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Nonlinear Dynamics in Optical Systems

Dynamic Optical Bistabilities in ZnSe/ZnS Multiple Quantum Wells

Yudong Liu, Xiangming Yang, Chunfei Li, Dezhen Shen, Xiwu Fan, Guanghan Fan, Lianchun Chen

Published Jan 1, 1990• 0 citations
Publisher

Abstract

The excitonic optical nonlinearities in II-VI semiconductor thin films and multiple quantum wells (MQWs) are much complicated than those of GaAs MQWs because the wider band gap and smaller excitons of II-VI semiconductor materials. We report here the observations of dynamic optical bistabilities in ZnSe/ZnS MQWs at low temperature caused by excitonic optical nonlinearity.

DOI
10.1364/nldos.1990.tdsls63

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The excitonic optical nonlinearities in II-VI semiconductor thin films and multiple quantum wells (MQWs) are much complicated than those of GaAs MQWs because the wider band gap and smaller excitons of II-VI semiconductor materials. We report here the observations of dynamic optical bistabilities in ZnSe/ZnS MQWs at low temperature caused by excitonic optical nonlinearity.
The excitonic nonlinearities in II-VI wide gap semiconductors have recently become an interesting research topic. Andersen et al.1 studied the saturating absorption of excitonic resonance in ZnSe single crystal films and (Zn, Mn)Se superlattices, which they attributed to Coulombic screening for the case of ZnSe film or a wide-well (Zn,Mn)Se quantum well structure at 77 K, and the Coulombic screening and phase space filling for a narrow-well structure. Gribkovskii et al.2 have observed the increase of excitonic absorption optical bistability in ZnSe film and attributed it to excitonic broadening and gap renormalization for the nonlinear mechanism. We report the first observation of optical bistability in ZnSe/ZnS MQWs grown by MOCVD on CaF2 substrates.
Excitonic optical bistability with nanosecond switching time in ZnSe-ZnS multiple quantum wells (MQWs) with a Fabry-Perot (FP) cavity is investigated at room temperature. The research result indicates that the threshold and contrast ratio for the optical bistability in ZnSe-ZnS MQWs with a FP cavity are about 0.2 MW/cm2 and 6:1, respectively. On the basis of the room temperature excitonic absorption spectra obtained here, we attribute the major nonlinear mechanism for the optical bistability to the excitonic saturating absorption due to phase space filling of excitonic states and excitonic band broadening.
The excitonic nonlinear refractive index was calculated by using Kramers-Kronig relation and the saturating absorption of ZnSe/CdZnSe multiple quantum wells (MQWs) was studied under different pump intensities. The maximum nonlinear refractive index change is about -6.19 X 10-3. Excitonic optical bistability in ZnSe/CdZnSe MQWs is investigated at room temperature. The result indicates that the threshold and contrast ratio for the optical bistability in ZnSe/CdZnSe MQWs are about 210Kw/cm2 and 2:1, respectively. On the basis of the excitonic nonlinear theories and excitonic absorption spectra in the ZnSe/CdZnSe MQWs, we attribute the major nonlinear mechanism of the optical bistability in the ZnSe/CdZnSe MQWs to the phase space filling of excitonic states and excitonic band broadening due to exciton-exciton interactions.