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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Spectral properties and nonlinear dynamics of spontaneous emission of a resonance photon by two-level atom trapped in damped nanocavity with a resonance mode

Vladislav Cheltsov

Published Aug 20, 2009• 1 citation
Publisher

Abstract

The time-dependent spectral properties and nonlinear dynamics of a spontaneous photon emitted by two level atom, trapped in damped nanocavity and coupled to a single resonance mode, have been investigated. The results have been obtained with the help of new nonperturbative approach by solving exactly the Schrödinger equation. The theory accounts exactly and simultaneously processes of emission, reabsorptions and leakage of photon. The solution was found with the Green functions formalism, supplemented with the novel algorithm in operating causal singular functions and fundamentals of the theory of quasi-stationary systems. The obtained distributions and emission dynamics are presented with plots as functions of photon frequency detuning and time for various value Γ/4g. For Γ/4g <1 the spectrum is a triplet inside the cavity and doublet outside it. In this case the total emission probability is described by decaying oscillations. For Γ/4g ≥ 1 and Γ/4g >> 1 the spectrum consists of a single central line decaying exponentially with profile depending on value Γ/4g.

DOI
10.1117/12.819877

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The time-dependent spectral properties and nonlinear dynamics of a spontaneous photon emitted by two level atom, trapped in damped nanocavity and coupled to a single resonance mode, have been investigated. The results have been obtained with the help of new nonperturbative approach by solving exactly the Schrödinger equation. The theory accounts exactly and simultaneously processes of emission, reabsorptions and leakage of photon. The solution was found with the Green functions formalism, supplemented with the novel algorithm in operating causal singular functions and fundamentals of the theory of quasi-stationary systems. The obtained distributions and emission dynamics are presented with plots as functions of photon frequency detuning and time for various value Γ/4g. For Γ/4g <1 the spectrum is a triplet inside the cavity and doublet outside it. In this case the total emission probability is described by decaying oscillations. For Γ/4g ≥ 1 and Γ/4g >> 1 the spectrum consists of a single central line decaying exponentially with profile depending on value Γ/4g.
The nonperturbative theory of the cooperative spontaneous emission from a two level atom trapped in one-dimentional damped nanocavity with a single resonance mode is presented. The time-dependent spectral properties and nonlinear dynamics of a separate photon emission by the micro-molecular-like system "excited atom coupled to a resonance decaying mode" have been analyzed. The investigation has been carried out by solving the Schrödinger equation in the interaction picture with the help of the Green functions method in the Heitler-Ma's form. The formalism was supplemented with the novel algorithm in operating causal singular functions and with fundamentals of the theory of quasi-stationary systems. The proposed theory accounts automatically of both reabsorptions of emitted photon and its simultaneous escaping out of the cavity. Solutions of the wave equation were found without using intermediate virtual states and series expansions. In accordance with the theory of quasi-stationary systems the field of mode decaying exponentially in the empty nanocavity was represented with the Lorenz-shaped packet of stationary photonic states (quasi-modes). The electro-dipolar interaction between the atom and the mode field was adopted to be switched on suddenly. The expressions and plots of emission probabilities spectral densities together with photon emission probability dynamics as functions of time for various ratios Γ/4g of photon escaping rate Γ and coupling constant g are presented. For Γ/4g <1 the transient emission spectrum reveals the presence of two symmetrical side-bands and of the central peak, the latter decaying in time at the rate ∝ Γ/2 so that the final spectrum is a doublet. In this case the photon emission probability is described by decaying oscillations. On the contrary for Γ/4g ≥ 1 the spectrum is a singlet and the emission occurs in exponentially decaying ways.
The nonperturbative theory of the cooperative spontaneous emission from a two level atom trapped in one-dimensional damped nanocavity with a single resonance mode is presented. The time-dependent spectral properties and nonlinear dynamics of a separate photon emission by the macroolecular-like system "excited atom coupled to a resonance decaying mode" have been analyzed. The investigation has been carried out by solving the Schrödinger equation in the interaction picture with the help of the Green functions method in the Heitler-Ma's form . The formalism was supplemented with the novel algorithm in operating causal singular functions and with fundamentals of the theory of quantum quasi-stationary systems. The proposed theory accounts automatically of both reabsorptions of emitted photon and its simultaneous escaping out of the cavity. Solutions of the wave equation were found without using intermediate virtual states and series expansions. In accordance with the theory of quasistationary systems the field of mode decaying exponentially in the empty nanocavity was represented with the Lorenz-shaped packet of stationary photonic states (quasi-modes). The electro-dipolar interaction between the atom and the mode field was adopted to be switched on suddenly. The expressions and plots of emission spectral densities probabilities together with photon emission probability dynamics as functions of time for various ratios Γ/4g. For Γ/4g<1 the transient emission spectrum reveals the presence of two symmetrical side-bands and the central peak interconnected with each other in the area of interaction with the atom. Since the central component oscillates, decaying simultaneously in time at two rates infinity Γ/2 and ~ Γ/4, in the area of interaction the emission is a triplet with satellites oscillating in the interaction area and being stable outside of it. So the final spectrum is a doublet outside of nanocavity. On the contrary for Γ/4g ≥1 the spectrum is a singlet, and the emission occurs in exponentially decaying way.
Nonperturbative theoretical analysis of the temporal evolution of a spontaneous photon with atomic frequency ωa, emitted by a motionless two-level atom in a one-dimensional high-finesse nanocavity into a single resonance decaying mode, is presented. The explicit solution of the Schrödinger equation was found in an interaction picture with use of the Green functions technique. It has been assumed that emission leaks out of the empty cavity by exponential law at rate Γ, which is a function of coupling constant g, distance between the mirrors, penetrability coefficient of the left mirror, and the velocity of light. The stationary superpositional co-phased structure of two photons with the same profiles and average frequencies 1/2(ωa ± g), quenched with continuum of final photonics states, has been revealed. The profile of this structure has been found to have the form Γt exp(−Γt/4) with maximum attained for Γ/4g = 0.05 and average photon cavity lifetime equal to 4lnΓ/ Γ.
The entangled photons components are found to be created in the lossless nanocavity with resonance mode. The smallness of Γ ( 0 ≤ Γ<< g- coupling constant for electro-dipolar interaction) was revealed playing the crucial part in their production. It’s known that Г determines limits (ωc ± Γ) of photon frequency deflection from the mode frequency ωc, when photon passes through empty cavity. When Γ = 0 and ωa=ωc , the Hamiltonian is time independent and has two eigenstates with eigenvalies (ωa ± g). Each state is superposition of the upper and lower atomic states, taken with signs plus and minus respectively. These states are stationary and form a time-depended superposition. Matrix elements of the interaction Hamiltonian, taken between that superposition and atomic unperturbed states, contain two anti-phases components of entangled photons. Since Γ = 0, their emission out of cavity is forbidden so they interfere, producing beatings of the resonance mode by sin (g•t). When 0 < Γ<< g those beatings become quasi-stationary, and with probability proportional to Γ/4g they go out through the partly transparent mirror and disintegrate into two photons, each of them taking its own spectral place outside the cavity. This process is illustrated by 3D-plots in the (ω, t)-space.
The spontaneous emission spectrum from two quantum dots (QDs) that are strongly coupled with a single-mode nanocavity is investigated using rigorous numerical calculations and simple analytical solutions of quantum dynamics. The emission spectra both from the side and along the axis of the cavity are considered. Modification of two parameters, the coupling strength and the detuning between the transition frequencies of the two quantum dots, allows us to efficiently control the shape of the spontaneous emission spectrum. Different profiles and their physical origins can be well understood in the dressed-state picture for the light—QD interaction in the on-resonance and off-resonance situations. In the on-resonance situation, the emission spectra exhibit symmetric features, and they are not altered by the asymmetry in the coupling parameters. The axis spectra show two emission peaks while the side spectra have three emission peaks. In the off-resonance situation, the emission spectra always show an asymmetrical three-peak feature. When the two QDs have different decay parameters, singular features (a peak or a dip) can take place at the frequency of the cavity mode, and this is attributed to the unbalanced process of the emission and absorption of a single photon.
The new cooperative nonlinear effects in emission and absorption of resonance photon by two level atoms trapped in damped single-mode one-dimensional microcavity have been revealed and investigated nonpertubatibely. Two cases have been considered: the case of an excited ultracold atom localized initially in the ground vibrational state of the trap's parabolic well and the case of one and two two level motionless atoms in diferent initial states. The dynamics and spectrum of emission (absorption) have been shown to be determined in particular by o --the rate of decaying of mode in the empty cavity. The gigantic optical ''Moessbauer'' effect has been discovered under resonance condition \omega _v=2g . Out of this condition there arise numerous resonances of the higher order on different frequencies so that one thermal impulse has been observed instead of the ''Moessbauer peak''. In the case of two motonless atoms non-emitting (''dark'') antisymmetric and emitting (''luminous'') symmetric atomic superpositional states have been revealed.