Phase Separation due to Quantum Mechanical Correlations

Kenichi Aoki, Tamao Kobayashi

James K. Freericks, Élliott H. Lieb, Daniel Ueltschi

Can phase separation be induced by strong electron correlations? We present a theorem that affirmatively answers this question in the Falicov-Kimball model away from half filling, for any dimension. In the ground state the itinerant electrons are spatially separated from the classical particles.

Gilad Gour

Sze N. Tan, Murray Holland, Daniel F. Walls

Nonlocal effects associated with quantum-mechanical states have been theoretically interesting because they emphasize the differences between classical and quantum mechanics. We describe a system in which a single input photon causes a nonlocal influence on two spatially separated homodyne detectors, as evidenced by a violation of Bell's inequalities. Unlike previous configurations for violating Bell's inequalities, the correlation is not imposed on a pair of particles that spatially separate before being detected. Rather, the correlation arises from the interaction of the local oscillators at each homodyne detector with the spatially extended field of the input photon. The above effect is only one of a class of situations in which nonlocal correlations can be imposed on separated homodyne detectors by quantum mechanical fields. By deriving the conditions for violating Bell's inequality with phase-sensitive detectors, new tests can be developed that relate to squeezed light and other nonclassical fields.

Gregory D. Scholes

The specific advance of this work is to propose a mechanism by which superpositions collapse during measurement of the separated subsystems of entangled quantum states. It is shown how the phase that locks together entangled states plays a special role in the measurement of isolated subsystems. This `contextual' phase is installed randomly into the entangled state, and decides the measurement outcomes for the subsystems by directing the collapse of each superposition to a particular classical outcome when a subsystem is measured. The measuring apparatus thus obtains a classical read-out of the quantum correlations embedded in an entangled state. More broadly, these results solidify the theory of measurement of quantum superpositions.

Sheng Zhang, Puhan Zhang, Gia-Wei Chern

Phase separation plays a central role in the emergence of novel functionalities of correlated electron materials. The structure of the mixed-phase states depends strongly on the nonequilibrium phase-separation dynamics, which has so far yet to be systematically investigated, especially on the theoretical side. With the aid of modern machine learning methods, we demonstrate the first-ever large-scale kinetic Monte Carlo simulations of the phase separation process for the Falicov-Kimball model, which is one of the canonical strongly correlated electron systems. We uncover an unusual phase-separation scenario where domain coarsening occurs simultaneously at two different scales: the growth of checkerboard clusters at smaller length scales and the expansion of super-clusters, which are aggregates of the checkerboard clusters of the same sign, at a larger scale. We show that the emergence of super-clusters is due to a hidden dynamical breaking of the sublattice symmetry. Arrested growth of the checkerboard patterns and of the super-clusters is shown to result from a correlation-induced self-trapping mechanism. Glassy behaviors similar to the one reported in this work could be generic for other correlated electron systems.