Abstract The progress in chiral light–matter interaction in the quantum regime leads to emergence of chiral quantum optics and quantum nonreciprocity. Spin‐momentum locking is at the heart of chiral quantum optics. In this short review, the basic knowledge of optical nonreciprocity and susceptibility‐momentum locking (SML) is introduced as a novel mechanism for conducting chiral quantum optics. Various approaches achieving optical nonreciprocity based on SML are also reviewed. A perspective regarding the challenges in this direction will also be provided.
Abstract The progress in chiral light–matter interaction in the quantum regime leads to emergence of chiral quantum optics and quantum nonreciprocity. Spin‐momentum locking is at the heart of chiral quantum optics. In this short review, the basic knowledge of optical nonreciprocity and susceptibility‐momentum locking (SML) is introduced as a novel mechanism for conducting chiral quantum optics. Various approaches achieving optical nonreciprocity based on SML are also reviewed. A perspective regarding the challenges in this direction will also be provided.
Summary form only given. Controlling the interaction of light and matter is the basis for diverse applications ranging from light technology to quantum information processing. Nowadays, many of these applications are based on nanophotonic structures. It turns out that the confinement of light in such nanostructures imposes an inherent link between its local polarization and its propagation direction, also referred to as spin-momentum locking of light [1]. Remarkably, this leads to chiral, i.e., propagation direction-dependent effects in the emission and absorption of light, and elementary processes of light-matter interaction are fundamentally altered. For example, when coupling plasmonic particles or atoms to evanescent fields, the intrinsic mirror symmetry of the particles' emission can be broken. In our group, we observed this effect in the interaction between single rubidium atoms and the evanescent part of a light field that is confined by continuous total internal reflection in a whispering-gallery-mode microresonator [2]. In the following, this allowed us to realize chiral nanophotonic interfaces in which the emission direction of light into the structure is controlled by the polarization of the excitation light [3] or by the internal quantum state of the emitter [4], respectively. Moreover, we employed this chiral interaction to demonstrate an integrated optical isolator [5] as well as an integrated optical circulator [6] which operate at the single-photon level and which exhibit low loss. The latter are the first two examples of a new class of nonreciprocal nanophotonic devices which exploit the chiral interaction between single quantum emitters and transversally confined photons.
Chiral quantum optics is a growing field of research in which light-matter interactions become asymmetrically dependent on momentum and spin, offering novel control over photonic and electronic degrees of freedom. Recently, the platforms for investigating chiral light-matter interactions have expanded from laser-cooled atoms and quantum dots to various solid-state systems, such as microcavity polaritons and two-dimensional layered materials, integrated into photonic structures such as waveguides, cavities, and ring resonators. In this Perspective, we begin by establishing the foundation for understanding and engineering these chiral light-matter regimes. We review the cutting-edge platforms that have enabled their successful realization in recent years, focusing on solid-state platforms, and discuss the most relevant experimental challenges to fully harness their potential. Finally, we explore the vast opportunities that these chiral light-matter interfaces present, particularly their ability to reveal exotic quantum many-body phenomena, such as chiral many-body superradiance and fractional quantum Hall physics.
Nanophotonic components allow the control of the flow of light in integrated optical environments. Thereby, the light’s strong confinement leads to an inherent link between its local polarization and propagation direction which fundamentally alters the physics of light-matter interaction and gives rise to phenomena such as directional emission and direction-dependent coupling strengths [1]. I will present the underlying principles of this chiral light-matter interaction and its consequences for integrated applications [1]. In particular, I will show how we employ this effect to control the direction of spontaneous emission [2] and to realize low-loss nonreciprocal transmission at the single-photon level through a silica nanofiber [3]. We use two different approaches where either an ensemble of spin-polarized atoms is weakly coupled to a nanofiber or a single atom is strongly coupled to the nanofiber via a whispering-gallery-mode resonator. The resulting optical isolators show a strong imbalance between the transmissions in forward and reverse direction and, at the same time, a forward transmissions exceeding 70%. We extended this system to a 4-port device, where a single atom routes photons nonreciprocally from one fiber port to the next. This realizes a quantum optical circulator [4] which can even be prepared in a superposition of its operational modes. The demonstrated systems exemplify a new class of (quantum) nanophotonic devices that are ideally suited for photonic quantum information processing and quantum simulation. [1] Nature 541, 473, (2017). [2] Science 346, 67 (2014). [3] Phys. Rev. X 5, 041036 (2015). [4] Science 354, 1577 (2016).
Abstract Nonreciprocal optical responses are investigated, induced by the chiral coupling in a cavity magnomechanical system, which contains a ring resonator and an yttrium iron garnet disk. Benefiting from the chiral magnon‐photon coupling, the signal from different directions can exhibit different optical responses for bistability, transmission, group delay, and quantum noise. Notably, optical nonreciprocity with isolation up to 30 dB can be realized based on chiral‐induced the breaking of Lorentzian reciprocity. Moreover, the introduction of magnon modes can achieve directional conversion between fast light and slow light, resulting in that direction‐dependent nonreciprocal fast‐slow light effect can also be achieved utilizing magnetic devices with chirality. At the same time, the nonreciprocal coexistence range of fast light and slow light can also be efficiently broadened by chiral magnon‐photon coupling strength. Furthermore, it can be observed that the quantum noise spectrum of the system is robust to temperature, even at 50 mK. This study not only reveals the important role of chiral coupling in the optical nonreciprocity, but also provides an efficient method for the development of optical nonreciprocal devices.
Chiral quantum optics is a new research area in light-matter interaction that depends on the direction of light propagation and offers a new path for the quantum regulation of light-matter interactions. In this paper, we study a spinning Kerr-type microresonator coupled with Λ-type atom ensembles, which are driven in opposite directions to generate asymmetric photon statistics. We find that a photon blockade can only be generated by driving the spinning resonator on right side without driving the spinning microresonator from the left side, resulting in chirality. The coupling strength between system modes can be precisely controlled by adjusting the detuning amount of the atomic pump field. Because of the splitting of the resonant frequency generated by the Fizeau drag, the destructive quantum interference generated in right side drive prevents the nonresonant transition path of state ∣1,0〉 to state ∣2,0〉. This direction-dependent chiral quantum optics is expected to be applied to chiral optical devices, single-photon sources and nonreciprocal quantum communications.
Chiral light-matter interactions lie at the heart of emerging technologies such as quantum network protocols and quantum logic gates. In the few photon regime, it has been shown that chiral interactions between photons and a waveguide-embedded two-level quantum emitter can break reciprocity and impart a directional π phase shift while the transmission remains intact. In this work, we present a model for multicolor, chiral nonlinear interactions in waveguides using a Green's Tensor formalism. We challenge previously held notions and demonstrate the complex photon dynamics hidden in multicolor light-matter interactions in the few photon regime. By modulating a stronger control beam, we can manipulate a weaker signal beam that contains much less than a single photon per emitter lifetime, on average. We develop equations for the transmission of the signal photons and removing the control photons to uncover the true strength of these nonlinearities, which we show is stronger than what is possible in symmetric geometries. The model predicts tunable unity extinction and up to 30% amplification in the signal, a $\sim100xincreasefromstandardpredictionsinwhichcontrolphotonsarepresent.Wealsopredictatunable0−π$ phase shift via control modulation with significant robustness to emitter imperfections. Our model opens a new regime of directional nonlinear quantum light-matter interactions for study, providing a route to efficient all-optical control of photons.