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Nature Physics

In situ control of effective Kerr nonlinearity with Pockels integrated photonics

Chaohan Cui, Liang Zhang, Linran Fan

Published Mar 31, 2022• 39 citations
Publisher
DOI
10.1038/s41567-022-01542-x

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Pockels effect-induced strong effective Kerr nonlinearity in a lithium niobate waveguide

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The utilization of Kerr nonlinearity in lithium niobate has been extensively investigated over the years. Nevertheless, the practical implementation of Kerr nonlinearity in waveguides has been constrained by the material's inherently low third-order nonlinear coefficients. Here, we present a significant advancement by demonstrating Pockels effect-induced strong effective Kerr nonlinearity in a periodically poled thin-film lithium niobate waveguide. Both effective four-wave mixing (FWM) and cascaded effective FWM processes are experimentally observed. The induced FWM process achieves a maximum output power of −8.5 dBm, spanning a wavelength spectrum of over 116.8 nm. Analysis reveals that the induced effective Kerr nonlinearity exhibits a substantial effective nonlinear refractive index n2,eff more than 2.9 × 10−15 m2/W, corresponding to an effective nonlinear refractive index enhancement factor of 1.6 × 104 relative to the intrinsic value. Moreover, a wavelength-converting experiment demonstrates a flat optic-to-optic response over a broadband radio frequency spectrum, confirming that signal integrity is well preserved after on-chip effective FWM conversion. Therefore, the demonstrated efficient and broadband Pockels effect-induced effective Kerr nonlinearity paves the way for novel applications in diverse fields, including spectroscopy, parametric amplification, quantum correlation studies, and wavelength conversion technologies.

Applied Physics Reviews•Mar 1, 2026•1 citation
Kerr nonlinearity in nanophotonic cavities provides a versatile platform to explore fundamental physical sciences and develop novel photonic technologies. This is driven by the precise dispersion control and significant field enhancement with nanoscale structures. Beyond dispersion and pump engineering, the direct control of Kerr nonlinearity can release the ultimate performance and functionality of photonic systems. Here, we report the in situ control of integrated Kerr nonlinearity through its interplay with the cascaded Pockels nonlinear process. Kerr nonlinearity is tuned over 10~dB dynamic range without modifying photonic structures. Fano resonance is observed with nonlinear spectrum, in contrast to standard linear transmission. This confirms the quantum interference between competing optical nonlinear pathways. Besides nonlinearity enhancement, we also demonstrate the novel capability to suppress the material intrinsic nonlinearity. Finally, we use the tunable nonlinearity to control the spectral brightness and coincidence-to-accidental ratio of single-photon generation. This work paves the way towards the complete nanoscale control of optical nonlinear processes at quantum level.
The utilization of Kerr nonlinearity in lithium niobate has been extensively investigated over the years. Nevertheless, the practical implementation of Kerr nonlinearity in waveguides has been constrained by the material's inherently low third-order nonlinear coefficients. Here, we present a significant advancement by demonstrating Pockels effect-induced strong effective Kerr nonlinearity in a periodically poled thin-film lithium niobate waveguide. Both effective four-wave mixing (FWM) and cascaded effective FWM processes are experimentally observed. The induced FWM process achieves a maximum output power of −8.5 dBm, spanning a wavelength spectrum of over 116.8 nm. Analysis reveals that the induced effective Kerr nonlinearity exhibits a substantial effective nonlinear refractive index n2,eff more than 2.9 × 10−15 m2/W, corresponding to an effective nonlinear refractive index enhancement factor of 1.6 × 104 relative to the intrinsic value. Moreover, a wavelength-converting experiment demonstrates a flat optic-to-optic response over a broadband radio frequency spectrum, confirming that signal integrity is well preserved after on-chip effective FWM conversion. Therefore, the demonstrated efficient and broadband Pockels effect-induced effective Kerr nonlinearity paves the way for novel applications in diverse fields, including spectroscopy, parametric amplification, quantum correlation studies, and wavelength conversion technologies.