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arXiv:2502.14757 · Physical Review Research

Nonequilibrium universality of Rydberg-excitation spreading on a dynamic network

Simon Ohler, Daniel Brady, Patrick Mischke, Jana Bender, Herwig Ott, Thomas Niederprüm, Winfried Ripken, Johannes Otterbach, Michael Fleischhauer

Published Jul 14, 2025• 2 citations
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Abstract

Understanding the universal properties of nonequilibrium phase transitions of spreading processes is a challenging problem. This applies in particular to irregular and dynamically varying networks. We here investigate an experimentally accessible model system for such processes, namely, the absorbing-state phase transition (ASPT) of Rydberg-excitation spreading, known as Rydberg facilitation, in a laser-driven gas of mobile atoms. It occurs on an irregular graph, set by the random atom positions in the gas, and, depending on temperature, changes its character from static to dynamic. By studying the behavior of the order parameter in the work of Brady . [], we showed numerical evidence for a crossover from directed percolation (DP) universality through various phases of anomalous directed percolation (ADP) to mean-field (MF) behavior when the temperature of the gas is increased. As the behavior of the order parameter is not sufficient to uniquely determine the universality class, we here analyze the distribution of avalanches—characteristic of nonequilibrium critical behavior—to fully characterize the ASPT. Performing extended numerical calculations and experiments on a cold Rb 87 atom gas, we confirm our earlier numerical findings and our phenomenological model that maps the dynamic network to a static one with power-law tails of the distribution of excitation distances. Furthermore, we discuss the influence of dissipation, present in the experiment and a necessary ingredient for the self-organization of the system to the critical point. In particular, we study the potential modification of the universality class by losses as a function of dissipation strength.

DOI
10.1103/8rlg-169g

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Understanding the universal properties of nonequilibrium phase transitions of spreading processes is a challenging problem. This applies in particular to irregular and dynamically varying networks. We here investigate an experimentally accessible model system for such processes, namely, the absorbing-state phase transition (ASPT) of Rydberg-excitation spreading, known as Rydberg facilitation, in a laser-driven gas of mobile atoms. It occurs on an irregular graph, set by the random atom positions in the gas, and, depending on temperature, changes its character from static to dynamic. By studying the behavior of the order parameter in the work of Brady . [], we showed numerical evidence for a crossover from directed percolation (DP) universality through various phases of anomalous directed percolation (ADP) to mean-field (MF) behavior when the temperature of the gas is increased. As the behavior of the order parameter is not sufficient to uniquely determine the universality class, we here analyze the distribution of avalanches—characteristic of nonequilibrium critical behavior—to fully characterize the ASPT. Performing extended numerical calculations and experiments on a cold Rb 87 atom gas, we confirm our earlier numerical findings and our phenomenological model that maps the dynamic network to a static one with power-law tails of the distribution of excitation distances. Furthermore, we discuss the influence of dissipation, present in the experiment and a necessary ingredient for the self-organization of the system to the critical point. In particular, we study the potential modification of the universality class by losses as a function of dissipation strength.
The facilitation of Rydberg excitations in a gas of atoms provides an ideal model system to study epidemic evolution on (dynamic) networks and self-organization of complex systems to the critical point of a nonequilibrium phase transition. Using Monte Carlo simulations and a machine learning algorithm we show that the universality class of this phase transition can be tuned but is robust against decay inherent to the self-organization process. The classes include directed percolation (DP), the most common class in short-range spreading models, and mean-field (MF) behavior, but also different types of anomalous directed percolation (ADP), characterized by rare long-range excitation processes. In a frozen gas, ground state atoms that can facilitate each other form a static network, for which we predict DP universality. With atomic motion the network becomes dynamic by long-range (Lévy-flight type) excitations. This leads to continuously varying critical exponents, varying smoothly between DP and MF values, corresponding to the ADP universality class. These findings also explain the recently observed critical exponent of Rydberg facilitation in an ultracold gas experiment [Helmrich et al., Nature (London) 577, 481 (2020)NATUAS0028-083610.1038/s41586-019-1908-6], which was in between DP and MF values.
We investigate the out-of-equilibrium behavior of a dissipative gas of Rydberg atoms that features a dynamical transition between two stationary states characterized by different excitation densities. We determine the structure and properties of the phase diagram and identify the universality class of the transition, both for the statics and the dynamics. We show that the proper dynamical order parameter is in fact not the excitation density and find evidence that the dynamical transition is in the "model A" universality class; i.e., it features a nontrivial Z2 symmetry and a dynamics with nonconserved order parameter. This sheds light on some relevant and observable aspects of dynamical transitions in Rydberg gases. In particular it permits a quantitative understanding of a recent experiment [C. Carr, Phys. Rev. Lett. 111, 113901 (2013)] which observed bistable behavior as well as power-law scaling of the relaxation time. The latter emerges not due to critical slowing down in the vicinity of a second order transition, but from the nonequilibrium dynamics near a so-called spinodal line.
Understanding and probing phase transitions in nonequilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a nonfluctuating absorbing phase, e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here, we report the observation of signatures of such a nonequilibrium phase transition in an open driven quantum system. In our experiment, rubidium atoms in a quasi-one-dimensional cold disordered gas are laser excited to Rydberg states under so-called facilitation conditions. This conditional excitation process competes with spontaneous decay and leads to a crossover between a stationary state with no excitations and one with a finite number of excitations. We relate the underlying physics to that of an absorbing-state phase transition in the presence of a field (i.e., off-resonant excitation processes) which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of nonequilibrium phase transitions in open many-body quantum systems.
The spread of excitations by Rydberg facilitation bears many similarities to epidemics. Such systems can be modeled with Monte Carlo simulations of classical rate equations to great accuracy as a result of high dephasing. Motivated by experiments, we theoretically analyze the dynamics of a Rydberg many-body system in the facilitation regime in the limits of high and low temperatures. In the high-temperature limit, a homogeneous mean-field behavior is recovered, while characteristic effects of heterogeneity can be seen in a frozen gas. At high temperatures, the system displays an absorbing-state phase transition and, in the presence of an additional loss channel, self-organized criticality. In a frozen or low-temperature gas, excitations are constrained to a network resembling an Erdős-Rényi graph. We show that the absorbing-state phase transition is replaced with an extended Griffiths phase, which we accurately describe by a susceptible-infected-susceptible model on the Erdős-Rényi network taking into account Rydberg blockade. Published by the American Physical Society 2024
The theory of continuous phase transitions predicts the universal collective properties of a physical system near a critical point, which for instance manifest in characteristic power-law behaviours of physical observables. The well-established concept at or near equilibrium, universality, can also characterize the physics of systems out of equilibrium. The most fundamental instance of a genuine non-equilibrium phase transition is the directed percolation (DP) universality class, where a system switches from an absorbing inactive to a fluctuating active phase. Despite being known for several decades it has been challenging to find experimental systems that manifest this transition. Here we show theoretically that signatures of the DP universality class can be observed in an atomic system with long-range interactions. Moreover, we demonstrate that even mesoscopic ensembles—which are currently studied experimentally—are sufficient to observe traces of this non-equilibrium phase transition in one, two and three dimensions.
Summary form only given. Understanding and probing phase transitions in non-equilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a non-fluctuating absorbing phase [1], e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here we report the observation of signatures of such a non-equilibrium phase transition in an open driven quantum system. In our experiment rubidium atoms in a quasi one-dimensional cold disordered gas are laser-excited to Rydberg states under so-called facilitation conditions [2]. This conditional excitation process competes with spontaneous decay (see Fig. 1a) and leads to a crossover between a stationary state with no excitations and one with a finite number of Rydberg excitations (see Fig. 1b, where the phase diagram is plotted as a function of the driving strength and detuning from resonance) [3]. We relate the underlying physics to that of an absorbing state phase transition in the presence of a field which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of non-equilibrium phase transitions in open many-body quantum systems.