Understanding and probing phase transitions in nonequilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a nonfluctuating absorbing phase, e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here, we report the observation of signatures of such a nonequilibrium phase transition in an open driven quantum system. In our experiment, rubidium atoms in a quasi-one-dimensional cold disordered gas are laser excited to Rydberg states under so-called facilitation conditions. This conditional excitation process competes with spontaneous decay and leads to a crossover between a stationary state with no excitations and one with a finite number of excitations. We relate the underlying physics to that of an absorbing-state phase transition in the presence of a field (i.e., off-resonant excitation processes) which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of nonequilibrium phase transitions in open many-body quantum systems.
Understanding and probing phase transitions in nonequilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a nonfluctuating absorbing phase, e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here, we report the observation of signatures of such a nonequilibrium phase transition in an open driven quantum system. In our experiment, rubidium atoms in a quasi-one-dimensional cold disordered gas are laser excited to Rydberg states under so-called facilitation conditions. This conditional excitation process competes with spontaneous decay and leads to a crossover between a stationary state with no excitations and one with a finite number of excitations. We relate the underlying physics to that of an absorbing-state phase transition in the presence of a field (i.e., off-resonant excitation processes) which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of nonequilibrium phase transitions in open many-body quantum systems.
Summary form only given. Understanding and probing phase transitions in non-equilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a non-fluctuating absorbing phase [1], e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here we report the observation of signatures of such a non-equilibrium phase transition in an open driven quantum system. In our experiment rubidium atoms in a quasi one-dimensional cold disordered gas are laser-excited to Rydberg states under so-called facilitation conditions [2]. This conditional excitation process competes with spontaneous decay (see Fig. 1a) and leads to a crossover between a stationary state with no excitations and one with a finite number of Rydberg excitations (see Fig. 1b, where the phase diagram is plotted as a function of the driving strength and detuning from resonance) [3]. We relate the underlying physics to that of an absorbing state phase transition in the presence of a field which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of non-equilibrium phase transitions in open many-body quantum systems.
We explore the nonequilibrium evolution and stationary states of an open many-body system that displays epidemic spreading dynamics in a classical and a quantum regime. Our study is motivated by recent experiments conducted in strongly interacting gases of highly excited Rydberg atoms where the facilitated excitation of Rydberg states competes with radiative decay. These systems approximately implement open quantum versions of models for population dynamics or disease spreading where species can be in a healthy, infected or immune state. We show that in a two-dimensional lattice, depending on the dominance of either classical or quantum effects, the system may display a different kind of nonequilibrium phase transition. We moreover discuss the observability of our findings in laser driven Rydberg gases with particular focus on the role of long-range interactions.
Understanding the universal properties of nonequilibrium phase transitions of spreading processes is a challenging problem. This applies in particular to irregular and dynamically varying networks. We here investigate an experimentally accessible model system for such processes, namely, the absorbing-state phase transition (ASPT) of Rydberg-excitation spreading, known as Rydberg facilitation, in a laser-driven gas of mobile atoms. It occurs on an irregular graph, set by the random atom positions in the gas, and, depending on temperature, changes its character from static to dynamic. By studying the behavior of the order parameter in the work of Brady . [], we showed numerical evidence for a crossover from directed percolation (DP) universality through various phases of anomalous directed percolation (ADP) to mean-field (MF) behavior when the temperature of the gas is increased. As the behavior of the order parameter is not sufficient to uniquely determine the universality class, we here analyze the distribution of avalanches—characteristic of nonequilibrium critical behavior—to fully characterize the ASPT. Performing extended numerical calculations and experiments on a cold Rb 87 atom gas, we confirm our earlier numerical findings and our phenomenological model that maps the dynamic network to a static one with power-law tails of the distribution of excitation distances. Furthermore, we discuss the influence of dissipation, present in the experiment and a necessary ingredient for the self-organization of the system to the critical point. In particular, we study the potential modification of the universality class by losses as a function of dissipation strength.
Stochastic processes with absorbing states feature examples of nonequilibrium universal phenomena. While the classical regime has been thoroughly investigated in the past, relatively little is known about the behavior of these nonequilibrium systems in the presence of quantum fluctuations. Here, we theoretically address such a scenario in an open quantum spin model which, in its classical limit, undergoes a directed percolation phase transition. By mapping the problem to a nonequilibrium field theory, we show that the introduction of quantum fluctuations stemming from coherent, rather than statistical, spin flips alters the nature of the transition such that it becomes first order. In the intermediate regime, where classical and quantum dynamics compete on equal terms, we highlight the presence of a bicritical point with universal features different from the directed percolation class in a low dimension. We finally propose how this physics could be explored within gases of interacting atoms excited to Rydberg states.
Far-from-equilibrium dynamics that lead to self-organization are highly relevant to complex dynamical systems not only in physics but also in life, earth, and social sciences.However, it is challenging to find systems with sufficiently controllable parameters that allow quantitatively modeling of emergent properties.Here, we study a nonequilibrium phase transition and observe signatures of self-organized criticality in a dilute thermal vapor of atoms optically excited to strongly interacting Rydberg states.Electromagnetically induced transparency provides excellent control over the population dynamics and enables highresolution probing of the driven-dissipative dynamics, which also exhibits phase bistability.Increased sensitivity compared to previous work allows us to reconstruct the complete phase diagram, including in the vicinity of the critical point.We observe that interaction-induced energy shifts and enhanced decay only occur in one of the phases above a critical Rydberg population.This case limits the application of generic mean-field models; however, a modified, threshold-dependent approach is in qualitative agreement with experimental data.Near threshold, we observe self-organized dynamics in the form of population jumps that return the density to a critical value.
Phase transitions to absorbing states are among the simplest examples of critical phenomena out of equilibrium. The characteristic feature of these models is the presence of a fluctuationless configuration that the dynamics cannot leave, which has proved a rather stringent requirement in experiments. Recently, a proposal to seek such transitions in highly tunable systems of cold atomic gases offers to probe this physics and, at the same time, to investigate the robustness of these transitions to quantum coherent effects. Here, the authors specifically focus on the interplay between classical and quantum fluctuations in a simple driven open quantum model which, in the classical limit, reproduces a contact process, which is known to undergo a continuous transition in the ``directed percolation'' universality class. The authors derive an effective long-wavelength field theory for the present class of open spin systems and show that, due to quantum fluctuations, the nature of the transition changes from second to first order, passing through a critical point which appears to belong instead to the ``tricritical directed percolation'' class.