Quantum Frequency Conversion of Single Photons from a Tin-Vacancy Center in Diamond
Julia M. Brevoord, Jan Fabian Geus, Tim Turan, Romero, Miguel Guerrero, Rodríguez, Daniel Bedialauneta, Nina Codreanu, Alexander M. Stramma, Ronald Hanson, Florian Elsen, Bernd Jungbluth
Diamond tin-vacancy (SnV) centers are promising candidates for building quantum network nodes. However, their native photon emission at 619 nm is incompatible with metropolitan-scale networks operating at low-loss telecom wavelengths. To address this, we demonstrate highly efficient, low-noise quantum frequency conversion (QFC) of 619 nm photons to the telecom S-band at 1480 nm. The conversion process combines 619 nm photons with 1064 nm pump light in an actively stabilized cavity containing a bulk monocrystalline potassium titanyl arsenate (KTA) crystal. We achieve an internal (external) conversion efficiency of (48 +/- 3)% ((28 +/- 2)%) and a noise photon rate per wavelength of 2.2 +/- 0.9 cts/s/pm, which is spectrally flat in the investigated frequency range of 40 GHz. Furthermore, we demonstrate that the efficiency remains above 80% of its maximum over a frequency range of 70 GHz. Finally, we generate a string of photons from a single waveguide-embedded SnV center using a train of excitation pulses and send these through the QFC. After the QFC, we observe a string of telecom photons displaying the SnV lifetime, confirming successful conversion. These results represent a critical step towards metropolitan-scale fiber-based quantum networks using SnV centers.
Diamond tin-vacancy (SnV) centers are promising candidates for building quantum network nodes. However, their native photon emission at 619 nm is incompatible with metropolitan-scale networks operating at low-loss telecom wavelengths. To address this, we demonstrate highly efficient, low-noise quantum frequency conversion (QFC) of 619 nm photons to the telecom S-band at 1480 nm. The conversion process combines 619 nm photons with 1064 nm pump light in an actively stabilized cavity containing a bulk monocrystalline potassium titanyl arsenate (KTA) crystal. We achieve an internal (external) conversion efficiency of (48 +/- 3)% ((28 +/- 2)%) and a noise photon rate per wavelength of 2.2 +/- 0.9 cts/s/pm, which is spectrally flat in the investigated frequency range of 40 GHz. Furthermore, we demonstrate that the efficiency remains above 80% of its maximum over a frequency range of 70 GHz. Finally, we generate a string of photons from a single waveguide-embedded SnV center using a train of excitation pulses and send these through the QFC. After the QFC, we observe a string of telecom photons displaying the SnV lifetime, confirming successful conversion. These results represent a critical step towards metropolitan-scale fiber-based quantum networks using SnV centers.
Diamond tin-vacancy (SnV) centers are promising candidates for building quantum network nodes. However, their native photon emission at 619 nm is incompatible with metropolitan-scale networks operating at low-loss telecom wavelengths. To address this, we demonstrate highly efficient, low-noise quantum frequency conversion (QFC) of 619 nm photons to the telecom S-band at 1480 nm. The conversion process combines 619 nm photons with 1064 nm pump light in an actively stabilized cavity containing a bulk monocrystalline potassium titanyl arsenate (KTA) crystal. We achieve an internal (external) conversion efficiency of (48 ± 3) % ((28 ± 2) %) and a noise photon rate per wavelength of (2.2 ± 0.9) cts/s/pm, which is spectrally flat in the investigated frequency range of 40 GHz. Furthermore, we demonstrate that the efficiency remains above 80% of its maximum over a frequency range of 70 GHz. Finally, we generate a string of photons from a single waveguide-embedded SnV − center using a train of excitation pulses and send these through the QFC. After the QFC, we observe telecom light displaying the SnV lifetime, confirming successful conversion. These results represent a critical step towards metropolitan-scale fiber-based quantum networks using SnV − centers.
Interfacing the different building blocks of a future large-scale quantum network will require efficient and noiseless frequency conversion of quantum light. Nitrogen-vacancy centers in diamond are a leading candidate to form the nodes of such a network. However, the performance of a suitable converter remains a bottleneck, with existing demonstrations severely limited by parasitic noise arising at the target telecommunication wavelength. Here we demonstrate a platform for efficient low-noise quantum frequency conversion based on a monolithic bulk periodically poled potassium titanyl phosphate cavity and show its suitability for the conversion of 637-nm single photons from nitrogen-vacancy centers in diamond to telecommunication wavelengths. By resonantly enhancing the power of an off-the-shelf pump laser, we achieve an internal conversion efficiency of $(72.3\ifmmode\pm\else\textpm\fi{}0.4)\mathrm{%}$ while generating noise of only $(110\ifmmode\pm\else\textpm\fi{}4)\phantom{\rule{0.2em}{0ex}}\mathrm{kHz}/\mathrm{nm}$ at the target wavelength without the need for any active stabilization. This constitutes a fivefold reduction in noise over existing state-of-the-art single-step converters at these wavelengths. We verify the almost-ideal preservation of nonclassical correlations by converting photons from a spontaneous-parametric-down-conversion source and moreover show the preservation of time-energy entanglement via Franson interferometry.
The silicon-vacancy center in diamond holds great promise as a qubit for quantum communication networks. However, since the optical transitions are located within the visible red spectral region, quantum frequency conversion to low-loss telecommunication wavelengths becomes a necessity for its use in long-range, fiber-linked networks. This work presents a highly efficient, low-noise quantum frequency conversion device for photons emitted by a silicon-vacancy (SiV) center in diamond to the telecom C-band. By using a two-stage difference-frequency mixing scheme SPDC noise is circumvented and Raman noise is minimized, resulting in a very low noise rate of 10.4±0.7 photons per second as well as an overall device efficiency of 35.6%. By converting single photons from SiV centers we demonstrate the preservation of photon statistics upon conversion.
Quantum networks promise secure communication, distributed sensing and modular quantum computing by interconnecting distant quantum nodes through photonic links. Extending such networks beyond metropolitan distances requires quantum repeaters to overcome the exponential attenuation of photons in optical fiber. Across all architectures, a key requirement is the indistinguishability of single photons, which directly impacts the fidelity of photonic operations based on two-photon interference, such as Bell-state measurements and fusion gates. Here, we demonstrate generation of highly indistinguishable single photons from a coherently excited tin-vacancy center in diamond, achieving raw Hong-Ou-Mandel interference visibilities exceeding 0.95. By separating intrinsic emitter properties from technical imperfections, we show that decoherence plays a negligible role and that the remaining limitations are predominantly technical in nature, arriving at an intrinsic indistinguishability of up to 0.999. We further show that quantum frequency conversion to the telecom C-band preserves the photon indistinguishability. In combination with the long-lived electron and nuclear spin coherence times, these results establish tin-vacancy centers in diamond as a competitive platform for long-distance quantum networks and photonic quantum information processing. We further substantiate this potential through Monte Carlo simulations of a quantum-repeater link, demonstrating that the SnV-center platform surpasses the bound set by direct transmission.
High-efficiency quantum frequency conversion (QFC) for group-IV color centers, such as silicon vacancies (SiV), is required for long-distance quantum networking protocols. Performance of QFC depends on the choices of network and pump wavelengths and the choice between bulk crystal and waveguide, since these directly determine the dominant noise processes. These furthermore lead to fiber-based or free-space, single- or multi-pass setups with different complexities, power requirements, losses, and hence, external efficiencies. Here, we present a QFC device design for SiV QFC with simultaneous state-of-the-art performance and simple setup. Namely, by choosing the C-band pump wavelength of λ p = 1561 nm, which leads to an E-band network wavelength of λ n = 1398 nm, we remain in the anti-Stokes noise regime in a one-stage, single-pass conversion scheme. The high-quality erbium-doped fiber amplifiers in this band aid in maximizing the internal nonlinear process. We measure an external (internal) photon conversion efficiency of 44.5 ± 1.8 % (8.5 ± 1.8 %) at an external (internal) pump power of 1.51 W (0.97 W), limited by fiber coupling efficiencies. This is an increase in efficiency by 9 % (25 %) compared to prior demonstrations for SiV QFC, which were limited by factors such as internal device efficiencies, limited available pump power, and losses. We measure a pump-generated noise spectral density of 4913 counts/s/nm, which can be attributed to the anti-Stokes Raman scattering, in line with other one-stage demonstrations, though higher by an order of magnitude than that obtained in two-stage conversion. Without extra filtering, we expect this to lead to a networking photon signal-to-noise ratio of above 7000 for cavity-integrated SiVs in emission-based schemes.
Signal photons emitted by quantum nodes typically fall outside the low-loss telecom window of optical fibers, leading to severe transmission losses. Quantum frequency conversion (QFC) offers an effective optical interface that bridges quantum nodes with telecom-band channels, enabling long-distance quantum communication. In this work, we demonstrate a compact, fiber-integrated QFC system with low noise and a high signal-to-noise ratio (SNR). Using a periodically poled lithium niobate (PPLN) waveguide, input photons at 637.2 nm are down-converted to telecom photons at 1588.3 nm. Our system achieves a total conversion efficiency of approximately 9%, with pump-induced noise suppressed to 154 Hz. For input photon rates of 32.7, 118.0, and 327.7 kHz, the corresponding SNRs are 12.3, 43.9, and 117.8, respectively. We further develop a theoretical model to simulate the entanglement fidelity between nitrogen-vacancy (NV) center spins and the frequency-converted telecom photons. At the emission rate of an NV center, our QFC system maintains an expected fidelity exceeding 52% over a transmission distance of 100 km. These findings highlight the potential of our QFC system for scalable, long-distance quantum networking.