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Physical Review Applied

Orbital-Angular-Momentum Quantum State Transformation Via a Nonlinear Process

Zhantong Qi, Yiwen Huang, Chuanyi Lu, Fengchao Ni, Yuanhua Li, Yuanlin Zheng, Xianfeng Chen

Published Jan 17, 2023• 10 citations
Publisher

Abstract

Orbital-angular-momentum- (OAM) based photonic nonlinear interfaces, such as the nonlinear manipulation of a single-photon OAM state between the communication wavelength for entanglement distribution and the near-visible wavelength for quantum memories. Here, we experimentally demonstrate this kind of quantum state transformation for simultaneously adjusting the weight of the spatial OAM modes and operating the wavelength of single photons by effectively cascading the frequency conversion and electro-optical (EO) polarization coupling in a periodically poled lithium niobate crystal. The fidelity of the OAM state is measured to be higher than 95% before and after the frequency conversion. The results show that the OAM state of single photons can be modulated on demand by applying a transverse electric field across the nonlinear crystal. Our work demonstrates the integration and high performance of our proposed transformation interface, and paves a route toward connecting different remote nodes based on quantum memories in a large-scale OAM-encoded quantum network.

DOI
10.1103/physrevapplied.19.014045

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Orbital-angular-momentum- (OAM) based photonic nonlinear interfaces, such as the nonlinear manipulation of a single-photon OAM state between the communication wavelength for entanglement distribution and the near-visible wavelength for quantum memories. Here, we experimentally demonstrate this kind of quantum state transformation for simultaneously adjusting the weight of the spatial OAM modes and operating the wavelength of single photons by effectively cascading the frequency conversion and electro-optical (EO) polarization coupling in a periodically poled lithium niobate crystal. The fidelity of the OAM state is measured to be higher than 95% before and after the frequency conversion. The results show that the OAM state of single photons can be modulated on demand by applying a transverse electric field across the nonlinear crystal. Our work demonstrates the integration and high performance of our proposed transformation interface, and paves a route toward connecting different remote nodes based on quantum memories in a large-scale OAM-encoded quantum network.
Light-carrying orbital angular momentum (OAM) has great potential in enhancing the information channel capacity in both classical and quantum optical communications. Long distance optical communication requires the wavelengths of light are situated in the low-loss communication windows, but most quantum memories currently being developed for use in a quantum repeater work at different wavelengths, so a quantum interface to bridge the wavelength gap is necessary. So far, such an interface for OAM-carried light has not been realized yet. Here, we report the first experimental realization of a quantum interface for a heralded single photon carrying OAM using a nonlinear crystal in an optical cavity. The spatial structures of input and output photons exhibit strong similarity. More importantly, single-photon coherence is preserved during up-conversion as demonstrated.
The efficient transport and engineering of photonic orbital angular momentum (OAM) lie at the heart of various related classical and quantum applications. Here, by leveraging the spatial-mode-engineered frequency conversion, we realize the remote transport of high-dimensional orbital angular momentum (OAM) states between two distant parties without direct transmission of information carriers. We exploit perfect vortices for preparing high-dimensional yet maximal O AM entanglement. Based on nonlinear sum-frequency generation working with a strong coherent wave packet and a single photon, we conduct the Bell-like state measurements for high-dimensional perfect vortices. We experimentally achieve an average transport fidelity 0.879 ± 0.048 and 0.796 ± 0.066 for a complete set of 3-dimensional and 5-dimensional OAM mutually unbiased bases, respectively. Furthermore, by exploring the full transverse entanglement, we construct another strategy of quantum imaging with interaction-free light. It is expected that, with the future advances in nonlinear frequency conversion, our scheme will pave the way for realizing truly secure high-dimensional quantum teleportation in the upcoming quantum network.
Light carrying orbital angular momentum (OAM) has exciting applications, including the studies of fundamental quantum physics, optical manipulation and trapping of particles, astrophysics, high-precision optical measurements and optical communication, etc. In quantum information field, a photon encoded with information in its OAM degrees of freedom enables networks to carry significantly more information and increase their capacity greatly due to the inherent infinite degrees of freedom for OAM. Therefore it is no surprise that many groups and researchers are active in building up a high-dimensional quantum network and many important progresses have been achieved during the past years. To realize a long-distance quantum communication, a quantum repeater has to be used to overcome the problem of communication fidelity decreasing exponentially with the channel length, where, quantum memories for photons, used for storing quantum information, which have been realized successfully during the past decade in many systems such as a cold/hot atomic system, a solid matter, a diamond, and others, are key components consisting of a quantum repeater. Photons acted as information candidates can connect different quantum repeaters. Long distance quantum communication requires the wavelengths of photons are situated in the low-loss communication windows, but most quantum memories currently being developed for use in a quantum repeater work at different wavelengths, only few memories can work in low-loss communication windows. Furthermore, the signal stored is an attenuated coherent light and has the Gaussian mode. Though the storage of photonic entanglement at telecom wavelength is realized in an erbium-doped optical fibre recently, the spatial mode used is Gaussian mode. Quantum memories for photons with OAM have recently been realized, but all work at different wavelengths. So a quantum interface to bridge the wavelength gap is necessary.
Optical frequency conversion provides a fundamental and important approach to manipulate light in frequency domain. In such a process, manipulating the frequency of light without changing information in other degrees of freedom of light will enable us to establish an interface between various optical systems operating in different frequency regions and have many classical and quantum applications. Here we experimentally demonstrate a frequency conversion with maintaining polarization and orbital angular momentum (OAM) by successfully upconverting various polarization-OAM composite states in a nonlinear Sagnac interferometer. Our scheme offers a new possibility for building different wave band interfaces in more degrees of freedom.
Entanglement is a vital resource for realizing many tasks such as teleportation, secure key distribution, metrology, and quantum computations. To effectively build entanglement between different quantum systems and share information between them, a frequency transducer to convert between quantum states of different wavelengths while retaining its quantum features is indispensable. Information encoded in the photon's orbital angular momentum (OAM) degrees of freedom is preferred in harnessing the information-carrying capacity of a single photon because of its unlimited dimensions. A quantum transducer, which operates at wavelengths from 1558.3 to 525 nm for OAM qubits, OAM-polarization hybrid-entangled states, and OAM-entangled states, is reported for the first time. Nonclassical properties and entanglements are demonstrated following the conversion process by performing quantum tomography, interference, and Bell inequality measurements. Our results demonstrate the capability to create an entanglement link between different quantum systems operating in a photon's OAM degrees of freedom, which will be of great importance in building a high-capacity OAM quantum network.
Frequency interface, namely, converting the colors of photons while retaining their other features, is indispensable for numerous applications ranging from up-conversion imaging to the multimode quantum network. However, limited by the nonuniform nonlinear frequency-conversion efficiency, constructing the frequency interface for high-dimensional spatial modes is still challenging. Here, to break this fundamental barrier, we construct a high-dimensional (HD) orbital-angular-momentum (OAM) frequency interface via conducting sum-frequency generation between HD OAM states to be converted and a radial structured pump. Specifically, by replacing the conventional Gaussian pump with an optimized coherent superposition of HD Laguerre-Gaussian radial modes (i.e., its azimuthal number is zero), we experimentally achieve the OAM frequency interface in nine dimensions with a record fidelity up to 90.38 %. Additionally, by increasing the number of radial modes, our scheme can be flexibly extended to higher dimension. Such a high-dimensional frequency interface could find potential applications in the high-capacity free-space optical communication and would also pave the way for constructing high-dimensional quantum networks.