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Annual Meeting Optical Society of America

Single cell Brillouin enhanced four-wave mixing with focusing geometry

Y. S. Kuo, Y. Fong, C. Wu, John Gerard McInerney, J. K. McIver

Published Jan 1, 1992• 0 citations
Publisher

Abstract

Brillouin enhanced four-wave mixing (BEFWM) is a judicious combination of SBS and FWM processes. In the traditional BEFWM experiments, two cells are used: one generates SBS, the other provides four-wave mixing. We demonstrated the generation of a phase conjugate signal by single cell BEFWM with focusing geometry. A single cell containing the optical nonlinear medium was used simultaneously for conventional SBS and FWM. Experiments were performed by using either CS2 or TiCl4 as the nonlinear medium; both have large Brillouin gain but differ greatly in their nonlinear indices of refraction. Thus the mechanism for four-wave mixing is shown to be Brillouin nonlinearity. In this experiment, the phase matching condition was satisfied and the frequency of the phase conjugate signal was not shifted from that of the master input beam. The operating regime of the experiment was far below the threshold of instability, which accounts for the low reflectivity that we observed. This single cell configuration is more compact and the optical alignment is easier than in the conventional BEFWM, in which two nonlinear cells are used.

DOI
10.1364/oam.1992.thw35

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Brillouin enhanced four-wave mixing (BEFWM) is a judicious combination of SBS and FWM processes. In the traditional BEFWM experiments, two cells are used: one generates SBS, the other provides four-wave mixing. We demonstrated the generation of a phase conjugate signal by single cell BEFWM with focusing geometry. A single cell containing the optical nonlinear medium was used simultaneously for conventional SBS and FWM. Experiments were performed by using either CS2 or TiCl4 as the nonlinear medium; both have large Brillouin gain but differ greatly in their nonlinear indices of refraction. Thus the mechanism for four-wave mixing is shown to be Brillouin nonlinearity. In this experiment, the phase matching condition was satisfied and the frequency of the phase conjugate signal was not shifted from that of the master input beam. The operating regime of the experiment was far below the threshold of instability, which accounts for the low reflectivity that we observed. This single cell configuration is more compact and the optical alignment is easier than in the conventional BEFWM, in which two nonlinear cells are used.
Brillouin enhanced four-wave mixing (BEFWM) is a judicious combination of SBS and FWM processes. Very high phase conjugate reflectivity (>106) has been reported. Various conditions have been presented that lead to these high reflectivities, but all those discussions are based on a single mode laser. Here we report the experimental results of BEFWM with a multimode laser. The laser mode spacing is 0.15 GHz, which is larger than the linewidth of the acoustic phonon (0.1 GHz), so we can neglect the gratings that are not resonant with the acoustic frequency. We observed that the phase conjugate reflectivity is smaller for the multimode pump. Assume there is no coupling between modes through BEFWM and each mode interacts with the nonlinear medium independently. It has been shown that the reflectivity will decrease as the input pump power decreases. Thus the reflectivity of a single mode pump is higher than the resultant reflectivity from a multimode pump. Further examination of the temporal profiles of the probe and phase conjugate pulses in the multimode case shows that the pulse modulation depth is decreased in the phase conjugate pulse.
The results of an experimental investigation of a new geometry for producing phase conjugation by Brillouin-enhanced four-wave mixing are presented. In this geometry, the four-wave mixing medium is carbon disulfide, and the backward-going pump wave is created from the transmitted forward-going pump wave by stimulated Brillouin scattering (SBS) in glycerol. The two pump waves are hence phase conjugates of each other, and the quality of the phase-conjugation process is not degraded even by the use of an aberrated pump wave. The probe wave is created by SBS in carbon disulfide, which has a Brillouin frequency half that of glycerol, and the conjugate wave is therefore generated at the same frequency as the probe. Since the pump and signal waves differ in frequency by the Brillouin frequency of the carbon disulfide four-wave mixing medium, high reflectivities (approximately 2000%) are obtained as a result of Brillouin resonance enhancement.
We present the results of an experimental investigation of a polarization-decoupled Brillouin-enhanced four-wave mixing (BEFWM) configuration used for short-pulse high-resolution imaging. In this geometry, the four-wave mixing medium is carbon disulphide (CS2) and the counterpropagating pump is generated from the forward pump by stimulated Brillouin scattering in a second CS2 cell. This configuration produced a good quality, high resolution (∼9 μm) phase conjugate image of a United States Air Force test chart, correcting for aberrations in the system.
Details of the frequency relationships among interacting beams in Brillouin enhanced four-wave mixing (BEFWM) are examined. A new technique using two individually injection-seeded single-mode lasers allows for precise control and knowledge of the relative wavelengths of the interacting beams. This is compared with the standard frequency-shifting technique employing a single laser in conjunction with stimulated Brillouin scattering (SBS) frequency shifters. A continuously tunable frequency difference ranging over many gigahertz is achieved, resulting in a valuable tool for the investigation of nondegenerate four-wave mixing processes such as BEFWM. Two variations of BEFWM are studied: ωpump1 − ωpump2 = 0 with noncollinear pumps; and ωpump1 − ωpump2 = ωSBS with collinear pumping. Resonance spectra of BEFWM gain versus probe–pump frequency shift show a significant detuning in the frequency for the gain maximum from the expected Brillouin shift for the former case. When the probe–pump frequency is tuned in compensation for this detuning, improvements in BEFWM phase conjugation are realized in comparison with more conventional techniques using SBS frequency shifting.
We present a theoretical treatment of four-wave mixing (FWM) in a Brillouin-active medium for the case in which the pump waves differ in frequency by approximately twice the Brillouin frequency shift of the medium and in which the probe-wave frequency is approximately the arithmetic mean of the frequencies of the two pump waves. Under these conditions, the conjugate wave produced by the FWM process has the desirable property of being at the same frequency as the probe. We derive the coupled amplitude equations describing this interaction. We solve these equations analytically in the limit of negligible pump depletion and find that large phase conjugate reflectivities are readily achievable. The coupled amplitude equations are solved numerically for the general case, and it is found that large power transfer from the pumps to the output wave is possible. The output wave is shown to be a nearly perfect phase conjugate of the probe wave, even far into the regime where pump depletion effects are important. Our formalism predicts the existence of a parametric instability in the propagation of the pump waves, but good performance is predicted before the onset of this instability.