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Annual Meeting Optical Society of America

Dynamics of the spontaneous emission of an atom into the photon-density-of-states gap

Javier J. Sanchez-Mondragon, Rashit F. Nabiev

Published Jan 1, 1992• 1 citation
Publisher

Abstract

We consider the dynamics of the spontaneous emission of a two-level atom embedded into a periodic layered dielectric structure. When the resonant atomic frequency lies within the photon-density-of-states gap (DOS) of width Γ, the atom spontaneous emission becomes fully inhibited for times tΓ ≥ 1. We discuss its enhancing by tuning the atomic resonance with a one mode microcavity. In the λ/4 shifted distributed feedback microcavities, which possess a δ function in the DOS, the spontaneous emission has damped Rabi oscillations and the damping depends on r and the gap depth.

DOI
10.1364/oam.1992.fee2

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Chinese Physics B•Sep 23, 2016•4 citations
We consider the dynamics of the spontaneous emission of a two-level atom embedded into a periodic layered dielectric structure. When the resonant atomic frequency lies within the photon-density-of-states gap (DOS) of width Γ, the atom spontaneous emission becomes fully inhibited for times tΓ ≥ 1. We discuss its enhancing by tuning the atomic resonance with a one mode microcavity. In the λ/4 shifted distributed feedback microcavities, which possess a δ function in the DOS, the spontaneous emission has damped Rabi oscillations and the damping depends on r and the gap depth.
We consider the process of spontaneous emission of a two-level atom embedded into a periodic layered dielectric structure. When the resonant atomic frequency lies within the photon-density-of-states gap, of width \ensuremath{\Gamma}, the atom emits light during a time interval t\ensuremath{\Gamma}\ensuremath{\ll}1 until the spontaneous emission becomes fully inhibited. We discuss the enhancing of spontaneous emission by tuning the atomic resonance with a one-mode microcavity. In the \ensuremath{\lambda}/4-shifted distributed feedback microcavities which possess the \ensuremath{\delta}-function-like density of states, in the middle of the gap, the process of spontaneous emission has damped Rabi oscillation behavior; the damping depends on the width of the gap and the height of its walls. A profile of the density-of-states gap can be determined from the experimental data on the temporal behavior of the atomic spontaneous decay.
The time-dependent spectral properties and nonlinear dynamics of a spontaneous photon emitted by two level atom, trapped in damped nanocavity and coupled to a single resonance mode, have been investigated. The results have been obtained with the help of new nonperturbative approach by solving exactly the Schrödinger equation. The theory accounts exactly and simultaneously processes of emission, reabsorptions and leakage of photon. The solution was found with the Green functions formalism, supplemented with the novel algorithm in operating causal singular functions and fundamentals of the theory of quasi-stationary systems. The obtained distributions and emission dynamics are presented with plots as functions of photon frequency detuning and time for various value Γ/4g. For Γ/4g <1 the spectrum is a triplet inside the cavity and doublet outside it. In this case the total emission probability is described by decaying oscillations. For Γ/4g ≥ 1 and Γ/4g >> 1 the spectrum consists of a single central line decaying exponentially with profile depending on value Γ/4g.
The nonperturbative theory of the cooperative spontaneous emission from a two level atom trapped in one-dimensional damped nanocavity with a single resonance mode is presented. The time-dependent spectral properties and nonlinear dynamics of a separate photon emission by the macroolecular-like system "excited atom coupled to a resonance decaying mode" have been analyzed. The investigation has been carried out by solving the Schrödinger equation in the interaction picture with the help of the Green functions method in the Heitler-Ma's form . The formalism was supplemented with the novel algorithm in operating causal singular functions and with fundamentals of the theory of quantum quasi-stationary systems. The proposed theory accounts automatically of both reabsorptions of emitted photon and its simultaneous escaping out of the cavity. Solutions of the wave equation were found without using intermediate virtual states and series expansions. In accordance with the theory of quasistationary systems the field of mode decaying exponentially in the empty nanocavity was represented with the Lorenz-shaped packet of stationary photonic states (quasi-modes). The electro-dipolar interaction between the atom and the mode field was adopted to be switched on suddenly. The expressions and plots of emission spectral densities probabilities together with photon emission probability dynamics as functions of time for various ratios Γ/4g. For Γ/4g<1 the transient emission spectrum reveals the presence of two symmetrical side-bands and the central peak interconnected with each other in the area of interaction with the atom. Since the central component oscillates, decaying simultaneously in time at two rates infinity Γ/2 and ~ Γ/4, in the area of interaction the emission is a triplet with satellites oscillating in the interaction area and being stable outside of it. So the final spectrum is a doublet outside of nanocavity. On the contrary for Γ/4g ≥1 the spectrum is a singlet, and the emission occurs in exponentially decaying way.
Dynamics of the spontaneous emission from a two-level atom embedded in a bisphere microcavity is analyzed theoretically. A bisphere supports a morphology-dependent resonance having such a high quality factor with local field enhancement that the strong coupling between the atom and the cavity can be realized. By taking full account of the photon degree of freedom, we derive theoretically the coupling constant between the atom and the cavity as well as the radiation damping constants, which are used in the conventional cavity QED approach. In addition, we show that the power spectrum of the spontaneous emission at a local observation point is strongly affected by the photon Green function.
The nonperturbative theory of the cooperative spontaneous emission from a two level atom trapped in one-dimentional damped nanocavity with a single resonance mode is presented. The time-dependent spectral properties and nonlinear dynamics of a separate photon emission by the micro-molecular-like system "excited atom coupled to a resonance decaying mode" have been analyzed. The investigation has been carried out by solving the Schrödinger equation in the interaction picture with the help of the Green functions method in the Heitler-Ma's form. The formalism was supplemented with the novel algorithm in operating causal singular functions and with fundamentals of the theory of quasi-stationary systems. The proposed theory accounts automatically of both reabsorptions of emitted photon and its simultaneous escaping out of the cavity. Solutions of the wave equation were found without using intermediate virtual states and series expansions. In accordance with the theory of quasi-stationary systems the field of mode decaying exponentially in the empty nanocavity was represented with the Lorenz-shaped packet of stationary photonic states (quasi-modes). The electro-dipolar interaction between the atom and the mode field was adopted to be switched on suddenly. The expressions and plots of emission probabilities spectral densities together with photon emission probability dynamics as functions of time for various ratios Γ/4g of photon escaping rate Γ and coupling constant g are presented. For Γ/4g <1 the transient emission spectrum reveals the presence of two symmetrical side-bands and of the central peak, the latter decaying in time at the rate ∝ Γ/2 so that the final spectrum is a doublet. In this case the photon emission probability is described by decaying oscillations. On the contrary for Γ/4g ≥ 1 the spectrum is a singlet and the emission occurs in exponentially decaying ways.
The spontaneous emission from a microwave-driven four-level atom embedded in an anisotropic photonic crystal is studied. Due to the modified density of state (DOS) in the anisotropic photonic band gap (PBG) and the coherent control induced by the coupling fields, spontaneous emission can be significantly enhanced when the position of the spontaneous emission peak gets close to the band gap edge. As a result of the closed-loop interaction between the fields and the atom, the spontaneous emission depends on the dynamically induced Autler–Townes splitting and its position relative to the PBG. Interesting phenomena, such as spectral-line suppression, enhancement and narrowing, and fluorescence quenching, appear in the spontaneous emission spectra, which are modulated by amplitudes and phases of the coherently driven fields and the effect of PBG. This theoretical study can provide us with more efficient methods to manipulate the atomic spontaneous emission.