiency of 35.6 %35.6\, \%35.6%. By converting single photons from SiV centers we demonstrate the preservation of photon statistics upon conversion.
Trapped ions are one of the leading candidates for scalable and long-distance quantum networks because of their long qubit coherence time, high-fidelity single- and two-qubit gates, and their ability to generate photons entangled with the qubit state of the ion. One method for creating ion-photon entanglement is to exploit optical transitions from the 6 P 1/2 to 6 S 1/2 levels, which naturally emit spin-photon entangled states. But these optical transitions typically lie in the ultraviolet and visible wavelength regions of the spectrum. These wavelengths exhibit significant fiber-optic propagation loss, thereby limiting the transfer of quantum information to tens of meters. Quantum frequency conversion is essential to convert these photons to telecom wavelengths so that they can propagate over long distances in fiber-based networks, as well as for compatibility with the vast number of telecom-based optoelectronic components. Here, we generate O-band telecom photons via a low-noise quantum frequency conversion scheme from photons emitted from the 6 P 1/2 to 6 S 1/2 dipole transition of a trapped barium ion. We use a two-stage quantum frequency conversion scheme to achieve a frequency shift of 375.4 THz between the input visible photon and the output telecom photon, achieving a conversion efficiency of 11%. We attain a signal-to-background ratio of over 100 for the converted O-band telecom photon with background noise of less than 15 counts/s. These results are an important step toward achieving trapped ion quantum networks over long distances for distributed quantum computing and quantum communication.