Diamond based quantum sensing is a fast-emerging field with both scientific and technological importance. The nitrogen-vacancy (NV) center, a crystal defect in diamond, is a unique model system for microwave sensing application due to its excellent photo-stability, long spin coherence time in ambient conditions. In this work, we systematically optimized the measurement parameters for microwave sensing. The system noise is analyzed, and 1/f noise is suppressed by introducing a differential algorithm. The gain of avalanche photodiode and the gating window of the pulsed fluorescence is optimized to further suppress the noise floor. The decoherence of spin is characterized by varying the duration of the laser and microwave. The minimal detectable power on a standard microstrip is characterized with sampling time down to 1 ms, showing flat frequency dependence. The results have important implications toward fast measurement of broadband microwave power, especially in the field of IC testing and radar signal processing under intense electromagnetic interference.
Diamond based quantum sensing is a fast-emerging field with both scientific and technological importance. The nitrogen-vacancy (NV) center, a crystal defect in diamond, is a unique model system for microwave sensing application due to its excellent photo-stability, long spin coherence time in ambient conditions. In this work, we systematically optimized the measurement parameters for microwave sensing. The system noise is analyzed, and 1/f noise is suppressed by introducing a differential algorithm. The gain of avalanche photodiode and the gating window of the pulsed fluorescence is optimized to further suppress the noise floor. The decoherence of spin is characterized by varying the duration of the laser and microwave. The minimal detectable power on a standard microstrip is characterized with sampling time down to 1 ms, showing flat frequency dependence. The results have important implications toward fast measurement of broadband microwave power, especially in the field of IC testing and radar signal processing under intense electromagnetic interference.
Diamond based quantum sensing is a fast-emerging field with both scientific and technological significance. The nitrogen–vacancy (NV) center, a crystal defect in diamond, has become a unique object for microwave sensing applications due to its excellent stability, long spin coherence time, and optical properties at ambient condition. In this work, we use diamond NV center as atomic receiver to demodulate on–off keying (OOK) signal transmitted in broad frequency range (2 GHz–14 GHz in a portable benchtop setup). We proposed a unique algorithm of voltage discrimination and demonstrated audio signal transceiving with fidelity above 99%. This diamond receiver is attached to the end of a tapered fiber, having all optic nature, which will find important applications in data transmission tasks under extreme conditions such as strong electromagnetic interference, high temperatures, and high corrosion.
High-resolution wide-spectrum measurement techniques have important applications in fields such as astronomy, wireless communication, and medical imaging. Nitrogen-vacancy (NV) center in diamond is well known for its high stability, high sensitivity, real-time monitoring, single-point detection, and suitability for long-term measurement, and has an outstanding choice for spectrum analyzers. Currently, spectrum analyzers based on NV centers as detectors can perform real-time spectrum analysis in the range of several tens of gigahertz, but their frequency resolution is limited to a MHz level. In this study, we construct a quantum diamond microwave spectrum imaging system by combining continuous wave-mixing techniques. According to the spin-related properties of the NV center in diamond, we implement optical pumping by 532 nm green laser light illuminating the diamond NV center. A spherical magnet is used to produce a magnetic field gradient along the direction of the diamond crystal. By adjusting the size and direction of the magnetic field gradient, spatial encoding of the resonance frequency of the NV center is achieved. The magnetic field gradient induces the Zeeman effect on the diamond surface at different positions, generating corresponding ODMR signals. Through accurate programming, we coordinate the frequency scanning step size of the microwave source with the camera exposure and image storage time, and synchronize them circularly according to the order of image acquisition. Ultimately, after algorithmic processing, we successfully obtain comprehensive spectrum data in a range from 900 MHz to 6.0 GHz. Within the measurable spectrum range, the system employs continuous wave-mixing, simultaneously applying resonant microwaves and slightly detuning auxiliary microwaves to effectively excite the NV center. This method triggers off microwave interference effects, disrupting the balance between laser-induced polarization and microwave-induced spontaneous relaxation. Specifically, microwave interference causes the phase and amplitude of the fluorescence signal to change, leading to the generation of alternating current fluorescence signals. This further enhances the response of the NV magnetometer to weak microwave signals. The method enables the system to achieve a frequency resolution of 1 Hz in the measurable spectrum range, and it can separately measure the frequency resolution of multiple frequency points with a frequency step size of 1 MHz. The research results indicate that the wide-spectrum measurement based on NV centers can achieve sub-hertz frequency resolution, providing robust technical support for future spectrum analysis and applications.
Precision optical measurements of the electron-spin precession of nitrogen-vacancy (NV) centers in diamond form the basis of numerous applications. The most sensitivity-demanding applications, such as femtotesla magnetometry, require the ability to measure changes in GHz spin transition frequencies at the sub-millihertz level, corresponding to a fractional resolution of better than 10 − 12 . Here we study the impact of microwave (MW) phase noise on the response of an NV sensor. Fluctuations of the phase of the MW waveform cause undesired rotations of the NV spin state. These fluctuations are imprinted in the optical readout signal and, left unmitigated, are indistinguishable from magnetic-field noise. We show that the phase noise of several common commercial MW generators results in an effective pT s 1 / 2 -range noise floor that varies with the MW carrier frequency and the detection frequency of the pulse sequence. The data are described by a frequency-domain model incorporating the MW phase-noise spectrum and the filter-function response of the sensing protocol. For controlled injection of white and random-walk phase noise, the observed NV magnetic noise floor is described by simple analytic expressions that accurately capture the scaling with pulse sequence length and the number of π pulses. We outline several strategies to suppress the impact of MW phase noise and implement a version, based on gradiometry, that realizes a > 10 -fold suppression. Our study highlights an important challenge in the pursuit of sensitive diamond quantum sensors and is applicable to other qubit systems with a large transition frequency. Published by the American Physical Society 2024
This article presents a method to simultaneously determine multiple microwave signals using the hole-burning effect based on nitrogen-vacancy (NV) centers in diamonds. Tracking the anomalous peaks caused by fixed-frequency microwave signals in the optically detected magnetic resonance spectrum, the frequencies under test can be detected with high precision and accuracy in real time. Meanwhile, the applicability of the scheme in detecting microwave signals of different power is evaluated systematically by adjusting the power of measured fixed-frequency microwave signals. In addition, the frequency resolution of the system is characterized by modulating the frequency of one of the microwave signals. The experiment results indicate that the frequency resolution is as small as 5 kHz and the recognition deviation is less than 0.40 kHz. The method will provide a new idea in the field of electromagnetic compatibility testing, radio signal processing, and Internet of Things Engineering.
Nitrogen-vacancy (NV) centers in single-crystal CVD diamond are promising candidates for quantum sensing due to their remarkable optical and spin properties [1]. These defects exhibit stable photoluminescence (PL), long spin coherence times, and high sensitivity to external fields [2]. In this study, we present a room-temperature PL characterization of NV centers excited with a 532 nm laser. The setup was optimized for high signal-to-noise ratio and spectral resolution. Key parameters analyzed include emission intensity, zero-phonon line (ZPL) at ~637 nm, phonon sidebands, and the charge state distribution between NV⁰ and NV⁻. The NV⁻ state, crucial for spin-based sensing, is evaluated to understand its stability under different nitrogen doping conditions [3]. The relative intensities of NV⁰ and NV⁻ provide insights into nitrogen incorporation and vacancy formation. These results contribute to optimizing synthesis conditions for enhanced NV⁻ concentration, supporting the advancement of diamond-based quantum sensing technologies.
Nitrogen-vacancy (NV) color centers in diamond serve as promising atomic spin systems for measurement applications requiring high accuracy and sensitivity. A key challenge in NV-based quantum sensing is minimizing spin readout noise to approach the standard quantum limit (SQL). Based on a six-level model, this work analyze the dependence of NV-based quantum sensing performance, including spin state readout noise and signal-to-noise ratio (SNR), on controllable parameters such as the Purcell factor and excitation laser pulse characteristics. This study demonstrates that a shorter excitation pulse duration results in a higher saturation value of ground-state spin polarization, while the total time required for the polarization process remains constant. Additionally, the spin readout noise does not improve monotonically with decreasing excitation pulse duration; instead, it initially decreases and subsequently increases as the pulse duration varies. The spin readout noise reaches its optimal level when the pulse duration is 3 ns. Furthermore, no positive correlation exists between the signal-to-noise ratio (SNR) and the Purcell factor, and there is also an optimal value for SNR. When the pulse duration ranges from 1 ns to 40 ns, the variation in SNR is relatively insignificant. This research offers a novel perspective for enhancing the performance of quantum sensing based on diamond defects, such as nitrogen-vacancy (NV) centers.