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Optica

Optical atomic clocks: defining the future of time and frequency metrology

Tara M. Fortier, Andre Nicholas Luiten, Helen S. Margolis

Published Dec 10, 2025• 17 citations
Publisher

Abstract

Optical atomic clocks based on laser-cooled trapped ions and atoms have advanced rapidly over the past decade. With fractional frequency uncertainties now surpassing 10 −18 , they are some of the most precise measurement tools ever built. Yet researchers are still pursuing new avenues of research to explore the fundamental limits to their stability, accuracy, and reproducibility. In this mini-review, we provide a survey of the current state of the art by describing the fundamental principles and techniques that underpin this progress, the architectures used to realize optical clocks, and the supporting laser technologies that are essential to their operation. We also examine the progress that has been made toward a redefinition of the second in the International System of Units and the inclusion of optical clocks into the global time and frequency metrology infrastructure. Finally, we discuss emerging applications of optical clocks and look at the prospects for making their precision more readily accessible to end users.

DOI
10.1364/optica.575770

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•Jan 1, 2011•0 citations
Optical atomic clocks based on laser-cooled trapped ions and atoms have advanced rapidly over the past decade. With fractional frequency uncertainties now surpassing 10 −18 , they are some of the most precise measurement tools ever built. Yet researchers are still pursuing new avenues of research to explore the fundamental limits to their stability, accuracy, and reproducibility. In this mini-review, we provide a survey of the current state of the art by describing the fundamental principles and techniques that underpin this progress, the architectures used to realize optical clocks, and the supporting laser technologies that are essential to their operation. We also examine the progress that has been made toward a redefinition of the second in the International System of Units and the inclusion of optical clocks into the global time and frequency metrology infrastructure. Finally, we discuss emerging applications of optical clocks and look at the prospects for making their precision more readily accessible to end users.
For the past 15 years, tremendous progress within the fields of laser stabilization, optical frequency combs and atom cooling and trapping have allowed the realization of optical atomic clocks with unrivaled performances. These instruments can perform frequency comparisons with fractional uncertainties well below 10-17, finding applications in fundamental physics tests, relativistic geodesy and time and frequency metrology. Even though most optical clocks are currently laboratory setups, several proposals for using these clocks for field measurements or within an optical clock network have been published, and most of time and frequency metrology institutes have started to develop transportable optical clocks. For the purpose of this special issue, we chose to focus on trapped-ion optical clocks. Even though their short-term fractional frequency stability is impaired by a lower signal-to-noise ratio, they offer a high potential for compactness: trapped ions demand low optical powers and simple loading schemes, and can be trapped in small vacuum chambers. We review recent advances on the clock key components, including ion trap and ultra-stable optical cavity, as well as existing projects and experiments which draw the picture of what future transportable, single-ion optical clocks may resemble.
Frequency and its inverse, time, are the most accurately measured quantities. Historically, improvements in the accuracy of clocks have enabled advances in navigation, communication, and science. Since 1967, the definition of the International System (SI) second has been based on the frequency of a microwave transition in cesium, and present day cesium atomic clocks have a fractional uncertainty near 10-16. Recently, a new type of atomic clock based on optical transitions has been developed, with a current fractional uncertainty near 10-18 (approximately one second divided by the age of the universe), and they are rapidly improving. This talk presents a brief summary of the development of optical atomic clocks, with a focus on the Al+ quantum-logic clock developed at NIST. We discuss the current state-of-the-art in optical clock performance, and describe new applications in sensing and fundamental physics. Future directions in optical atomic clock research are also considered.
Transitions between discrete energy levels in well-isolated atomic systems are highly reproducible and therefore make ideal references for highly accurate frequency standards or clocks. In particular, a single laser-cooled ion confined in a radiofrequency ion trap closely approximates the spectroscopic ideal of a particle at rest in a perturbation-free environment. Narrow optical transitions in such systems are therefore very promising for the realization of optical clocks with accuracy around 2 orders of magnitude higher than current microwave primary standards. In this paper the fundamental aspects, current performance and applications of trapped ion optical clocks are reviewed and the potential for future improvements is considered.
Guidelines for developing optical clocks with 10−1810^{-18}10−18 fractional frequency uncertainty
There has been tremendous progress in the performance of optical frequency standards since the first proposals to carry out precision spectroscopy on trapped, single ions in the 1970s. The estimated fractional frequency uncertainty of today's leading optical standards is currently in the 10−18 range, approximately two orders of magnitude better than that of the best caesium primary frequency standards. This exceptional accuracy and stability is resulting in a growing number of research groups developing optical clocks. While good review papers covering the topic already exist, more practical guidelines are needed as a complement. The purpose of this document is therefore to provide technical guidance for researchers starting in the field of optical clocks. The target audience includes national metrology institutes (NMIs) wanting to set up optical clocks (or subsystems thereof) and PhD students and postdocs entering the field. Another potential audience is academic groups with experience in atomic physics and atom or ion trapping, but with less experience of time and frequency metrology and optical clock requirements. These guidelines have arisen from the scope of the EMPIR project "Optical clocks with 1×10−18 uncertainty" (OC18). Therefore, the examples are from European laboratories even though similar work is carried out all over the world. The goal of OC18 was to push the development of optical clocks by improving each of the necessary subsystems: ultrastable lasers, neutral-atom and single-ion traps, and interrogation techniques. This document shares the knowledge acquired by the OC18 project consortium and gives practical guidance on each of these aspects.
In the mid-20th century, atoms were realized to be good candidates for time or frequency standards since transition energies or frequencies between two energy levels of some unperturbed atoms are more stable than those defined by the rotation of the earth or artefact-based clocks such as quartz crystal clocks. This motivated extensive research on realization and improvement of such kind of quantum-based time or frequency standards. The ultra-stable laser, referred to as a local oscillator in a clock, still drifts over time due to environmentally induced length fluctuations of the reference cavity. With the development of ion traps, ultra-narrow linewidth lasers and optical frequency combs, optical clocks based on single trapped ions as a new type of clocks have been realized in many laboratories. Ions can only stay in the trap within a certain region, which is called stability region. There is a variety of potential sources of systematic shifts associated with the clock transition in ion optical clocks.
8half a century ago and have provided the definition of the second since 1967. The international atomic time (TAI) is currently kept by an ensemble of Cs clocks with a fractional uncertainty of Δν/ν0 ≈ 10 –15 , and some Cs fountain clocks 9,10 operate at even smaller uncertainties. Although Cs atomic clocks operate at the microwave transition of ν0 ≈ 9.2 GHz, using optical transition frequencies of several hundred terahertz should improve the fractional uncertainty Δν/ν0 by 4–5 orders of magnitude, as most measurement uncertainties Δν are independent of ν0 (except the Doppler shift Δ νD = (v/c)ν0, where v is the atomic velocity and c is the speed of light). The invention of the laser and the subsequent improvement of laser frequency stabilities 11 has allowed the realization of optical clocks to become a reality 2,3,12