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Optical Interference Coatings

Dielectric Thin Films to take up the microcavity challenges?

Hervé Rigneault, S. Robert, Claude Amra, C. Begon, Jean‐Michel Gérard

Published Jan 1, 1997• 0 citations
Publisher

Abstract

Spontaneous emission control for luminescent species located inside multilayer dielectric thin films is investigated theoretically in the framework of classical and quantum electrodynamics. Theory is compared to experimental results concerning rare earth ions implanted inside Ta2O5/SiO2 microcavities. We show that although the planar cavities can control the radiation pattern of sources, these structures are unable to affect significantly the atomic lifetime. The first attempts to etch 3D microcavities are presented.

DOI
10.1364/oic.1998.tue.3

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Physical Review A•Feb 1, 1997•46 citations
Spontaneous emission control for luminescent species located inside multilayer dielectric thin films is investigated theoretically in the framework of classical and quantum electrodynamics. Theory is compared to experimental results concerning rare earth ions implanted inside Ta2O5/SiO2 microcavities. We show that although the planar cavities can control the radiation pattern of sources, these structures are unable to affect significantly the atomic lifetime. The first attempts to etch 3D microcavities are presented.
We investigate theoretically and experimentally the optical properties of planar Ta2O5/SiO2 multilayer structures implanted with rare earth ions such as erbium and praseodymium. We demonstrate that the spontaneous emission can be strongly enhanced in a direction normal to the layers if the luminescent ions are located in the spacer of a resonant Fabry-Perot type microcavity. Nevertheless, we show that a large amount of light is emitted into the guided modes of the planar stack reducing the optical confinement which is likely to be reached within this type of dielectric microcavities.
Spontaneous emission control around 490 nm for praseodymium ions implanted inside planar dielectric structures, such as microcavities, is investigated and compared with a theory. Using an Ar+ laser at 457.9 nm as the pump beam, we demonstrate the existence of an optimal pumping angle. Furthermore, we obtain enhanced and directive radiation patterns for the wavelength at which the cavities are tuned (490 nm) and underline very wavelength-dependent behavior of the patterns. In any case, good agreement is obtained between experiment and theory when we take the intrinsic Pr spectrum of emission into account independently of the structures’ influence.
We study lifetime modifications induced by luminescent microcavities in the case of praseodymium-doped planar Ta2O5–SiO2 multidielectric structures. From the experimental point of view we measure different decay times of the 1D2 excited level for different wavelengths in the inhomogeneous praseodymium emission spectrum. Decay times depend on the spectral detuning between considered ions and the cavity, and we observe significant changes around the resonance wavelength of the microcavity. The decay times are explained with an electromagnetic modal analysis of spontaneous emission developed in the case of less-loss microcavities.
The spontaneous emission lifetime and intensity of Er implanted into SiO2{\mathrm{SiO}}_{2}SiO2​ is modified by a Si/SiO2{\mathrm{SiO}}_{2}SiO2​ planar microcavity. The cavity strongly affects the coupling of the optically excited Er3+{\mathrm{Er}}^{3+}Er3+ to the radiative and waveguiding modes of the system, resulting in a spontaneous lifetime of 14.8 ms for a cavity off-resonance with the Er3+{\mathrm{Er}}^{3+}Er3+ versus a lifetime of 9.1 ms for an on-resonance cavity. The observed spontaneous emission lifetime changes agree well with calculated values based on a computation method which is also presented.
Spontaneous emission of erbium atoms implanted in various planar multidielectric stacks is investigated. Computational and experimental analyses are performed so as to assess the amount of light leaking into the radiative and the guided modes of the structures. The key point is the demonstration of the dominant emission into the guided modes, even though the atoms are implanted in the spacer of a resonant microcavity structure. The result is of practical interest since it challenges the conventional idea about the electromagnetic confinement, which is likely to be reached within planar microcavities.