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Scientific Reports

Controllable atom-photon entanglement via quantum interference near plasmonic nanostructure

Behzad Sangshekan, Mostafa Sahrai, Seyyed Hossein Asadpour, Jafar Poursamad Bonab

Published Jan 13, 2022• 28 citations
Publisher

Abstract

A five-level atomic system is proposed in vicinity of a two-dimensional (2D) plasmonic nanostructure with application in atom-photon entanglement. The behavior of the atom-photon entanglement is discussed with and without a control laser field. The amount of atom-photon entanglement is controlled by the quantum interference created by the plasmonic nanostructure. Thus, the degree of atom-photon entanglement is affected by the atomic distance from the plasmonic nanostructure. In the presence of a control field, maximum entanglement between the atom and its spontaneous emission field is observed.

DOI
10.1038/s41598-021-04641-6

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A five-level atomic system is proposed in vicinity of a two-dimensional (2D) plasmonic nanostructure with application in atom-photon entanglement. The behavior of the atom-photon entanglement is discussed with and without a control laser field. The amount of atom-photon entanglement is controlled by the quantum interference created by the plasmonic nanostructure. Thus, the degree of atom-photon entanglement is affected by the atomic distance from the plasmonic nanostructure. In the presence of a control field, maximum entanglement between the atom and its spontaneous emission field is observed.
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A nondiffracting propagation of an optical beam through a four-level double-V-type quantum system near a plasmonic nanostructure is investigated. We study the linear absorption and dispersion properties of the quantum system as it interacts with two laser fields. We discuss the effect of the control beam with a Laguerre-Gaussian (LG) profile on the focusing of the probe beam in the presence of a plasmonic nanostructure. An appropriately selected control beam excites one transition of the atomic system and generates a spatially varying refraction index modulation for a weak probe beam that couples to the other transition. We demonstrate that placing a plasmonic nanostructure at a nanometer distance from the atomic system and using a control field with the spatial structure leads to the diffraction-less propagation of the probe beam through the atomic system. Also, it is shown that the optical properties and probe beam focusing can be controlled by adjusting the distance of the plasmonic nanostructure from the atomic system. The proposed all-optical waveguide with high contrast and transmission can be used to implement applications such as image transfer through the medium and image processing.
We show that the quantum interference between two spontaneous emission channels can be greatly enhanced when a three-level V-type atom is placed near plasmonic nanostructures such as metallic slabs, nanospheres, or periodic arrays of metal-coated spheres. The spontaneous emission rate is calculated by a rigorous first-principles electromagnetic Green's tensor technique. The enhancement of quantum interference is attributed to the strong dependence of the spontaneous emission rate on the orientation of an atomic dipole relative to the surface of the nanostructure at the excitation frequencies of surface plasmons.
The ability to harness light-matter interactions at the few-photon level plays a pivotal role in quantum technologies. Single photons-the most elementary states of light-can be generated on demand in atomic and solid state emitters. Two-photon states are also key quantum assets, but achieving them in individual emitters is challenging because their generation rate is much slower than competing one-photon processes. We demonstrate that atomically thin plasmonic nanostructures can harness two-photon spontaneous emission, resulting in giant far field two-photon production, a wealth of resonant modes enabling tailored photonic and plasmonic entangled states, and plasmon-assisted single-photon creation orders of magnitude more efficient than standard one-photon emission. We unravel the two-photon spontaneous emission channels and show that their spectral line shapes emerge from an intricate interplay between Fano and Lorentzian resonances. Enhanced two-photon spontaneous emission in two-dimensional nanostructures paves the way to an alternative efficient source of light-matter entanglement for on-chip quantum information processing and free-space quantum communications.
When an atomic/molecular system controlled by an external field (to imprint information on it, such as preparing a qubit), is brought near a plasmonic nanostructure, the control problem changes. On one hand, the field experienced by the atom is modified due to the plasmon effects of the nanostructure. On the other hand, due to atom-nanostructure interactions the quantum state spontaneous emission is increased. Purification of states is fundamental to the implementation of quantum technologies. My approach for state purification is based on the interplay of control fields and spontaneous emission from a two-level quantum system in presence of a gold nanoparticle (GNP). For a specific location of the system around the GNP, I can find a control field that increases the purity of the system more than without the GNP. Unlike previous efforts of state purification that involve cooling to the ground state, here the excited state population remains significant.
The density matrix equations of motion in near-degenerate three-level V-type closed-loop atomic system are calculated numerically in Floquet frame. The dynamical behavior of atom- photon entanglement between the dressed atom and its spontaneous emission is studied in semi classical approach beyond the two-photon resonance condition in such a system. The quantum entropy of these two subsystems is investigated by using the von Neumann entropy. It is shown that, the degree of entanglement measure (DEM) can be controlled via the intensity and the detuning of coupling optical field and quantum interference induced by spontaneous emission. Moreover in the absence of quantum interference the steady state behavior of DEM can be achieved even in beyond the two- photon resonance condition. Furthermore in the absence of quantum interference for special parameters of Rabi frequency and detuning of driving laser field disentanglement can be occurred. Also the electromagnetically induced transparency condition can be obtained when the system is disentangled.