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arXiv:cond-mat/0606554 · Physical Review A

Input-output theory of cavities in the ultrastrong coupling regime: The case of time-independent cavity parameters

Cristiano Ciuti, Iacopo Carusotto

Published Sep 18, 2006• 283 citations
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Abstract

We present a full quantum theory for the dissipative dynamics of an optical cavity in the ultrastrong light-matter coupling regime, in which the vacuum Rabi frequency is a significant fraction of the active electronic transition frequency and the antiresonant terms of the light-matter coupling play an important role. In particular, our model can be applied to the case of intersubband transitions in doped semiconductor quantum wells embedded in a microcavity. The coupling of the intracavity photonic mode and of the electronic polarization to the external, frequency-dependent, dissipation baths is taken into account by means of quantum Langevin equations in the input-output formalism. In the case of a time-independent vacuum Rabi frequency, exact analytical expressions for the operators are obtained, which allows us to characterize the quantum dissipative response of the cavity to an arbitrary initial condition (vacuum, coherent field, thermal excitation). For a vacuum input in both the photonic and electronic polarization modes, the ground state of the cavity system is a two-mode squeezed vacuum state with a finite population in both photonic and electronic modes. These excitations are, however, virtual and cannot escape from the cavity: for a vacuum input, a vacuum output is found, without any trace of the intracavity squeezing. For a coherent photonic input the linear optical response spectra (reflectivity, absorption, transmission) have been studied, and signatures of the ultrastrong coupling have been identified in the asymmetric and peculiar anticrossing of the polaritonic eigenmodes. Finally, we have calculated the electroluminescence spectra in the case of an incoherent electronic input: the emission intensity in the ultrastrong coupling regime results in being significantly enhanced as compared to the case of an isolated quantum well without a surrounding cavity.

DOI
10.1103/physreva.74.033811

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We present a full quantum theory for the dissipative dynamics of an optical cavity in the ultrastrong light-matter coupling regime, in which the vacuum Rabi frequency is a significant fraction of the active electronic transition frequency and the antiresonant terms of the light-matter coupling play an important role. In particular, our model can be applied to the case of intersubband transitions in doped semiconductor quantum wells embedded in a microcavity. The coupling of the intracavity photonic mode and of the electronic polarization to the external, frequency-dependent, dissipation baths is taken into account by means of quantum Langevin equations in the input-output formalism. In the case of a time-independent vacuum Rabi frequency, exact analytical expressions for the operators are obtained, which allows us to characterize the quantum dissipative response of the cavity to an arbitrary initial condition (vacuum, coherent field, thermal excitation). For a vacuum input in both the photonic and electronic polarization modes, the ground state of the cavity system is a two-mode squeezed vacuum state with a finite population in both photonic and electronic modes. These excitations are, however, virtual and cannot escape from the cavity: for a vacuum input, a vacuum output is found, without any trace of the intracavity squeezing. For a coherent photonic input the linear optical response spectra (reflectivity, absorption, transmission) have been studied, and signatures of the ultrastrong coupling have been identified in the asymmetric and peculiar anticrossing of the polaritonic eigenmodes. Finally, we have calculated the electroluminescence spectra in the case of an incoherent electronic input: the emission intensity in the ultrastrong coupling regime results in being significantly enhanced as compared to the case of an isolated quantum well without a surrounding cavity.
We present a full quantum theory for the dissipative dynamics of an optical cavity in the ultra-strong light-matter coupling regime, in which the vacuum Rabi frequency is comparable to the electronic transition frequency and the anti-resonant terms of the light-matter coupling play an important role. In particular, our model can be applied to the case of intersubband transitions in doped semiconductor quantum wells embedded in a microcavity. The coupling of the intracavity photonic mode and of the electronic polarization to the external, frequency-dependent, dissipation baths is taken into account by means of quantum Langevin equations in the input-output formalism. Observable spectra (reflection, absorption, transmission and electroluminescence) are calculated analytically in the case of a time-independent vacuum Rabi frequency.
In this invited paper of the 28th International Conference of the Physics of Semiconductors (ICPS-28), we discuss the peculiar quantum electrodynamical properties of a semiconductor microcavity system, in which a cavity photon mode is strongly coupled to an intersubband transition of a doped quantum well system. In this kind of semiconductor system, it is possible to achieve an unprecedented ultrastrong coupling regime, in which the vacuum Rabi frequency is comparable to the electronic transition frequency. We discuss the anomalous quantum properties of the quantum ground state (a squeezed vacuum) and of the intersubband cavity polariton excitations. We address the role of dissipation and point out some future perspectives concerning the investigation of quantum vacuum radiation effects induced by an ultrafast time modulation of the quantum vacuum.
We study the extracavity quantum vacuum radiation generated by a sudden switch on and off of the vacuum Rabi frequency of a single two-level system coupled to a single cavity mode in the strong and ultrastrong coupling regime. Dissipation is described by including the qubit-resonator coupling in the derivation of the master equation. The output stream of photons and their second-order correlation functions are calculated by exploiting a recently developed input-output formulation of resonators valid for arbitrary light-matter couplings. The obtained output photon correlations provide direct information on the quantum correlations among the virtual excitations of the dressed vacuum.
We have investigated theoretically a dissipative polariton system in the ultrastrong light-matter coupling regime without using the rotating-wave approximation on system-reservoir coupling. Photons in a cavity and excitations in matter respectively couple two large ensembles of harmonic oscillators (photonic and excitonic reservoirs). Inheriting the quantum statistics of polaritons in the ultrastrong coupling regime, in the ground state of the whole system, the two reservoirs are not in the vacuum states but they are squeezed and correlated. We presume the reservoirs to be in this nonvacuum state in the master equation and in the input-output formalism with Langevin equations. Both approaches consistently guarantee the decay of the polariton system to its ground state; no photon detection is also obtained when the polariton system is in the ground state.
Cavity quantum-electrodynamics (QED) is a rich area of optical physics, where extreme light–matter coupling can give rise to ultrastrong coupling. The ultrastrong coupling regime presents some fascinating uniquely quantum mechanical effects, such as ground state virtual photons and vacuum squeezing. Focusing on the widely adopted Hopfield model with cavity dissipation, we show how the linear spectrum of an ultrastrong coupled cavity and a dipole can be described either classically or quantum mechanically, but only when the quantum model includes (i) corrections to maintain gauge invariance, and (ii) a specific type of cavity bath coupling, which has so far not been identified. We also show the impact of this bath model on the quantum Rabi model, which has no classical analog in ultrastrong coupling. These results can be used to guide emerging experiments and significantly impact current models and interpretations of ultrastrong coupling between light and matter.
We develop a general theory of the quantum vacuum radiation generated by an arbitrary time modulation of the vacuum Rabi frequency of an intersubband transition in a doped quantum well system embedded in a planar microcavity. Both nonradiative and radiative losses are included within an input-output quantum Langevin framework. The intensity and the spectral signatures of the extra-cavity emission are characterized versus the modulation properties. For realistic parameters, the photon pair emission is predicted to largely exceed the blackbody radiation in the mid and far infrared. For strong and resonant modulation a parametric oscillation regime is achievable.