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Fast extraction of the electron spin-relaxation rate in the SERF magnetometer from a transient response

Yanning Ma, Kaixuan Zhang, Yaoguo Wang, Ke Yang, Yueyang Zhai, Jixi Lu

Published May 2, 2022• 12 citations
Publisher

Abstract

The magnitude of the electron spin-relaxation rate Rrel of the atomic ensemble directly affects the sensitivity of the spin-exchange relaxation-free (SERF) atomic magnetometer (AM). The rapid and in-situ characterization of Rrel is of great importance. In this work, a fast extraction method of Rrel is proposed with a measurement period shorten to 0.5 s, merely detecting the transient response of SERF AM to a transverse DC excitation magnetic field after switching off the pump beam. In contrast to the conventional methods based on the measurement of the magnetic resonance linewidth, this method circumvents the involvement of optical pumping rate, and enables monitoring Rrel under arbitrary polarization, which is expected to improve the authenticity of Rrel measurement in a more convenient way.

DOI
10.1364/oe.459995

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The magnitude of the electron spin-relaxation rate Rrel of the atomic ensemble directly affects the sensitivity of the spin-exchange relaxation-free (SERF) atomic magnetometer (AM). The rapid and in-situ characterization of Rrel is of great importance. In this work, a fast extraction method of Rrel is proposed with a measurement period shorten to 0.5 s, merely detecting the transient response of SERF AM to a transverse DC excitation magnetic field after switching off the pump beam. In contrast to the conventional methods based on the measurement of the magnetic resonance linewidth, this method circumvents the involvement of optical pumping rate, and enables monitoring Rrel under arbitrary polarization, which is expected to improve the authenticity of Rrel measurement in a more convenient way.
Maintaining a near-zero magnetic field condition is a requisite for atomic magnetometer under the spin-exchange relaxation-free (SERF) regime. Therefore, the precise determination of the residual magnetic fields is of great significance. Herein, we proposed an in-situ measurement method of residual magnetic fields in a dual-beam atomic magnetometer based on a transient response of the transverse polarization along the probe beam direction after switching off the pump beam. Proceeding from the Bloch equation, we established a complete evolution expression of the polarization vector under any static residual magnetic field with the pump beam switched off. On this basis, we analyzed the transient response of the transverse polarization by numerical simulation under different situations of residual magnetic fields. Besides, we also considered two possible conditions when the residual magnetic fields are relatively large or small, respectively. Accordingly, we presented an efficient and convenient estimation method of the residual magnetic fields based on certain time characteristics of the transient response. We verified the feasibility of our method by experiment and achieved a triaxial residual magnetic fields measurement within 0.5 s. This method can realize an in situ and real-time measurement of the residual magnetic fields in a fast and convenient way. Furthermore, this method can evaluate the effectiveness of different magnetic field compensation methods without introducing any modulation or extra devices.
The spin-exchange relaxation-free (SERF) atomic magnetometer (AM) has vital importance in advanced research and has been widely applied in different fields. To improve the sensitivity and robustness of SERF magnetometers, understanding the relaxation mechanism is a significant approach. By controlling the amplitude and direction of external magnetic fields, and switching statuses of the pump and probe laser beam, we measured both the transverse and longitudinal relaxation rate in two experimental methods, respectively, and obtained the Larmor precession frequency, the spin-exchange relaxation rate, the spin-destruction relaxation rate, and the relaxation rate due to collisions between atoms and vapor cell walls. All experimental results are verified with the theoretical calculations. The final longitudinal relaxation rate of our magnetometer is 53 Hz. Furthermore, we measured the sensitivity of our SERF magnetometer reaching 5 fT/Hz1/2 from 5 to 70 Hz after differential measurement with the 3-dB bandwidth of 70 Hz. Our work helps to improve the detection capability of SERF magnetometers, providing performance assurance for searching for exotic spin-dependent interactions and applications, including magnetoencephalograms and magnetocardiograms.
The sensitivity and bandwidth (BW) as the primary criteria of spin-exchange relaxation-free (SERF) atomic magnetometer (AM) are closely related to the transverse relaxation rate of atomic ensemble. In this study, we show an effective method for transverse relaxation rate measurement drawing on the golden Section algorithm. With no requirement of offline fitting, the measuring time of this method is only 7 s. This is especially advantageous for reducing measurement errors due to the drifts of spatial magnetic field and light intensity and using multiple measurements to better monitor the performance of magnetometers. Moreover, the reset after measuring is optimized as the sensitive axis magnetic field correction, ensuring the integrity of measurement while improving the accuracy of magnetic compensation. Furthermore, we find that the acquired experimental data using this method can be adopted for the evaluation of magnetic field compensation performance and the monitoring of magnetic anomaly states. This determination method for transverse relaxation rate is anticipated to play a greater important role in multichannel SERF AMs’ arrays.
A novel method to determine the spin polarization and its distribution for a spin-exchange relaxation-free (SERF) atomic magnetometer are proposed in this paper. The Larmor precession frequency is measured using the fast Fourier transform (FFT) analysis result of the transient response of the magnetometer under the excitation of a series of the step-changed magnetic field. The spin polarization is extracted from the slow-down factor of the precession frequency. The variation of the spin polarization with different pump light intensities and the distribution of the spin polarization along the direction of the pump light are analyzed, and the experimental results are well consistent with the theoretical predictions. The expanded uncertainties of the experimental results vary from 2% to 11% with the increase of the spin polarization and the reason for this variation is analyzed. The advantage of this method is that it allows the accurate measurement of the spin polarization in the pump beam direction within the SERF regime operating state, and it is unaffected by the large optical depth of the vapor cell.
In the optical pumping systems based on the pump-probe arrangement, the spin polarization of the atoms is generally monitored utilizing the probe laser beam, in which way an extra perturbation must be introduced and thus affects the normal operation of the sensors. By investigating the absorption rate of the circularly polarized pump laser, here we demonstrate the feasibility of extracting the electron-spin polarization from the transmitted pump laser intensity. We experimentally validate the method in a spin-exchange relaxation free (SERF) magnetometer and the results are in excellent agreement with the theory. The scheme operates in a silent mode and features a real-time observation. We also study the corresponding magnetic field response of the SERF magnetometer and a term arising from the diffusion effects has been added to the original model to explain the discrepancy of the response.
The spin-exchange relaxation of electron spins directly affects the sensitivity of the atomic magnetometers. Rapid determination of the spin-exchange relaxation is essential. In this work, we propose a novel method for measuring the spin-exchange relaxation that allows being operated in the range of zero to earth-scale magnetic field. The longitudinal and transverse relaxation are synchronously extracted from the magnetic resonance linewidth and radio-frequency field amplitude corresponding to the maximum slope of the dispersive resonance curve. The spin-exchange relaxation is further obtained from the difference. The experimental results are consistent with the conventional linewidth fitting method in near-zero magnetic field and with the theoretical expectation in earth-scale magnetic field. This method not only improves authenticity compared to the conventional linewidth fitting method by considering the effect of rf field on relaxation, but also provides a fast and reliable measurement of the spin-exchange relaxation in earth-scale field.