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Optics Letters

Cascaded frequency up-conversion of bright squeezed vacuum: spectral and correlation properties

Andrei Rasputnyi, Denis A. Kopylov, T. V. Murzina, Maria V. Chekhova

Published Jan 3, 2022• 2 citations
Publisher

Abstract

High-gain parametric down-conversion (PDC) is inevitably accompanied by cascaded up-conversion (CUpC) of PDC radiation in a nonlinear crystal even if CUpC is nonphase matched. Here we study experimentally and theoretically the spectral properties of broadband phase-matched and nonphase-matched CUpC radiation in a beta barium borate (BBO) crystal. Our calculations of the normalized second-order correlation function predict the super-bunching of CUpC radiation.

DOI
10.1364/ol.448790

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High-gain parametric down-conversion (PDC) is inevitably accompanied by cascaded up-conversion (CUpC) of PDC radiation in a nonlinear crystal even if CUpC is nonphase matched. Here we study experimentally and theoretically the spectral properties of broadband phase-matched and nonphase-matched CUpC radiation in a beta barium borate (BBO) crystal. Our calculations of the normalized second-order correlation function predict the super-bunching of CUpC radiation.
Quantum cascaded up-conversion (CUpC) of parametric down conversion (PDC) in a finite nonlinear ${\ensuremath{\chi}}^{(2)}$ crystal is studied theoretically within parametric approximation. The exact solution for creation and annihilation operators presented in the form of Bogoliubov transformation is valid for the high-gain regime and explicitly includes the nonzero wave-vector mismatch both for PDC and CUpC. Characteristic equation is used to analyze parametric amplification and oscillating regimes for degenerate, three- and four-mode cases. We show that the parametric amplification exists under the fulfillment of the cascaded phase-matching conditions while both the PDC and CUpC processes are separately non-phase-matched. The influence of CUpC on quadrature squeezing of degenerate PDC is estimated.
High-gain parametric down-conversion (PDC) is a source of bright squeezed vacuum, which is a macroscopic nonclassical state of light and a promising candidate for quantum information applications. Here we study its properties, such as the intensity spectral width and the spectral width of pairwise correlations. In agreement with the theory, we observe an increase in the spectral width by 27% compared with the low-gain PDC. Frequency cross- and auto-correlations are registered by measuring the reduction of noise in the difference of PDC intensities at various pairs of wavelengths. The noise reduction plots also demonstrate super-bunching typical for collinear frequency-degenerate PDC.
The effect of the quantum properties of light on nonlinear processes has been well studied theoretically. It has been shown that the efficiency of n-photon nonlinear processes in many cases scales as the normalized n-th order correlation function. For light with high intensity correlation function, the efficiency of the n-th harmonic generation will be considerably higher than for coherent light. The experimental observation of this effect remained difficult until recently, because of the absence of bright sources with strong and fast intensity fluctuations. For the experimental demonstration of statistical effects in optical harmonic generation we use as a pump the radiation of high-gain parametric down conversion. Such light shows quantum properties (e.g. quadrature or two-mode squeezing) and has large number of photons in one mode. The normalized n-th order correlation function for this light is (2n - 1)!!, which makes it more attractive for nonlinear processes than both coherent and thermal light. For the generation of optical harmonics we used broadband parametric down conversion around frequency-degeneracy (1600 nm) produced in 1cm BBO crystal from Ti:Sapphire laser (800 nm, 1.6ps, 5kHz, 3W mean intensity). Due to spectral filtering and post-selection technique we could vary the statistics of light from coherent to super-bunched, which allowed us to demonstrate the efficiency enhancement for second-, third-, and fourth-harmonic generation. The obtained experimental results show a good agreement with the theory.