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Nanomaterials

Quantum Coherence and Total Phase in Semiconductor Microcavities for Multi-Photon Excitation

Abeer S. Altowyan, K. Berrada, S. Abdel‐Khalek, Hichem Eleuch

Published Aug 3, 2022• 8 citations
Publisher

Abstract

We examine how the weak excitation regime of a quantum well confined in a semiconductor microcavity (SM) influences the dynamics of quantum coherence and the total phase. We analyze the impact of the physical parameters on different quantumness measures, and illustrate their numerical results. We show that the amount of the coherence and total phase in the SMs for multi-photon excitation can be improved and controlled by the strength of the field, exciton-photon coupling, cavity dissipation rate, and excitonic spontaneous emission rate. We illustrate how the fidelity varies depending on the physical parameters. These results might have far-reaching ramifications not just in quantum information processing and optics, but also in physics at large.

DOI
10.3390/nano12152671

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We examine how the weak excitation regime of a quantum well confined in a semiconductor microcavity (SM) influences the dynamics of quantum coherence and the total phase. We analyze the impact of the physical parameters on different quantumness measures, and illustrate their numerical results. We show that the amount of the coherence and total phase in the SMs for multi-photon excitation can be improved and controlled by the strength of the field, exciton-photon coupling, cavity dissipation rate, and excitonic spontaneous emission rate. We illustrate how the fidelity varies depending on the physical parameters. These results might have far-reaching ramifications not just in quantum information processing and optics, but also in physics at large.
We study how the interplay of weak excitation regime of quantum well confined in a semiconductor microcavity affects the dynamics of correlations and the statistical properties of photons. We discuss how the system parameters can impact the quantum entropy and Mandel’s parameter, and illustrate our concerns with numerical simulations. We have found that the enhancement of the correlations and the control of the statistical properties of photons in semiconductor microcavities for multi-photon excitation highly benefits from the combination of the strength of the field, excitonic spontaneous emission rate, cavity dissipative rate, and the coupling between the exciton and photons. Our results may have important implications not only for those specially interested in quantum optics and information, but also for the general physics community.
We report on the optical response of a semiconductor microcavity featuring a strong exciton–photon coupling. The weak excitation regime is investigated experimentally by means of time-resolved transmission and four-wave mixing experiments. The influence of electronic disorder on the coherent exciton–photon dynamics is discussed in terms of the solutions of the Maxwell-Bloch equations. The high excitation regime is investigated by using transient sub-picosecond pump–probe experiments. Optical amplification of the probe beam (up to a factor of five), as well as a fundamental change of the optical spectra, have been found close to and above the exciton saturation density. The observed oscillations are corresponding to the Rabi frequency of the excitons in the pump field.
Summary form only given. Optical interactions in semiconductor microcavities embedded with quantum wells enter a nonperturbative regime when the dipole coupling rate between the exciton and the cavity mode exceeds relevant decay rates. In this regime, coherent energy exchange between the exciton and the cavity mode, i.e. normal mode oscillation (NMO), takes place when the cavity mode is excited impulsively by a short laser pulse. Similar coherent oscillations have also been observed in transient four-wave mixing (FWM) responses. In this paper, we present experimental and theoretical studies on the nature of oscillations in these transient FWM responses. We show that, in contrast to earlier beliefs, oscillations in time-integrated transient FWM do not correspond to NMO of the exciton or photon populations. Theoretical studies further reveal that FWM arising from different physical mechanisms including band filling, excitation-induced dephasing, and renormalized electric fields is characterized by highly distinct coherent dynamics. Oscillations in transient FWM reflect interference between these coherent optical processes and can be used as a unique probe for exciton many-body interactions in the nonperturbative regime.
Semiconductor microcavities have great potential for quantum information science, quantum optics, and quantum sensing. Researchers designing devices based on these microcavities could benefit from having accurate figures of merit to guide their design and enhance the entanglement latency and strength of their devices. This article presents a closed formula for computing the exciton-photon concurrence in semiconductor microcavities. The formula is tailored for the ultralow density limit of both excitons and photons, allowing a better understanding of the entanglement properties in this regime. The closed formula allows for accurate and easy quantification of the exciton-photon coupling strength in terms of the parameters of the system like the couplings, frequencies, and linewidths, which has applications in quantum optics and quantum information science. The presented formulas can be used in rational microcavity design for various applications, such as single-photon sources, quantum light sources, and optoelectronic devices. This contributes to the systematic design and control of entanglement properties of quantum devices tailored for specific tasks in quantum information science, quantum optics, and quantum sensing. In summary, this work represents a valuable contribution to both practical applications and fundamental research in the fields of nanostructures, quantum optics, and quantum information science.
We investigate the appearance of spontaneous coherence in the parametric emission from planar semiconductor microcavities in the strong coupling regime. Calculations are performed by means of a quantum Monte Carlo technique based on the Wigner representation of the coupled exciton and cavity-photon fields. The numerical results are interpreted in terms of a nonequilibrium phase transition occurring at the parametric oscillation threshold: below the threshold, the signal emission is incoherent, and both the first and the second-order coherence functions have a finite correlation length which becomes macroscopic as the threshold is approached. Above the threshold, the emission is instead phase coherent over the whole two-dimensional sample and intensity fluctuations are suppressed. Similar calculations for quasi-one-dimensional microcavities show that in this case the phase coherence of the signal emission has a finite extension even above the threshold, while intensity fluctuations are suppressed.
We study the dynamics of a quantum dot embedded in a three-dimensional microcavity in the strong coupling regime in which the quantum dot exciton has an energy close to the frequency of a confined cavity mode. Under the continuous pumping of the system, the confined electron and hole can recombine either by spontaneous emission through a leaky mode or by stimulated emission of a cavity mode that can escape from the cavity. The numerical integration of a master equation including all these effects gives the dynamics of the density matrix. By using the quantum regression theorem, we compute the first- and second-order coherence functions required to calculate the photon statistics and the spectrum of the emitted light. Our main result is the determination of a range of parameters in which a state of cavity modes with Poissonian or sub-Poissonian (nonclassical) statistics can be built up within the microcavity. Depending on the relative values of pumping and rate of stimulated emission, either one or two peaks close to the excitation energy of the dot and/or to the natural frequency of the cavity are observed in the emission spectrum. The physics behind these results is discussed.