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IEEE Journal of Quantum Electronics

Non-frequency-shifted phase conjugation by Brillouin-enhanced four-wave mixing

Paul Narum, Robert W. Boyd

Published Jul 1, 1987• 15 citations
Publisher

Abstract

We present a theoretical treatment of four-wave mixing (FWM) in a Brillouin-active medium for the case in which the pump waves differ in frequency by approximately twice the Brillouin frequency shift of the medium and in which the probe-wave frequency is approximately the arithmetic mean of the frequencies of the two pump waves. Under these conditions, the conjugate wave produced by the FWM process has the desirable property of being at the same frequency as the probe. We derive the coupled amplitude equations describing this interaction. We solve these equations analytically in the limit of negligible pump depletion and find that large phase conjugate reflectivities are readily achievable. The coupled amplitude equations are solved numerically for the general case, and it is found that large power transfer from the pumps to the output wave is possible. The output wave is shown to be a nearly perfect phase conjugate of the probe wave, even far into the regime where pump depletion effects are important. Our formalism predicts the existence of a parametric instability in the propagation of the pump waves, but good performance is predicted before the onset of this instability.

DOI
10.1109/jqe.1987.1073474

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It has previously been shown that Brillouin enhanced four-wave mixing can lead to large phase conjugate reflectivities for moderate laser powers.1,2 However, in the geometry considered by previous workers the pumps have equal frequency and hence the conjugate signal is shifted in frequency with respect to the probe. We have conducted an experimental and theoretical study of Brillouin-enhanced four-wave mixing for the different case in which the two pump waves differ in frequency by twice the Brillouin frequency of the four-wave mixing medium, and in which the probe wave frequency is halfway between those of the pump waves. In this case, the phase conjugate wave has the same frequency as the probe. Reflectivities > 100 % have been measured. Experimental results are compared to those of a theory that includes the effects of phase mismatch, pump depletion, and the finite response time of the medium.

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We present a theoretical treatment of four-wave mixing (FWM) in a Brillouin-active medium for the case in which the pump waves differ in frequency by approximately twice the Brillouin frequency shift of the medium and in which the probe-wave frequency is approximately the arithmetic mean of the frequencies of the two pump waves. Under these conditions, the conjugate wave produced by the FWM process has the desirable property of being at the same frequency as the probe. We derive the coupled amplitude equations describing this interaction. We solve these equations analytically in the limit of negligible pump depletion and find that large phase conjugate reflectivities are readily achievable. The coupled amplitude equations are solved numerically for the general case, and it is found that large power transfer from the pumps to the output wave is possible. The output wave is shown to be a nearly perfect phase conjugate of the probe wave, even far into the regime where pump depletion effects are important. Our formalism predicts the existence of a parametric instability in the propagation of the pump waves, but good performance is predicted before the onset of this instability.
It has previously been shown that Brillouin enhanced four-wave mixing can lead to large phase conjugate reflectivities for moderate laser powers.1,2 However, in the geometry considered by previous workers the pumps have equal frequency and hence the conjugate signal is shifted in frequency with respect to the probe. We have conducted an experimental and theoretical study of Brillouin-enhanced four-wave mixing for the different case in which the two pump waves differ in frequency by twice the Brillouin frequency of the four-wave mixing medium, and in which the probe wave frequency is halfway between those of the pump waves. In this case, the phase conjugate wave has the same frequency as the probe. Reflectivities > 100 % have been measured. Experimental results are compared to those of a theory that includes the effects of phase mismatch, pump depletion, and the finite response time of the medium.
The results of an experimental investigation of a new geometry for producing phase conjugation by Brillouin-enhanced four-wave mixing are presented. In this geometry, the four-wave mixing medium is carbon disulfide, and the backward-going pump wave is created from the transmitted forward-going pump wave by stimulated Brillouin scattering (SBS) in glycerol. The two pump waves are hence phase conjugates of each other, and the quality of the phase-conjugation process is not degraded even by the use of an aberrated pump wave. The probe wave is created by SBS in carbon disulfide, which has a Brillouin frequency half that of glycerol, and the conjugate wave is therefore generated at the same frequency as the probe. Since the pump and signal waves differ in frequency by the Brillouin frequency of the carbon disulfide four-wave mixing medium, high reflectivities (approximately 2000%) are obtained as a result of Brillouin resonance enhancement.
Brillouin enhanced four-wave mixing (BEFWM) is a judicious combination of SBS and FWM processes. Very high phase conjugate reflectivity (>106) has been reported. Various conditions have been presented that lead to these high reflectivities, but all those discussions are based on a single mode laser. Here we report the experimental results of BEFWM with a multimode laser. The laser mode spacing is 0.15 GHz, which is larger than the linewidth of the acoustic phonon (0.1 GHz), so we can neglect the gratings that are not resonant with the acoustic frequency. We observed that the phase conjugate reflectivity is smaller for the multimode pump. Assume there is no coupling between modes through BEFWM and each mode interacts with the nonlinear medium independently. It has been shown that the reflectivity will decrease as the input pump power decreases. Thus the reflectivity of a single mode pump is higher than the resultant reflectivity from a multimode pump. Further examination of the temporal profiles of the probe and phase conjugate pulses in the multimode case shows that the pulse modulation depth is decreased in the phase conjugate pulse.
We have derived an analytic expression for the intensity distribution of two counterpropagating waves of arbitrary input intensity in a saturable absorber. We use this distribution to extend the theory of degenerate four-wave mixing to include the effects of pump wave absorption. In particular, the spatial variation of the nonlinear absorption and coupling constants that appear in the coupled-amplitude equations for the probe and the signal (i.e., conjugate) waves are determined. These coupled-amplitude equations are solved numerically in a noniterative manner, leading to a prediction for the phase-conjugate reflectivity. The nature of the predictions differs qualitatively from those1,2 derived from theories that ignore pumpwave absorption, especially for the case of off-line-center excitation. At large values of the input pump intensities, the phase conjugate reflectivity can be larger than that predicted by theories that ignore pump-wave absorption.