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arXiv:2411.06495 · PRX Quantum

Chiral Quantum Optics: Recent Developments and Future Directions

D. G. Suárez-Forero, Mahmoud Jalali Mehrabad, Carlos Vega, Alejandro González-Tudela, Mohammad Hafezi

Published Apr 18, 2025• 56 citations
arXivHTMLPDF

Abstract

Chiral quantum optics is a growing field of research in which light-matter interactions become asymmetrically dependent on momentum and spin, offering novel control over photonic and electronic degrees of freedom. Recently, the platforms for investigating chiral light-matter interactions have expanded from laser-cooled atoms and quantum dots to various solid-state systems, such as microcavity polaritons and two-dimensional layered materials, integrated into photonic structures such as waveguides, cavities, and ring resonators. In this Perspective, we begin by establishing the foundation for understanding and engineering these chiral light-matter regimes. We review the cutting-edge platforms that have enabled their successful realization in recent years, focusing on solid-state platforms, and discuss the most relevant experimental challenges to fully harness their potential. Finally, we explore the vast opportunities that these chiral light-matter interfaces present, particularly their ability to reveal exotic quantum many-body phenomena, such as chiral many-body superradiance and fractional quantum Hall physics.

DOI
10.1103/prxquantum.6.020101

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Chiral quantum optics is a growing field of research in which light-matter interactions become asymmetrically dependent on momentum and spin, offering novel control over photonic and electronic degrees of freedom. Recently, the platforms for investigating chiral light-matter interactions have expanded from laser-cooled atoms and quantum dots to various solid-state systems, such as microcavity polaritons and two-dimensional layered materials, integrated into photonic structures such as waveguides, cavities, and ring resonators. In this Perspective, we begin by establishing the foundation for understanding and engineering these chiral light-matter regimes. We review the cutting-edge platforms that have enabled their successful realization in recent years, focusing on solid-state platforms, and discuss the most relevant experimental challenges to fully harness their potential. Finally, we explore the vast opportunities that these chiral light-matter interfaces present, particularly their ability to reveal exotic quantum many-body phenomena, such as chiral many-body superradiance and fractional quantum Hall physics.
High Resolution Image Download MS PowerPoint Slide Spin-dependent, directional light–matter interactions form the basis of chiral quantum networks. In the solid state, quantum emitters commonly possess circularly polarized optical transitions with spin-dependent handedness. We demonstrate numerically that spin-dependent chiral coupling can be realized by embedding such an emitter in a waveguide-coupled nanocavity, which supports two near-degenerate, orthogonally polarized cavity modes. The chiral behavior arises due to direction-dependent interference between the cavity modes upon coupling to two single-mode output waveguides. Notably, an experimentally realistic cavity design simultaneously supports near-unity chiral contrast, efficient (>95%) cavity-waveguide coupling and enhanced light–matter interaction strength (Purcell factor F P > 70). In combination, these parameters enable the development of highly coherent spin–photon interfaces ready for integration into nanophotonic circuits.
Nonlinear interactions between photons are fundamentally weak as the photons do not interact directly with each other, and any interaction is mediated by matter. This has motivated researchers over many decades to search for strongly nonlinear materials (by controlling electronic properties) and optical resonators with strong spatial and temporal confinement of light. An extreme form of nonlinear optics is quantum nonlinear optics, where we can realize nonlinear interaction between single photons. Such quantum nonlinear optics is at the heart of any photonic quantum information system including analog quantum simulation and fault-tolerant quantum computing. While engineering light-matter interactions can effectively create photon-photon interactions, the required photon number to observe any nonlinearity are normally very high, where any quantum-mechanical signature disappears. However, with emerging low-dimensional materials and engineered photonic resonators, the photon number can be reduced to reach the quantum nonlinear optical regime. In this review paper, we discuss different mechanisms exploited in solid-state platforms to attain quantum nonlinear optics. We review emerging materials and optical resonator architectures with different dimensionalities. We also present future research directions and open problems in this field.
Quantum optics is the branch of physics that investigates the interaction of light with matter at the quantum level, where the discrete nature of photons and quantum states of atoms, molecules, and solid-state systems become dominant. Quantum optics systems provide the experimental and theoretical foundation for understanding nonclassical states of light, quantum coherence, entanglement, and measurement at the quantum limit. Over the past few decades, advances in laser technology, nonlinear optics, and precision measurement have transformed quantum optics from a fundamental discipline into a key enabler of quantum technologies, including quantum communication, quantum computing, quantum sensing, and quantum metrology. This review presents a comprehensive overview of the physical principles, system architectures, and experimental platforms of quantum optics. Emphasis is placed on light sources, atom–photon interaction systems, detection techniques, and emerging applications, along with current challenges and future research directions.
Nonlinear interactions between single quantum particles are at the heart of any quantum information system, including analog quantum simulation and fault-tolerant quantum computing. This remains a particularly difficult problem for photonic qubits, as photons do not interact with each other. While engineering light-matter interaction can effectively create photon-photon interaction, the required photon number to observe any nonlinearity is very high, where any quantum mechanical signature disappears. However, with emerging low-dimensional materials, and engineered photonic resonators, the photon number can be potentially reduced to reach the quantum nonlinear optical regime. In this review paper, we discuss different mechanisms exploited in solid-state platforms to attain quantum nonlinear optics. We review emerging materials and optical resonator architecture with different dimensionalities. We also present new research directions and open problems in this field.
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In this paper, exciting progress of quantum optics in solid state is reviewed. The focus is on semiconductor microcavities with self-assembled quantum dots embedded in the active layer. Due to enormous progress in semiconductor nanotechnology, such photonic structures have become a model system for the study of quantum optics on a scalable and integrable technology platform with high potential for future applications in quantum information technology. Quantum optical phenomena have become accessible due to 3-D confinement of light and matter on the length scale of their wavelength in state-of-the-art semiconductor micro- and nanostructures. This confinement leads to a quantization of the associated photonic and electronic energy levels and requires a quantum mechanical description of the system in the framework of cavity quantum electrodynamics (cQED). This approach considers the dipole interaction between two-level quantum emitters and discrete photonic states of a microcavity. Within the well-known Jaynes-Cummings model, the dipole interaction is described in terms of a coherent exchange of energy between the emitter and the resonator mode. This coherent interaction in the so-called strong coupling regime of cQED is reflected in a normal mode splitting, the vacuum Rabi splitting, of the involved modes and represents a central feature of quantum optics in solid state. Another important example of quantum optics in semiconductor nanostructures is the generation of nonclassical light in specific quantum devices. Of particular interest is the realization of Fock states which represent states containing a well-defined number of photons. Single-photon sources, for instance, allow for the generation of single photons on demand, which is highly desirable for quantum communication systems. In this context, this review paper will present recent experimental studies of quantum optics in solid state. This paper is meant for readers who would like to become familiar with this topic and for experts being interested in the progress in this field. It will cover a broad range of studies ranging from examples of fundamental light-matter interaction in the quantum limit to devices capable of emitting single photons and entangled photon pairs on demand.