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PhotonicsViews

Ultrastable, ultraprecise, portable

Patrizia Krok, Malcolm Simpson

Published Nov 27, 2022• 1 citation
Publisher

Abstract

Abstract In quantum applications such as optical clocks ultrastable laser sources address extremely narrow atomic transitions without introducing noise to the system. This level of stability and precision has historically only been achieved under controlled laboratory conditions. Novel commercial solutions combined with new approaches are now meeting the high demands for field applications of emerging quantum technologies.

DOI
10.1002/phvs.202200049

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Abstract In quantum applications such as optical clocks ultrastable laser sources address extremely narrow atomic transitions without introducing noise to the system. This level of stability and precision has historically only been achieved under controlled laboratory conditions. Novel commercial solutions combined with new approaches are now meeting the high demands for field applications of emerging quantum technologies.
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Optical atomic clocks with fractional uncertainties around and below 10−17 [1] and fractional instabilities at one second interrogation time of below 10−15 [2] have outperformed the best microwave clocks like the cesium atomic clock. In optical atomic clocks a highly stable laser is used to interrogate optical transitions in laser-cooled atoms, ions, or molecules. The increase in accuracy and stability of the optical atomic clocks results from the increased line quality factor Q= ν/Δν given by the five orders of magnitude higher frequency of optical transitions as compared to the transition relevant in the microwave domain. To utilize this potential it is furthermore necessary to realize a suitable narrow linewidth of the interrogated line. The linewidth of any optical transition is given by the different broadening mechanisms of the respective quantum transition relevant for particular interrogation process as well as by the coherence properties of the interrogating laser.
High-precision, portable, and deployable frequency standards are required for modern navigation and communication technologies. Optical frequency standards are attractive for their improved stability over their microwave counterparts; however, increased complexities have anchored them in the laboratory. Sacrificing the sensitivity of the most stable optical clocks has led to the recent development of deployable and portable optical frequency standards, leveraging hot atomic or molecular vapor. The short-term limit for a majority of previous reports on two-photon rubidium standards is either the shot-noise or intermodulation limit hindering the 1 s fractional frequency stability to around 1 × 10 − 13 . The answer for the shot-noise limit is to increase optical power and collected fluorescence, while the intermodulation limit solution requires improvements in laser linewidth, stimulated Brillouin scattering (SBS) lasers are known to reduce frequency noise, suppressing noise of the pump laser. We investigate an optical frequency standard based on the two-photon transition in Rb 87 probed with a narrow photonic integrated circuit SBS laser with a quality factor over 130 million and instantaneous linewidth < 10 Hz . The use of a narrow clock laser coupled with operating at higher optical intensities yielded clock instabilities of 2 × 10 − 14 at 1 s, currently the best reported short-term stability for a two-photon rubidium optical frequency standard.
Clocks based on optical transitions in ions and atoms are quickly moving to the forefront of the frequency standards field mainly because of the high spec-tral resolution, and therefore the potential stability and accuracy, which can be achieved. In this thesis a new optical clock based on neutral atoms trapped in an optical lattice is presented, demonstrating spectroscopy of the clock transition free of any lineshape or accuracy degradation due to atomic motion. The system simu-lates a single trapped ion clock, but allows use of thousands of atoms for improved signal to noise ratio, and clock stability. High accuracy can also be achieved as the lattice can be designed to shift the energy of the two atomic clock states equally, such that the transition frequency is unchanged. Strontium is a natural candidate for such a clock as it offers an extremely narrow optical transition (∼1 mHz) based on atomic states which are very insensitive to external fields. The strontium level structure allows efficient laser cooling to 1 µK with diode laser sources, and a con-venient wavelength of 813 nm for the zero-differential Stark shift optical lattice. The strontium lattice clock system has allowed observation of high signal-to-noise