Summary form only given. Understanding and probing phase transitions in non-equilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a non-fluctuating absorbing phase [1], e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here we report the observation of signatures of such a non-equilibrium phase transition in an open driven quantum system. In our experiment rubidium atoms in a quasi one-dimensional cold disordered gas are laser-excited to Rydberg states under so-called facilitation conditions [2]. This conditional excitation process competes with spontaneous decay (see Fig. 1a) and leads to a crossover between a stationary state with no excitations and one with a finite number of Rydberg excitations (see Fig. 1b, where the phase diagram is plotted as a function of the driving strength and detuning from resonance) [3]. We relate the underlying physics to that of an absorbing state phase transition in the presence of a field which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of non-equilibrium phase transitions in open many-body quantum systems.
Summary form only given. Understanding and probing phase transitions in non-equilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a non-fluctuating absorbing phase [1], e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here we report the observation of signatures of such a non-equilibrium phase transition in an open driven quantum system. In our experiment rubidium atoms in a quasi one-dimensional cold disordered gas are laser-excited to Rydberg states under so-called facilitation conditions [2]. This conditional excitation process competes with spontaneous decay (see Fig. 1a) and leads to a crossover between a stationary state with no excitations and one with a finite number of Rydberg excitations (see Fig. 1b, where the phase diagram is plotted as a function of the driving strength and detuning from resonance) [3]. We relate the underlying physics to that of an absorbing state phase transition in the presence of a field which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of non-equilibrium phase transitions in open many-body quantum systems.
Understanding and probing phase transitions in nonequilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a nonfluctuating absorbing phase, e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here, we report the observation of signatures of such a nonequilibrium phase transition in an open driven quantum system. In our experiment, rubidium atoms in a quasi-one-dimensional cold disordered gas are laser excited to Rydberg states under so-called facilitation conditions. This conditional excitation process competes with spontaneous decay and leads to a crossover between a stationary state with no excitations and one with a finite number of excitations. We relate the underlying physics to that of an absorbing-state phase transition in the presence of a field (i.e., off-resonant excitation processes) which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of nonequilibrium phase transitions in open many-body quantum systems.
Abstract Far-from equilibrium dynamics that lead to self-organization are highly relevant to complex dynamical systems not only in physics, but also in life-, earth-, and social sciences. It is challenging however to find systems with sufficiently controllable parameters that allow quantitatively modelling of emergent properties. Here, we study a non-equilibrium phase transition and observe signatures of self-organized criticality in a dilute thermal vapour of atoms optically excited to strongly interacting Rydberg states. Electromagnetically induced transparency (EIT) provides excellent control over the population dynamics and enables high-resolution probing of the driven-dissipative dynamics, which also exhibits phase bistability. Increased sensitivity compared to previous work allows us to reconstruct the complete phase diagram including in the vicinity of the critical point. We observe that interaction-induced energy shifts and enhanced decay only occur in one of the phases above a critical Rydberg population. This limits the application of generic mean-field models, however a modified, threshold-dependent approach is in qualitative agreement with experimental data. Near threshold, we observe self-organized dynamics in the form of population jumps that return the density to a critical value.
This thesis presents several experiments investigating the regimes of behaviour of a proto-typical open quantum many-body system far away from equilibrium. The experimental platform is based on ultracold atoms laser-excited to Rydberg states, which we engineer to emulate a strongly interacting, driven-dissipative quantum spin system. The high degree of control over the relevant microscopic processes and their parameters, as well as the ability to widely tune interaction and driving strengths provides the means to address fundamental questions on how different regimes of dynamical behaviour emerge in complex open quantum systems and how they can be characterised. \n \nIn the first part, we discuss how control over the relevant properties of Rydberg spin systems, like temperature, density, long evolution times, strong interactions, tunable driving, and dissipation can be achieved. We introduce the new experimental apparatus developed during this thesis, which combines both single-photon and two-photon Rydberg excitation schemes with high atom densities and long excitation times using an optical dipole trap. Additionally, we investigate theoretically how long coherence times exceeding motional timescales combined with strong many-body interactions can be achieved in such a system. We identify an optimal parameter regime for two-photon excitation where such conditions can be generated with coherence times and interaction strengths comparable to what is achievable for single-photon excitation. \n \nIn the second part we explore the macroscopic non-equilibrium behaviour of our system and devise suitable observables for characterising different regimes of behaviour. We discover that the slow atom loss inherent to our system provides a convenient observable for the many-body state of the system. Focussing on evolution times where the effect of the atom loss on the evolution is small, we discover that the rate of atom loss exhibits powerlaw scaling with the driving strength over several orders of magnitude. The measured scaling exponents reveal the non-equilibrium phase structure of the many-body system and allow us to distinguish dissipation-dominated, paramagnetic and critical regimes, as well as an instability. In the observed critical regime, collectively enhanced driving dominates over dissipation, leading to scaling associated to the critical point of the non-dissipative equilibrium Rydberg spin system. Based on the known microscopic processes of our system, we perform classical many-body rate equation simulations, which agree well with the observed phase structure as well as the position and associated scaling exponents of the individual regimes. These findings open up new means to study and classify out of equilibrium systems based on slow particle loss and powerlaw scaling. \n \nIn the last part of this thesis we reveal a second type of criticality in our system, which is genuinely non-equilibrium in character and arises from an absorbing state phase transition. The critical state of this phase transition dominates the system evolution at late times where particle loss is no longer negligible. We identify self-organisation as the mechanism driving the system to this critical state, which we observe through powerlaw scaling of the non-equilibrium steady-state. These experiments establish Rydberg atoms as a well controlled platform for implementing and exploring models of absorbing state phase transitions and self-organised criticality with unprecedented access to the underlying microscopic properties of the system.
Understanding the universal properties of nonequilibrium phase transitions of spreading processes is a challenging problem. This applies in particular to irregular and dynamically varying networks. We here investigate an experimentally accessible model system for such processes, namely, the absorbing-state phase transition (ASPT) of Rydberg-excitation spreading, known as Rydberg facilitation, in a laser-driven gas of mobile atoms. It occurs on an irregular graph, set by the random atom positions in the gas, and, depending on temperature, changes its character from static to dynamic. By studying the behavior of the order parameter in the work of Brady . [], we showed numerical evidence for a crossover from directed percolation (DP) universality through various phases of anomalous directed percolation (ADP) to mean-field (MF) behavior when the temperature of the gas is increased. As the behavior of the order parameter is not sufficient to uniquely determine the universality class, we here analyze the distribution of avalanches—characteristic of nonequilibrium critical behavior—to fully characterize the ASPT. Performing extended numerical calculations and experiments on a cold Rb 87 atom gas, we confirm our earlier numerical findings and our phenomenological model that maps the dynamic network to a static one with power-law tails of the distribution of excitation distances. Furthermore, we discuss the influence of dissipation, present in the experiment and a necessary ingredient for the self-organization of the system to the critical point. In particular, we study the potential modification of the universality class by losses as a function of dissipation strength.
The theory of continuous phase transitions predicts the universal collective properties of a physical system near a critical point, which for instance manifest in characteristic power-law behaviours of physical observables. The well-established concept at or near equilibrium, universality, can also characterize the physics of systems out of equilibrium. The most fundamental instance of a genuine non-equilibrium phase transition is the directed percolation (DP) universality class, where a system switches from an absorbing inactive to a fluctuating active phase. Despite being known for several decades it has been challenging to find experimental systems that manifest this transition. Here we show theoretically that signatures of the DP universality class can be observed in an atomic system with long-range interactions. Moreover, we demonstrate that even mesoscopic ensembles—which are currently studied experimentally—are sufficient to observe traces of this non-equilibrium phase transition in one, two and three dimensions.
In this thesis we explore different phenomena occurring in open quantum many-body systems. This is a research field which is becoming increasingly more important due to the experimental progress towards realization of quantum-simulators and quantum computers using a variety of platforms, from ultracold atoms to superconducting qubit arrays. These systems are inherently driven and open, and it is an ongoing effort to develop theoretical tools and approaches to study their non-equilibrium physics. In the first part of this thesis we explore the different non-equilibrium condensate phases of resonantly interacting bosons in the presence of coherent pump and incoherent losses. This study might be of relevance to existing Rydberg-polariton setups. We derive an effective non-equilibrium field-theory of this model and study its resulting phase diagram. We find a rich phase diagram in- cluding a phase where particles form a condensate of tightly bound molecules. By changing the detuning from the scattering resonance it is possible to drive an Ising phase transition from the molecule condensate phase to a more standard atom condensate phase. In the second part of this thesis we explore the many-body localization (MBL) transition in an open-driven system. Typically, coupling to a bath is expected to destroy localization and transform the sharp MBL transition to a crossover. Here we show how one can use the couplings to non- equilibrium baths in order to detect sharp signatures of the transition, including the divergence of the dynamical exponent in the Griffith regime of the ergodic phase. This is done by solving for the steady-state of the Lindblad quantum-master equation using matrix-product operator tech- niques. Our work here suggests a new scalable numerical approach to study the MBL transition. In the third part of this thesis we study the entanglement properties of measurement trajectories in a free-fermion system subject to dephasing noise. These trajectories describe the evolution of an open system when photons exiting the system are continuously monitored. We are inspired by recent works which studied the entanglement dynamics in hybrid quantum circuits consisting of random-unitary gates and projective measurements. There it was found that a phase transition between a phase with volume-law scaling of entanglement and an area-law phase occurs at a critical value of the measurement rate. In our case we find a new regime, where at weak noise rate the system exhibits logarithmic entanglement scaling, similar to that of (1 + 1)d conformal field- theories. For some measurement protocols, we find a transition to an area-law phase at a critical noise strength.