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Chinese Science Bulletin (Chinese Version)

Frequency conversion of orbital angular momentum carrying photons

Zhi‐Yuan Zhou, Bao-Sen Shi

Published Jul 8, 2016• 2 citations
Publisher

Abstract

Light carrying orbital angular momentum (OAM) has exciting applications, including the studies of fundamental quantum physics, optical manipulation and trapping of particles, astrophysics, high-precision optical measurements and optical communication, etc. In quantum information field, a photon encoded with information in its OAM degrees of freedom enables networks to carry significantly more information and increase their capacity greatly due to the inherent infinite degrees of freedom for OAM. Therefore it is no surprise that many groups and researchers are active in building up a high-dimensional quantum network and many important progresses have been achieved during the past years. To realize a long-distance quantum communication, a quantum repeater has to be used to overcome the problem of communication fidelity decreasing exponentially with the channel length, where, quantum memories for photons, used for storing quantum information, which have been realized successfully during the past decade in many systems such as a cold/hot atomic system, a solid matter, a diamond, and others, are key components consisting of a quantum repeater. Photons acted as information candidates can connect different quantum repeaters. Long distance quantum communication requires the wavelengths of photons are situated in the low-loss communication windows, but most quantum memories currently being developed for use in a quantum repeater work at different wavelengths, only few memories can work in low-loss communication windows. Furthermore, the signal stored is an attenuated coherent light and has the Gaussian mode. Though the storage of photonic entanglement at telecom wavelength is realized in an erbium-doped optical fibre recently, the spatial mode used is Gaussian mode. Quantum memories for photons with OAM have recently been realized, but all work at different wavelengths. So a quantum interface to bridge the wavelength gap is necessary.

DOI
10.1360/n972016-00137

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Light carrying orbital angular momentum (OAM) has exciting applications, including the studies of fundamental quantum physics, optical manipulation and trapping of particles, astrophysics, high-precision optical measurements and optical communication, etc. In quantum information field, a photon encoded with information in its OAM degrees of freedom enables networks to carry significantly more information and increase their capacity greatly due to the inherent infinite degrees of freedom for OAM. Therefore it is no surprise that many groups and researchers are active in building up a high-dimensional quantum network and many important progresses have been achieved during the past years. To realize a long-distance quantum communication, a quantum repeater has to be used to overcome the problem of communication fidelity decreasing exponentially with the channel length, where, quantum memories for photons, used for storing quantum information, which have been realized successfully during the past decade in many systems such as a cold/hot atomic system, a solid matter, a diamond, and others, are key components consisting of a quantum repeater. Photons acted as information candidates can connect different quantum repeaters. Long distance quantum communication requires the wavelengths of photons are situated in the low-loss communication windows, but most quantum memories currently being developed for use in a quantum repeater work at different wavelengths, only few memories can work in low-loss communication windows. Furthermore, the signal stored is an attenuated coherent light and has the Gaussian mode. Though the storage of photonic entanglement at telecom wavelength is realized in an erbium-doped optical fibre recently, the spatial mode used is Gaussian mode. Quantum memories for photons with OAM have recently been realized, but all work at different wavelengths. So a quantum interface to bridge the wavelength gap is necessary.
Abstract Electromagnetic waves have both spin momentum and orbital angular momentum (OAM). Light carrying OAM has broad applications in micro-particle manipulation, high-precision optical metrology, and potential high-capacity optical communications. In the concept of quantum information, a photon encoded with information in its OAM degree of freedom enables quantum networks to carry much more information and increase their channel capacity greatly compared with those of current technology because of the inherent infinite dimensions for OAM. Quantum memories are indispensable to construct quantum networks. Storing OAM states has attracted considerable attention recently, and many important advances in this direction have been achieved during the past few years. Here we review recent experimental realizations of quantum memories using OAM states, including OAM qubits and qutrits at true single photon level, OAM states entangled in a two-dimensional or a high-dimensional space, hyperentanglement and hybrid entanglement consisting of OAM and other degree of freedom in a physical system. We believe that all achievements described here are very helpful to study quantum information encoded in a high-dimensional space.
Light-carrying orbital angular momentum (OAM) has great potential in enhancing the information channel capacity in both classical and quantum optical communications. Long distance optical communication requires the wavelengths of light are situated in the low-loss communication windows, but most quantum memories currently being developed for use in a quantum repeater work at different wavelengths, so a quantum interface to bridge the wavelength gap is necessary. So far, such an interface for OAM-carried light has not been realized yet. Here, we report the first experimental realization of a quantum interface for a heralded single photon carrying OAM using a nonlinear crystal in an optical cavity. The spatial structures of input and output photons exhibit strong similarity. More importantly, single-photon coherence is preserved during up-conversion as demonstrated.
Quantum memory is a key component of quantum networks. A successful development in enabling the distribution of quantum information requires the storage of single-photon light. Usually quantum information is encoded using a 2D space, spanned, for example, by the orthogonal polarization states of a photon. In this case, each photon carries a quantum bit of information. If the photon could be encoded in a high-dimensional space instead, the information carried by each photon could be increased from a bit to |log⁡2d\log {}_2dlog2​d| bits, where d is the dimension of the Hilbert space in which the photon is described. The channel capacity of the network and the transmission efficiency would then be greatly enlarged [1]. Moreover, storing high-dimensional states in quantum memory can reduce its sensitivity to memory coherence time [2], leading to significant improvements in storage capacity [3]. It is thus no surprise that many research groups are actively working on different physical systems for storing light encoded using a high-dimensional space. The degrees of freedom for position, linear momentum, time-bin or orbital angular momentum (OAM) of a photon can all be considered as a high-dimensional space for encoding. The photon's OAM has the most potential for encoding [4]. Electromagnetic waves have both spin and OAM. Spin angular momentum produces polarization. Photons with OAM can be regarded as helices with left and right handedness twisted to varying degrees (Fig. 1). Information is encoded using this handedness and the amount of twist. Because of the inherent infinite degrees of freedom for OAM, a photon can in principle carry an arbitrarily large amount of information, and hence the eagerness to store light encoded in OAM space. Although some work on this has been reported for different physical systems, what is lacking is a way of storing and releasing at some later time a true single photon, including its shape and structure [5–7]. Constructing this basic element of quantum memory has been a major challenge. The wavefront of an OAM light is a helical structure (left and center), with an optical vortex at its center in the intensity distribution of light (right). The vortex of light can carry non-zero OAM of any order m. OAM states of a different order are orthogonal. A group at the Key Laboratory of Quantum Information, Chinese Academy of Science, at the University of Science and Technology of China finally resolved this problem [8]. They reported on the first experimental realization of a true single-photon-carrying OAM stored via electromagnetically induced transparency (EIT) in a cold atomic ensemble (Fig. 2). With such a suitable candidate, this work indicates a means of constructing high-dimensional quantum memory. After this, similar results were reported by Laurat's group at Laboratoire Kastler Brossel, at Université Pierre et Marie Curie in France [9], where an extremely weak laser at single-photon level carrying OAM was also stored via EIT in a cold atomic ensemble. Ding et al. [8] first prepared two cold 85Rb atomic clouds in two magnetic-optical traps (MOT) using laser cooling and trapping techniques. They generated non-classical correlated photon pairs using spontaneous four-wave mixing in an atomic cloud. One photon of each pair was used as a trigger; the other mapped and stored in a second atomic cloud via EIT. Each photon to be stored carried one OAM unit. After a programed storage time, the photon was retrieved. What they achieved during storage included (1) proof that the non-classical correlation between the trigger photon and the retrieved photon is retained by demonstrating a strong violation of the Cauchy–Schwarz inequality, (2) a demonstration that the single-photon property of the signal photon is maintained by performing the Hanbury–Brown and Twiss experiment on the trigger photon, (3) proof that the spatial structure of the photon is also very well preserved by showing a high similarity between input and output, and (4) evidence, gathered by Sagnac interferometry, that the coherence of a single photon is also preserved. A heralded single photon is generated through spontaneous four-wave mixing in MOT 1 (a); this single photon carrying OAM is then stored through EIT in MOT 2 (b); (c) shows an image of the photon carrying OAM. Experimental measurements in the transverse position of the image carried by the photon before and after storage are presented in (d) and (e), respectively; (f) shows the simplified experimental setup for storage of a superposition of OAM. Interference patterns taken at different angle settings of the half-wave plate are shown in (g). The left column represents the experimental angle settings of the half-wave and the quarter-wave plates, the middle column gives the experimental results, and the right column gives results from theoretical simulations; (h) and (i) present the interference patterns of the input signal photon and the retrieved signal with plate angle, respectively. This is a significant breakthrough towards the realization of a quantum internet and, potentially, quantum computing. This work addresses the ability to generate, store, retrieve on demand an arbitrary single-photon-level photonic state encoded in OAM space. It signifies an important step in the development of practical quantum-enabled technologies, opens up the possibility for realizing high-dimensional quantum memories based on this degree of freedom of light, and will have a large impact in a broad physical community, especially in the quantum information and quantum optics communities. The Technology Review website of MIT comments on their work very positively with an article entitled ‘First Quantum Memory That Records the Shape of a Single Photon Unveiled in China’. Further, Nature Photonics selected this work as a research highlight. Clearly, memory that can preserve the spatial structure of photons will make the internet far more flexible and capable. Of course, there are still many basic problems remaining that need to be solved to build the future quantum internet, one of which is the construction of quantum memory exploiting entanglement. This derives from the fact that a quantum network needs the distribution of quantum-entangled photons over channels between different nodes [10]. A high-dimensional quantum internet needs to store OAM-entangled states and perform entanglement swapping to efficiently extend the achievable communication distances. While Ding et al. [8] reported the storage of light with OAM at the single-photon level, the photon was, however, still encoded in a 2D space. Therefore, whether it is possible to construct a high-dimensional quantum memory remains an open issue that needs to be investigated further.
Entanglement is a vital resource for realizing many tasks such as teleportation, secure key distribution, metrology, and quantum computations. To effectively build entanglement between different quantum systems and share information between them, a frequency transducer to convert between quantum states of different wavelengths while retaining its quantum features is indispensable. Information encoded in the photon's orbital angular momentum (OAM) degrees of freedom is preferred in harnessing the information-carrying capacity of a single photon because of its unlimited dimensions. A quantum transducer, which operates at wavelengths from 1558.3 to 525 nm for OAM qubits, OAM-polarization hybrid-entangled states, and OAM-entangled states, is reported for the first time. Nonclassical properties and entanglements are demonstrated following the conversion process by performing quantum tomography, interference, and Bell inequality measurements. Our results demonstrate the capability to create an entanglement link between different quantum systems operating in a photon's OAM degrees of freedom, which will be of great importance in building a high-capacity OAM quantum network.
Quantum memories are indispensible for establishing a long-distance quantum network. High-dimensional quantum memories enable a higher channel capacity compared to a quantum memory working in a two-dimensional space, and have a lower requirement for storage lifetime in the field of quantum coomunication. The photonic transverse spatial modes such as Laguerra-Gaussian modes orbital angular momentum (OAM) are ideal candidates for encoding high-dimensional information, because it can form an infinite-dimensional Hilbert space. Although the faithful storage of an OAM qubit or qutrit has been realized in pioneering works, the longest storage lifetime for the former is only in the order of a few microseconds, and hundreds of nano-seconds for the latter. Here we implement a quantum memory for OAM qubits and qutrits using a cold atomic ensemble, the experimental results clearly show that our memory can still beat the classical limit after a storage time of 400μs400μs400μs,which is two orders of magnitude higher than the previous work. The retrieval efficiency at this time equals to 44%44\%44% of the value when the storage time is set to be 10μs10μs10μs. Our work is very promising for establishing a high dimensional quantum network.
Quantum light sources are one of key devices for quantum information processing, and they are also the important foundation for applications such as in quantum computing, quantum communication, and quantum simulation. Improving the capacity of quantum information coding by using the quantum light source is a major challenge in the development of quantum information technology. Photons with a helical phase front can carry a discrete, unlimited but quantized amount of orbital angular momentum (OAM). The infinite number of states with different OAMs can greatly increase the capacity of optical communication and information processing in quantum regimes. To date photons carrying OAM have mainly been generated by using bulk crystals, which limits the efficiency and the scalability of the source. With the advancement of quantum photonic technology, many significant quantum photonic devices can now be realized on integrated chips. However, creating high-dimensional OAM quantum states at a micro-nano scale is still a challenge. And the research of harnessing high-dimensional OAM mode by using integrated quantum photonic technologies is still in its infancy. Here, the authors review the recent progress and discuss the integrated quantum light sources with OAM. The authors introduce the research progress of using OAM for both single photons and entangled photons and emphasize the exciting work on pushing boundaries in high-dimensional quantum states. This may pave the way for the research and practical applications of high-dimensional quantum light sources.