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CRC Press eBooks

R1.6 The thermodynamic spin magnetization of strongly correlated 2d electrons in a silicon inversion layer

J.H Davies, A.R Long

Published May 1, 2003• 0 citations
Publisher

Abstract

The nature of the ground state of degenerate two dimensional (2D) fermions at zero magnetic field is an outstanding open problem, which has not been deciphered despite decades of research. In the absence of disorder, the ground state is believed to be determined by the interplay between the kinetic energy, E f, and the inter-particle interaction energy, Ec = e2/ica, where a = (nn)~1^ 2 is the typical inter-particle distance, n is the areal particle density, and k is the host dielectric constant. The relative importance of the two energy scales is characterized by rs = a/ao, with ao being the Bohr radius. For electrons in a single band, rs = Ec/ E f while for the (100) surface of silicon rs = Ec/2E p , due to the two-fold valley degeneracy. At very high densities (rs <£ 1) a 2D system approaches the paramagnetic limit of a non-interacting degenerate gas characterized by the Pauli susceptibility, xo • As the density is reduced, the growing ferromagnetic correlations lead to substantial enhancement of the spin susceptibility, The system is predicted to remain paramagnetic up to rs « 20, where numerical calculations [1] find a quantum phase transition to a ferromagnetic liquid phase [2]. At lower density, rs & 37 [3], the Coulomb correlations are predicted to lead to a second phase transition to an anti-ferromagnetic quantum Wigner crystal. The energy balance between the ferro and paramagnetic states is very subtle, therefore the density window where ferromagnetism can take place is small [1].

DOI
10.1201/9781482269055-27

Related papers

Quantum Phase Transitions in Two-Dimensional Electron

Systems Alexander Shashkin, Sergey Kravchenko

Alexander Shashkin Institute of Solid State Physics, Chernogolovka, Moscow District 142432, Russia Sergey Kravchenko Physics Department, Northeastern University, Boston, Massachusetts 02115, U.S.A. Two-dimensional (2D) electron systems are realized when the electrons are free to move in a plane but their motion perpendicular to the plane is quantized in a confining potential well. Quantum phase transitions realized experimentally in such systems so far include metal-insulator transitions in perpendicular magnetic fields, metal-insulator transition in zero magnetic field, and a possible transition to a Wigner crystal. The first transition is governed by the externally controlled electron density or magnetic field, while the other two are governed by the electron density. At low electron densities in 2D systems, the strongly-interacting limit is reached because the kinetic energy is overwhelmed by the energy of electron-electron interactions. The interaction strength is characterized by the ratio between the Coulomb energy and the Fermi energy, r∗s = Eee/EF . Assuming that the effective electron mass is equal to the band mass, the interaction parameter r∗s in the single-valley case reduces to the Wigner-Seitz radius, rs = 1/(πns)1/2aB, and therefore increases as the electron density, ns, decreases (here aB is the Bohr radius in the semiconductor). Possible candidates for the ground state of the system include a Wigner crystal characterized by spatial and spin ordering [1], a ferromagnetic Fermi liquid with spontaneous spin ordering [2], a paramagnetic Fermi liquid [3], etc. In the strongly-interacting limit (rs 1), no analytical theory has been developed to date. According to numerical simulations [4], Wigner crystallization is expected in a very dilute regime, when rs reaches approximately 35. Refined numerical simulations [5] have predicted that prior to the crystallization, in the range of the interaction parameter 25 ≤ rs ≤ 35, the ground state of the system is a strongly correlated ferromagnetic Fermi liquid. At higher electron densities, rs ∼ 1, the electron liquid is expected to be paramagnetic, with the effective mass, m, and Lande´ g factor renormalized by interactions. Apart from the ferromagnetic Fermi liquid, other intermediate phases between the Wigner crystal and the paramagnetic Fermi liquid may also exist.

CRC Press eBooks•Nov 2, 2010•1 citation

Correlation-induced phase transitions in two-dimensional electron systems

A. Isihara, Liderio Citrangulo Ioriatti Junior

The electrons in inversion or accumulation layers of MOSFETS or in semiconductor-semiconductor interfaces show prominent many-body effects. A new theory of the correlation energy is developed for these electrons such that the results are applicable to a wide density range. The ground-state energy is obtained for all densities. It is continuous and convergent, but changes its analytical form at rs = 1.414. Associated with this change is a divergence of the compressibility that occurs at rs = 1.989. Hence, around this rs, the system can be considered to be in a liquidlike state. In the [001] direction of silicon inversion layers, the two valleys, occupied equally by the electrons at high densities, may be populated unevenly due to electron correlations. This unbalance will cause a valley occupancy phase transition at rs = 8.011, in close agreement with a recent experiment. Under a magnetic field, the susceptibility is enhanced nonlinearly when the density of electrons is reduced. This enhancement becomes very strong toward rs = 13.0, beyond which a spin-polarized state is favored.

International Journal of Quantum Chemistry•Jun 19, 2009•35 citations

Observation of spontaneous ferromagnetism in a two-dimensional electron system

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What are the ground states of an interacting, low-density electron system? In the absence of disorder, it has long been expected that as the electron density is lowered, the exchange energy gained by aligning the electron spins should exceed the enhancement in the kinetic (Fermi) energy, leading to a (Bloch) ferromagnetic transition. At even lower densities, another transition to a (Wigner) solid, an ordered array of electrons, should occur. Experimental access to these regimes, however, has been limited because of the absence of a material platform that supports an electron system with very high quality (low disorder) and low density simultaneously. Here we explore the ground states of interacting electrons in an exceptionally clean, two-dimensional electron system confined to a modulation-doped AlAs quantum well. The large electron effective mass in this system allows us to reach very large values of the interaction parameter [Formula: see text], defined as the ratio of the Coulomb to Fermi energies. As we lower the electron density via gate bias, we find a sequence of phases, qualitatively consistent with the above scenario: a paramagnetic phase at large densities, a spontaneous transition to a ferromagnetic state when [Formula: see text] surpasses 35, and then a phase with strongly nonlinear current-voltage characteristics, suggestive of a pinned Wigner solid, when [Formula: see text] exceeds [Formula: see text] However, our sample makes a transition to an insulating state at [Formula: see text], preceding the onset of the spontaneous ferromagnetism, implying that besides interaction, the role of disorder must also be taken into account in understanding the different phases of a realistic dilute electron system.

arXiv:2011.01335•Proceedings of the National Academy of Sciences•Dec 3, 2020•63 citations

Probing spin susceptibility of a correlated two-dimensional electron system by transport and magnetization measurements

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We report temperature and density dependences of the spin susceptibility of strongly interacting electrons in Si inversion layers. We measured (i) the itinerant electron susceptibility ${\ensuremath{\chi}}^{*}$ from the Shubnikov-de Haas oscillations in crossed magnetic fields and (ii) thermodynamic susceptibility ${\ensuremath{\chi}}_{\mathrm{T}}$ sensitive to all the electrons in the layer. Both ${\ensuremath{\chi}}^{*}$ and ${\ensuremath{\chi}}_{\mathrm{T}}$ are strongly enhanced with lowering the electron density in the metallic phase. However, there is no sign of divergency of either quantity at the density of the metal-insulator transition ${n}_{c}$. Moreover, the value of ${\ensuremath{\chi}}_{\mathrm{T}}$, which can be measured across the transition down to very low densities deep in the insulating phase, increases with density at $n<{n}_{c}$, as expected. In the absence of magnetic field, we found the temperature dependence of ${\ensuremath{\chi}}^{*}$ to be consistent with Fermi-liquid-based predictions, and to be much weaker than the power law predicted by non-Fermi-liquid models. We attribute a much stronger temperature dependence of ${\ensuremath{\chi}}_{\mathrm{T}}$ to localized spin droplets. In strong enough in-plane magnetic field, we found the temperature dependence of ${\ensuremath{\chi}}^{*}$ to be stronger than that expected for the Fermi liquid interaction corrections.

arXiv:1810.03560•Physical review. B./Physical review. B•Oct 3, 2018•17 citations

Thermodynamic properties of a 2D itinerant ferromagnet - a sign-problem free quantum Monte Carlo study

Shenglong Xu, Yi Li, Congjun Wu

The microscopic mechanism of itinerant ferromagnetism is a long-standing problem due to the lack of non-perturbative methods to handle strong magnetic fluctuations of itinerant electrons. We have non-pertubatively studied thermodynamic properties and magnetic phase transitions of a two-dimensional multi-orbital Hubbard model exhibiting ferromagnetic ground states. Quantum Monte-Carlo simulations are employed, which are proved in a wide density region free of the sign problem usually suffered by simulations for fermions. Both Hund's coupling and electron itinerancy are essential for establishing the ferromagnetic coherence. No local magnetic moments exist in the system as a priori, nevertheless, the spin channel remains incoherent showing the Curie-Weiss type spin magnetic susceptibility down to very low temperatures at which the charge channel is already coherent exhibiting a weakly temperature-dependent compressibility. For the SU(2) invariant systems, the spin susceptibility further grows exponentially as approaching zero temperature in two dimensions. In the paramagnetic phase close to the Curie temperature, the momentum space Fermi distributions exhibit strong resemblance to those in the fully polarized state. The long-range ferromagnetic ordering appears when the symmetry is reduced to the Ising class, and the Curie temperature is accurately determined. These simulations provide helpful guidance to searching for novel ferromagnetic materials in both strongly correlated $d$-orbital transition metal oxide layers and the $p$-orbital ultra-cold atom optical lattice systems.

Bulletin of the American Physical Society•Nov 3, 2014•0 citations

Critical behavior of the Pauli spin susceptibility in a strongly correlated 2D electron liquid

S. Anissimova, A. A. Shashkin, S. V. Kravchenko +3 more

Thermodynamic measurements reveal that the Pauli spin susceptibility in a strongly correlated low-disordered two-dimensional electron system in silicon becomes enhanced by almost an order of magnitude at low electron densities and has a critical behavior close to the metalinsulator transition point. This provides thermodynamic evidence for the existence of a phase transition.

Bulletin of the American Physical Society•Mar 23, 2005•0 citations
The nature of the ground state of degenerate two dimensional (2D) fermions at zero magnetic field is an outstanding open problem, which has not been deciphered despite decades of research. In the absence of disorder, the ground state is believed to be determined by the interplay between the kinetic energy, E f, and the inter-particle interaction energy, Ec = e2/ica, where a = (nn)~1^ 2 is the typical inter-particle distance, n is the areal particle density, and k is the host dielectric constant. The relative importance of the two energy scales is characterized by rs = a/ao, with ao being the Bohr radius. For electrons in a single band, rs = Ec/ E f while for the (100) surface of silicon rs = Ec/2E p , due to the two-fold valley degeneracy. At very high densities (rs <£ 1) a 2D system approaches the paramagnetic limit of a non-interacting degenerate gas characterized by the Pauli susceptibility, xo • As the density is reduced, the growing ferromagnetic correlations lead to substantial enhancement of the spin susceptibility, The system is predicted to remain paramagnetic up to rs « 20, where numerical calculations [1] find a quantum phase transition to a ferromagnetic liquid phase [2]. At lower density, rs & 37 [3], the Coulomb correlations are predicted to lead to a second phase transition to an anti-ferromagnetic quantum Wigner crystal. The energy balance between the ferro and paramagnetic states is very subtle, therefore the density window where ferromagnetism can take place is small [1].
Alexander Shashkin Institute of Solid State Physics, Chernogolovka, Moscow District 142432, Russia Sergey Kravchenko Physics Department, Northeastern University, Boston, Massachusetts 02115, U.S.A. Two-dimensional (2D) electron systems are realized when the electrons are free to move in a plane but their motion perpendicular to the plane is quantized in a confining potential well. Quantum phase transitions realized experimentally in such systems so far include metal-insulator transitions in perpendicular magnetic fields, metal-insulator transition in zero magnetic field, and a possible transition to a Wigner crystal. The first transition is governed by the externally controlled electron density or magnetic field, while the other two are governed by the electron density. At low electron densities in 2D systems, the strongly-interacting limit is reached because the kinetic energy is overwhelmed by the energy of electron-electron interactions. The interaction strength is characterized by the ratio between the Coulomb energy and the Fermi energy, r∗s = Eee/EF . Assuming that the effective electron mass is equal to the band mass, the interaction parameter r∗s in the single-valley case reduces to the Wigner-Seitz radius, rs = 1/(πns)1/2aB, and therefore increases as the electron density, ns, decreases (here aB is the Bohr radius in the semiconductor). Possible candidates for the ground state of the system include a Wigner crystal characterized by spatial and spin ordering [1], a ferromagnetic Fermi liquid with spontaneous spin ordering [2], a paramagnetic Fermi liquid [3], etc. In the strongly-interacting limit (rs 1), no analytical theory has been developed to date. According to numerical simulations [4], Wigner crystallization is expected in a very dilute regime, when rs reaches approximately 35. Refined numerical simulations [5] have predicted that prior to the crystallization, in the range of the interaction parameter 25 ≤ rs ≤ 35, the ground state of the system is a strongly correlated ferromagnetic Fermi liquid. At higher electron densities, rs ∼ 1, the electron liquid is expected to be paramagnetic, with the effective mass, m, and Lande´ g factor renormalized by interactions. Apart from the ferromagnetic Fermi liquid, other intermediate phases between the Wigner crystal and the paramagnetic Fermi liquid may also exist.
The electrons in inversion or accumulation layers of MOSFETS or in semiconductor-semiconductor interfaces show prominent many-body effects. A new theory of the correlation energy is developed for these electrons such that the results are applicable to a wide density range. The ground-state energy is obtained for all densities. It is continuous and convergent, but changes its analytical form at rs = 1.414. Associated with this change is a divergence of the compressibility that occurs at rs = 1.989. Hence, around this rs, the system can be considered to be in a liquidlike state. In the [001] direction of silicon inversion layers, the two valleys, occupied equally by the electrons at high densities, may be populated unevenly due to electron correlations. This unbalance will cause a valley occupancy phase transition at rs = 8.011, in close agreement with a recent experiment. Under a magnetic field, the susceptibility is enhanced nonlinearly when the density of electrons is reduced. This enhancement becomes very strong toward rs = 13.0, beyond which a spin-polarized state is favored.
What are the ground states of an interacting, low-density electron system? In the absence of disorder, it has long been expected that as the electron density is lowered, the exchange energy gained by aligning the electron spins should exceed the enhancement in the kinetic (Fermi) energy, leading to a (Bloch) ferromagnetic transition. At even lower densities, another transition to a (Wigner) solid, an ordered array of electrons, should occur. Experimental access to these regimes, however, has been limited because of the absence of a material platform that supports an electron system with very high quality (low disorder) and low density simultaneously. Here we explore the ground states of interacting electrons in an exceptionally clean, two-dimensional electron system confined to a modulation-doped AlAs quantum well. The large electron effective mass in this system allows us to reach very large values of the interaction parameter [Formula: see text], defined as the ratio of the Coulomb to Fermi energies. As we lower the electron density via gate bias, we find a sequence of phases, qualitatively consistent with the above scenario: a paramagnetic phase at large densities, a spontaneous transition to a ferromagnetic state when [Formula: see text] surpasses 35, and then a phase with strongly nonlinear current-voltage characteristics, suggestive of a pinned Wigner solid, when [Formula: see text] exceeds [Formula: see text] However, our sample makes a transition to an insulating state at [Formula: see text], preceding the onset of the spontaneous ferromagnetism, implying that besides interaction, the role of disorder must also be taken into account in understanding the different phases of a realistic dilute electron system.
We report temperature and density dependences of the spin susceptibility of strongly interacting electrons in Si inversion layers. We measured (i) the itinerant electron susceptibility ${\ensuremath{\chi}}^{*}$ from the Shubnikov-de Haas oscillations in crossed magnetic fields and (ii) thermodynamic susceptibility ${\ensuremath{\chi}}_{\mathrm{T}}$ sensitive to all the electrons in the layer. Both ${\ensuremath{\chi}}^{*}$ and ${\ensuremath{\chi}}_{\mathrm{T}}$ are strongly enhanced with lowering the electron density in the metallic phase. However, there is no sign of divergency of either quantity at the density of the metal-insulator transition nc{n}_{c}nc​. Moreover, the value of ${\ensuremath{\chi}}_{\mathrm{T}}$, which can be measured across the transition down to very low densities deep in the insulating phase, increases with density at n<ncn<{n}_{c}n<nc​, as expected. In the absence of magnetic field, we found the temperature dependence of ${\ensuremath{\chi}}^{*}$ to be consistent with Fermi-liquid-based predictions, and to be much weaker than the power law predicted by non-Fermi-liquid models. We attribute a much stronger temperature dependence of ${\ensuremath{\chi}}_{\mathrm{T}}$ to localized spin droplets. In strong enough in-plane magnetic field, we found the temperature dependence of ${\ensuremath{\chi}}^{*}$ to be stronger than that expected for the Fermi liquid interaction corrections.
The microscopic mechanism of itinerant ferromagnetism is a long-standing problem due to the lack of non-perturbative methods to handle strong magnetic fluctuations of itinerant electrons. We have non-pertubatively studied thermodynamic properties and magnetic phase transitions of a two-dimensional multi-orbital Hubbard model exhibiting ferromagnetic ground states. Quantum Monte-Carlo simulations are employed, which are proved in a wide density region free of the sign problem usually suffered by simulations for fermions. Both Hund's coupling and electron itinerancy are essential for establishing the ferromagnetic coherence. No local magnetic moments exist in the system as a priori, nevertheless, the spin channel remains incoherent showing the Curie-Weiss type spin magnetic susceptibility down to very low temperatures at which the charge channel is already coherent exhibiting a weakly temperature-dependent compressibility. For the SU(2) invariant systems, the spin susceptibility further grows exponentially as approaching zero temperature in two dimensions. In the paramagnetic phase close to the Curie temperature, the momentum space Fermi distributions exhibit strong resemblance to those in the fully polarized state. The long-range ferromagnetic ordering appears when the symmetry is reduced to the Ising class, and the Curie temperature is accurately determined. These simulations provide helpful guidance to searching for novel ferromagnetic materials in both strongly correlated ddd-orbital transition metal oxide layers and the ppp-orbital ultra-cold atom optical lattice systems.