Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

International Journal of Quantum Chemistry

Correlation-induced phase transitions in two-dimensional electron systems

A. Isihara, Liderio Citrangulo Ioriatti Junior

Published Jun 19, 2009• 35 citations
Publisher

Abstract

The electrons in inversion or accumulation layers of MOSFETS or in semiconductor-semiconductor interfaces show prominent many-body effects. A new theory of the correlation energy is developed for these electrons such that the results are applicable to a wide density range. The ground-state energy is obtained for all densities. It is continuous and convergent, but changes its analytical form at rs = 1.414. Associated with this change is a divergence of the compressibility that occurs at rs = 1.989. Hence, around this rs, the system can be considered to be in a liquidlike state. In the [001] direction of silicon inversion layers, the two valleys, occupied equally by the electrons at high densities, may be populated unevenly due to electron correlations. This unbalance will cause a valley occupancy phase transition at rs = 8.011, in close agreement with a recent experiment. Under a magnetic field, the susceptibility is enhanced nonlinearly when the density of electrons is reduced. This enhancement becomes very strong toward rs = 13.0, beyond which a spin-polarized state is favored.

DOI
10.1002/qua.560220816

Related papers

R1.6 The thermodynamic spin magnetization of strongly correlated 2d electrons in a silicon inversion layer

J.H Davies, A.R Long

The nature of the ground state of degenerate two dimensional (2D) fermions at zero magnetic field is an outstanding open problem, which has not been deciphered despite decades of research. In the absence of disorder, the ground state is believed to be determined by the interplay between the kinetic energy, E f, and the inter-particle interaction energy, Ec = e2/ica, where a = (nn)~1^ 2 is the typical inter-particle distance, n is the areal particle density, and k is the host dielectric constant. The relative importance of the two energy scales is characterized by rs = a/ao, with ao being the Bohr radius. For electrons in a single band, rs = Ec/ E f while for the (100) surface of silicon rs = Ec/2E p , due to the two-fold valley degeneracy. At very high densities (rs <£ 1) a 2D system approaches the paramagnetic limit of a non-interacting degenerate gas characterized by the Pauli susceptibility, xo • As the density is reduced, the growing ferromagnetic correlations lead to substantial enhancement of the spin susceptibility, The system is predicted to remain paramagnetic up to rs « 20, where numerical calculations [1] find a quantum phase transition to a ferromagnetic liquid phase [2]. At lower density, rs & 37 [3], the Coulomb correlations are predicted to lead to a second phase transition to an anti-ferromagnetic quantum Wigner crystal. The energy balance between the ferro and paramagnetic states is very subtle, therefore the density window where ferromagnetism can take place is small [1].

CRC Press eBooks•May 1, 2003•0 citations

Quantum Phase Transitions in Two-Dimensional Electron

Systems Alexander Shashkin, Sergey Kravchenko

Alexander Shashkin Institute of Solid State Physics, Chernogolovka, Moscow District 142432, Russia Sergey Kravchenko Physics Department, Northeastern University, Boston, Massachusetts 02115, U.S.A. Two-dimensional (2D) electron systems are realized when the electrons are free to move in a plane but their motion perpendicular to the plane is quantized in a confining potential well. Quantum phase transitions realized experimentally in such systems so far include metal-insulator transitions in perpendicular magnetic fields, metal-insulator transition in zero magnetic field, and a possible transition to a Wigner crystal. The first transition is governed by the externally controlled electron density or magnetic field, while the other two are governed by the electron density. At low electron densities in 2D systems, the strongly-interacting limit is reached because the kinetic energy is overwhelmed by the energy of electron-electron interactions. The interaction strength is characterized by the ratio between the Coulomb energy and the Fermi energy, r∗s = Eee/EF . Assuming that the effective electron mass is equal to the band mass, the interaction parameter r∗s in the single-valley case reduces to the Wigner-Seitz radius, rs = 1/(πns)1/2aB, and therefore increases as the electron density, ns, decreases (here aB is the Bohr radius in the semiconductor). Possible candidates for the ground state of the system include a Wigner crystal characterized by spatial and spin ordering [1], a ferromagnetic Fermi liquid with spontaneous spin ordering [2], a paramagnetic Fermi liquid [3], etc. In the strongly-interacting limit (rs 1), no analytical theory has been developed to date. According to numerical simulations [4], Wigner crystallization is expected in a very dilute regime, when rs reaches approximately 35. Refined numerical simulations [5] have predicted that prior to the crystallization, in the range of the interaction parameter 25 ≤ rs ≤ 35, the ground state of the system is a strongly correlated ferromagnetic Fermi liquid. At higher electron densities, rs ∼ 1, the electron liquid is expected to be paramagnetic, with the effective mass, m, and Lande´ g factor renormalized by interactions. Apart from the ferromagnetic Fermi liquid, other intermediate phases between the Wigner crystal and the paramagnetic Fermi liquid may also exist.

CRC Press eBooks•Nov 2, 2010•1 citation

Chapter 2 Metal-Insulator Transition in a Strongly Correlated Two-Dimensional Electron System

A. A. Shashkin, S. V. Kravchenko

This chapter focuses on experimental results obtained in low-disordered strongly interacting two-dimensional (2D) electron systems; in particular in (100)-silicon metal-oxide-semiconductor field-effect transistors (MOSFET). It describes the additional confirmation in favor of zero-temperature zero-field metal-insulator transition is provided by magnetic and thermopower measurements. The chapter argues that the metal-insulator transition in silicon samples with very low level of disorder is driven by interactions. In a low-disordered 2D electron system in silicon MOSFETs, the resistivity at a certain "critical" electron density shows virtually no temperature dependence over a wide range of temperatures. In 2000, it was experimentally found that the ratio between the spin and the cyclotron splittings in silicon MOSFETs strongly increases at low electron densities. The strong enhancement of the spin susceptibility has indicated that at low electron densities, the system behaves well beyond the weakly interacting Fermi liquid.

•May 25, 2017•3 citations

Stiff liquid and solid of electrons in two dimensions

V. M. Pudalov

Electrons in two-dimensional (2D) layers at semiconductor interfaces may be driven to a solid phase by reducing their density. Understandmg of this electron liquid-solid transition at mK-temperatures and the origin of the 2D electron solid phase remain challenging. The experimental system under study is subject to strong interactions and disorder. Charge transport in the electron solid phase demonstrates many features anticipated for the pinned crystal, though no direct imaging of a spatial charge- or magnetic-ordering is available by now. Rich information has been recently obtained for dilute electron liquid phase on strong renormalization of the Pauli spin susceptibility, magnetization, and the effective mass. These data provide a set of the Fermi-liquid coupling parameters for densities down to and at the transition. The steep density dependence of the susceptibility is intriguing because it might indicate a developing magnetic transition, though it is more likely reflects a tendency to crystallization.

Journal de Physique IV (Proceedings)•Nov 1, 2002•4 citations

Critical behavior of the Pauli spin susceptibility in a strongly correlated 2D electron liquid

S. Anissimova, A. A. Shashkin, S. V. Kravchenko +3 more

Thermodynamic measurements reveal that the Pauli spin susceptibility in a strongly correlated low-disordered two-dimensional electron system in silicon becomes enhanced by almost an order of magnitude at low electron densities and has a critical behavior close to the metalinsulator transition point. This provides thermodynamic evidence for the existence of a phase transition.

Bulletin of the American Physical Society•Mar 23, 2005•0 citations

Probing spin susceptibility of a correlated two-dimensional electron system by transport and magnetization measurements

V. M. Pudalov, A. Yu. Kuntsevich, M. E. Gershenson +2 more

We report temperature and density dependences of the spin susceptibility of strongly interacting electrons in Si inversion layers. We measured (i) the itinerant electron susceptibility ${\ensuremath{\chi}}^{*}$ from the Shubnikov-de Haas oscillations in crossed magnetic fields and (ii) thermodynamic susceptibility ${\ensuremath{\chi}}_{\mathrm{T}}$ sensitive to all the electrons in the layer. Both ${\ensuremath{\chi}}^{*}$ and ${\ensuremath{\chi}}_{\mathrm{T}}$ are strongly enhanced with lowering the electron density in the metallic phase. However, there is no sign of divergency of either quantity at the density of the metal-insulator transition ${n}_{c}$. Moreover, the value of ${\ensuremath{\chi}}_{\mathrm{T}}$, which can be measured across the transition down to very low densities deep in the insulating phase, increases with density at $n<{n}_{c}$, as expected. In the absence of magnetic field, we found the temperature dependence of ${\ensuremath{\chi}}^{*}$ to be consistent with Fermi-liquid-based predictions, and to be much weaker than the power law predicted by non-Fermi-liquid models. We attribute a much stronger temperature dependence of ${\ensuremath{\chi}}_{\mathrm{T}}$ to localized spin droplets. In strong enough in-plane magnetic field, we found the temperature dependence of ${\ensuremath{\chi}}^{*}$ to be stronger than that expected for the Fermi liquid interaction corrections.

arXiv:1810.03560•Physical review. B./Physical review. B•Oct 3, 2018•17 citations
The electrons in inversion or accumulation layers of MOSFETS or in semiconductor-semiconductor interfaces show prominent many-body effects. A new theory of the correlation energy is developed for these electrons such that the results are applicable to a wide density range. The ground-state energy is obtained for all densities. It is continuous and convergent, but changes its analytical form at rs = 1.414. Associated with this change is a divergence of the compressibility that occurs at rs = 1.989. Hence, around this rs, the system can be considered to be in a liquidlike state. In the [001] direction of silicon inversion layers, the two valleys, occupied equally by the electrons at high densities, may be populated unevenly due to electron correlations. This unbalance will cause a valley occupancy phase transition at rs = 8.011, in close agreement with a recent experiment. Under a magnetic field, the susceptibility is enhanced nonlinearly when the density of electrons is reduced. This enhancement becomes very strong toward rs = 13.0, beyond which a spin-polarized state is favored.
The nature of the ground state of degenerate two dimensional (2D) fermions at zero magnetic field is an outstanding open problem, which has not been deciphered despite decades of research. In the absence of disorder, the ground state is believed to be determined by the interplay between the kinetic energy, E f, and the inter-particle interaction energy, Ec = e2/ica, where a = (nn)~1^ 2 is the typical inter-particle distance, n is the areal particle density, and k is the host dielectric constant. The relative importance of the two energy scales is characterized by rs = a/ao, with ao being the Bohr radius. For electrons in a single band, rs = Ec/ E f while for the (100) surface of silicon rs = Ec/2E p , due to the two-fold valley degeneracy. At very high densities (rs <£ 1) a 2D system approaches the paramagnetic limit of a non-interacting degenerate gas characterized by the Pauli susceptibility, xo • As the density is reduced, the growing ferromagnetic correlations lead to substantial enhancement of the spin susceptibility, The system is predicted to remain paramagnetic up to rs « 20, where numerical calculations [1] find a quantum phase transition to a ferromagnetic liquid phase [2]. At lower density, rs & 37 [3], the Coulomb correlations are predicted to lead to a second phase transition to an anti-ferromagnetic quantum Wigner crystal. The energy balance between the ferro and paramagnetic states is very subtle, therefore the density window where ferromagnetism can take place is small [1].
Alexander Shashkin Institute of Solid State Physics, Chernogolovka, Moscow District 142432, Russia Sergey Kravchenko Physics Department, Northeastern University, Boston, Massachusetts 02115, U.S.A. Two-dimensional (2D) electron systems are realized when the electrons are free to move in a plane but their motion perpendicular to the plane is quantized in a confining potential well. Quantum phase transitions realized experimentally in such systems so far include metal-insulator transitions in perpendicular magnetic fields, metal-insulator transition in zero magnetic field, and a possible transition to a Wigner crystal. The first transition is governed by the externally controlled electron density or magnetic field, while the other two are governed by the electron density. At low electron densities in 2D systems, the strongly-interacting limit is reached because the kinetic energy is overwhelmed by the energy of electron-electron interactions. The interaction strength is characterized by the ratio between the Coulomb energy and the Fermi energy, r∗s = Eee/EF . Assuming that the effective electron mass is equal to the band mass, the interaction parameter r∗s in the single-valley case reduces to the Wigner-Seitz radius, rs = 1/(πns)1/2aB, and therefore increases as the electron density, ns, decreases (here aB is the Bohr radius in the semiconductor). Possible candidates for the ground state of the system include a Wigner crystal characterized by spatial and spin ordering [1], a ferromagnetic Fermi liquid with spontaneous spin ordering [2], a paramagnetic Fermi liquid [3], etc. In the strongly-interacting limit (rs 1), no analytical theory has been developed to date. According to numerical simulations [4], Wigner crystallization is expected in a very dilute regime, when rs reaches approximately 35. Refined numerical simulations [5] have predicted that prior to the crystallization, in the range of the interaction parameter 25 ≤ rs ≤ 35, the ground state of the system is a strongly correlated ferromagnetic Fermi liquid. At higher electron densities, rs ∼ 1, the electron liquid is expected to be paramagnetic, with the effective mass, m, and Lande´ g factor renormalized by interactions. Apart from the ferromagnetic Fermi liquid, other intermediate phases between the Wigner crystal and the paramagnetic Fermi liquid may also exist.
This chapter focuses on experimental results obtained in low-disordered strongly interacting two-dimensional (2D) electron systems; in particular in (100)-silicon metal-oxide-semiconductor field-effect transistors (MOSFET). It describes the additional confirmation in favor of zero-temperature zero-field metal-insulator transition is provided by magnetic and thermopower measurements. The chapter argues that the metal-insulator transition in silicon samples with very low level of disorder is driven by interactions. In a low-disordered 2D electron system in silicon MOSFETs, the resistivity at a certain "critical" electron density shows virtually no temperature dependence over a wide range of temperatures. In 2000, it was experimentally found that the ratio between the spin and the cyclotron splittings in silicon MOSFETs strongly increases at low electron densities. The strong enhancement of the spin susceptibility has indicated that at low electron densities, the system behaves well beyond the weakly interacting Fermi liquid.
Electrons in two-dimensional (2D) layers at semiconductor interfaces may be driven to a solid phase by reducing their density. Understandmg of this electron liquid-solid transition at mK-temperatures and the origin of the 2D electron solid phase remain challenging. The experimental system under study is subject to strong interactions and disorder. Charge transport in the electron solid phase demonstrates many features anticipated for the pinned crystal, though no direct imaging of a spatial charge- or magnetic-ordering is available by now. Rich information has been recently obtained for dilute electron liquid phase on strong renormalization of the Pauli spin susceptibility, magnetization, and the effective mass. These data provide a set of the Fermi-liquid coupling parameters for densities down to and at the transition. The steep density dependence of the susceptibility is intriguing because it might indicate a developing magnetic transition, though it is more likely reflects a tendency to crystallization.
We report temperature and density dependences of the spin susceptibility of strongly interacting electrons in Si inversion layers. We measured (i) the itinerant electron susceptibility ${\ensuremath{\chi}}^{*}$ from the Shubnikov-de Haas oscillations in crossed magnetic fields and (ii) thermodynamic susceptibility ${\ensuremath{\chi}}_{\mathrm{T}}$ sensitive to all the electrons in the layer. Both ${\ensuremath{\chi}}^{*}$ and ${\ensuremath{\chi}}_{\mathrm{T}}$ are strongly enhanced with lowering the electron density in the metallic phase. However, there is no sign of divergency of either quantity at the density of the metal-insulator transition nc{n}_{c}nc​. Moreover, the value of ${\ensuremath{\chi}}_{\mathrm{T}}$, which can be measured across the transition down to very low densities deep in the insulating phase, increases with density at n<ncn<{n}_{c}n<nc​, as expected. In the absence of magnetic field, we found the temperature dependence of ${\ensuremath{\chi}}^{*}$ to be consistent with Fermi-liquid-based predictions, and to be much weaker than the power law predicted by non-Fermi-liquid models. We attribute a much stronger temperature dependence of ${\ensuremath{\chi}}_{\mathrm{T}}$ to localized spin droplets. In strong enough in-plane magnetic field, we found the temperature dependence of ${\ensuremath{\chi}}^{*}$ to be stronger than that expected for the Fermi liquid interaction corrections.