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Input-output theory of cavities in the ultra-strong coupling regime: the case of a time-independent vacuum Rabi frequency

Cristiano Ciuti, Iacopo Carusotto

Published Jan 1, 2006• 0 citations
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Abstract

We present a full quantum theory for the dissipative dynamics of an optical cavity in the ultra-strong light-matter coupling regime, in which the vacuum Rabi frequency is comparable to the electronic transition frequency and the anti-resonant terms of the light-matter coupling play an important role. In particular, our model can be applied to the case of intersubband transitions in doped semiconductor quantum wells embedded in a microcavity. The coupling of the intracavity photonic mode and of the electronic polarization to the external, frequency-dependent, dissipation baths is taken into account by means of quantum Langevin equations in the input-output formalism. Observable spectra (reflection, absorption, transmission and electroluminescence) are calculated analytically in the case of a time-independent vacuum Rabi frequency.

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We present a full quantum theory for the dissipative dynamics of an optical cavity in the ultra-strong light-matter coupling regime, in which the vacuum Rabi frequency is comparable to the electronic transition frequency and the anti-resonant terms of the light-matter coupling play an important role. In particular, our model can be applied to the case of intersubband transitions in doped semiconductor quantum wells embedded in a microcavity. The coupling of the intracavity photonic mode and of the electronic polarization to the external, frequency-dependent, dissipation baths is taken into account by means of quantum Langevin equations in the input-output formalism. Observable spectra (reflection, absorption, transmission and electroluminescence) are calculated analytically in the case of a time-independent vacuum Rabi frequency.
We present a full quantum theory for the dissipative dynamics of an optical cavity in the ultrastrong light-matter coupling regime, in which the vacuum Rabi frequency is a significant fraction of the active electronic transition frequency and the antiresonant terms of the light-matter coupling play an important role. In particular, our model can be applied to the case of intersubband transitions in doped semiconductor quantum wells embedded in a microcavity. The coupling of the intracavity photonic mode and of the electronic polarization to the external, frequency-dependent, dissipation baths is taken into account by means of quantum Langevin equations in the input-output formalism. In the case of a time-independent vacuum Rabi frequency, exact analytical expressions for the operators are obtained, which allows us to characterize the quantum dissipative response of the cavity to an arbitrary initial condition (vacuum, coherent field, thermal excitation). For a vacuum input in both the photonic and electronic polarization modes, the ground state of the cavity system is a two-mode squeezed vacuum state with a finite population in both photonic and electronic modes. These excitations are, however, virtual and cannot escape from the cavity: for a vacuum input, a vacuum output is found, without any trace of the intracavity squeezing. For a coherent photonic input the linear optical response spectra (reflectivity, absorption, transmission) have been studied, and signatures of the ultrastrong coupling have been identified in the asymmetric and peculiar anticrossing of the polaritonic eigenmodes. Finally, we have calculated the electroluminescence spectra in the case of an incoherent electronic input: the emission intensity in the ultrastrong coupling regime results in being significantly enhanced as compared to the case of an isolated quantum well without a surrounding cavity.
In this invited paper of the 28th International Conference of the Physics of Semiconductors (ICPS-28), we discuss the peculiar quantum electrodynamical properties of a semiconductor microcavity system, in which a cavity photon mode is strongly coupled to an intersubband transition of a doped quantum well system. In this kind of semiconductor system, it is possible to achieve an unprecedented ultrastrong coupling regime, in which the vacuum Rabi frequency is comparable to the electronic transition frequency. We discuss the anomalous quantum properties of the quantum ground state (a squeezed vacuum) and of the intersubband cavity polariton excitations. We address the role of dissipation and point out some future perspectives concerning the investigation of quantum vacuum radiation effects induced by an ultrafast time modulation of the quantum vacuum.
We develop a general theory of the quantum vacuum radiation generated by an arbitrary time modulation of the vacuum Rabi frequency of an intersubband transition in a doped quantum well system embedded in a planar microcavity. Both nonradiative and radiative losses are included within an input-output quantum Langevin framework. The intensity and the spectral signatures of the extra-cavity emission are characterized versus the modulation properties. For realistic parameters, the photon pair emission is predicted to largely exceed the blackbody radiation in the mid and far infrared. For strong and resonant modulation a parametric oscillation regime is achievable.
We study the extracavity quantum vacuum radiation generated by a sudden switch on and off of the vacuum Rabi frequency of a single two-level system coupled to a single cavity mode in the strong and ultrastrong coupling regime. Dissipation is described by including the qubit-resonator coupling in the derivation of the master equation. The output stream of photons and their second-order correlation functions are calculated by exploiting a recently developed input-output formulation of resonators valid for arbitrary light-matter couplings. The obtained output photon correlations provide direct information on the quantum correlations among the virtual excitations of the dressed vacuum.
The prototypical system constituted by a two-level atom interacting with a quantized single-mode electromagnetic field is described by the quantum Rabi model (QRM). The QRM is potentially valid at any light-matter interaction regime, ranging from the weak (where the decay rates exceeds the coupling rate) to the deep strong coupling (where the interaction rate exceeds the bare transition frequencies of the subsystems). However, when reaching the ultrastrong coupling regime, several theoretical issues may prevent the correct description of the observable dynamics of such a system: (i) the standard quantum optics master equation fails to correctly describe the interaction of this system with the reservoirs; (ii) the correct output photon rate is no longer proportional to the intracavity photon number; and (iii) they appear to violate gauge invariance. Here, we study the photon flux emission rate of this system under the incoherent excitation of the two-level atom for any light-matter interaction strength and consider different effective temperatures. The dependence of the emission spectra on the coupling strength is the result of the interplay between energy levels, matrix elements of the observables, and the density of states of the reservoirs. Within this approach, we also study the occurrence of light-matter decoupling in the deep strong-coupling regime and show how all of the obtained results are gauge invariant.
We derive the quantum mechanical description of light-matter interactions in optical cavities characterized solely by radiative decay. Unique to radiative decay is the conservation of photon number and coherence, in stark contrast to absorptive losses. This prohibits the description of such cavities by traditional means, e.g., coupling it to a bath of harmonic oscillators into which energy is dissipated. Here, we propose a description of cavities with radiative decay by introducing cavity and noise operators in terms of scattering modes. A multimode input-output formalism to predict measurable far field quantities arises naturally. We apply our general model to the special case of the single excitation regime. We find dynamics reminiscent of the dissipative Jaynes-Cummings model, but with vanishing backaction and a rich temporal and spectral structure of the output modes.