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Optics Express

Optimized gas pressure of an Rb vapor cell in a single-beam SERF magnetometer

Yaxiang Wang, Ge Jin, Junjian Tang, Weiyong Zhou, Bangcheng Han, BinQuan Zhou, Tao Shi

Published Dec 15, 2021• 42 citations
Publisher

Abstract

We present a theoretical and experimental study of a single-beam spin-exchange relaxation-free magnetometer in 87Rb vapor cells under different nitrogen gas pressures. The spin relaxation rate is a key component to limit the magnetic sensitivity, and the zero-field resonance method was used to measure the spin relaxation rates of different alkali metal cells. Simultaneously, in a single-beam spin-exchange-relaxation-free (SERF) magnetometer, we demonstrated that the fundamental magnetic field sensitivity was also limited by the pumping light intensity. Based on our theoretical analysis and experimental results, we determined the optimal pumping light intensity and optimal gas pressure. We experimentally demonstrated that the magnetic field sensitivity was 8.89 fT / Hz in the single-beam configuration, with an active measurement volume of 3 × 3 × 3~mm3.

DOI
10.1364/oe.447456

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A new magnetometer with Cs vapor in the spin exchange relaxation free(SERF) regime is described.Cs has a higher saturated vapor pressure than other alkali metals;so cesium SERF magnetometer is particularly attractive in applications that require lower power dissipation.Four factors affect atomic transverse relaxations in the SERF magnetometer,including collisions and diffusions among Cs,N2 and He,laser pumping and detecting processes;the buffer gas pressure of He that affects the relaxation is calculated and discussed emphatically in theory at 105 ℃,the result shows that the optimum buffer gas pressure is 350×133.3 Pa.Under the optimum pressure,the polarized spectrum linewidth as the function of the cell temperature is discussed briefly.It is found the least linewidth is only 3.7 Hz corresponding to the electric spin relaxation rate of 278 s-1 at 105 ℃.The result provides a help to increase the sensitivity of the magnetometer with Cs vapor.

Journal of Optoelectronics·laser•Jan 1, 2010•0 citations
We present a theoretical and experimental study of a single-beam spin-exchange relaxation-free magnetometer in 87Rb vapor cells under different nitrogen gas pressures. The spin relaxation rate is a key component to limit the magnetic sensitivity, and the zero-field resonance method was used to measure the spin relaxation rates of different alkali metal cells. Simultaneously, in a single-beam spin-exchange-relaxation-free (SERF) magnetometer, we demonstrated that the fundamental magnetic field sensitivity was also limited by the pumping light intensity. Based on our theoretical analysis and experimental results, we determined the optimal pumping light intensity and optimal gas pressure. We experimentally demonstrated that the magnetic field sensitivity was 8.89 fT / Hz in the single-beam configuration, with an active measurement volume of 3 × 3 × 3~mm3.
Optically pumped magnetometers (OPM) are core quantum payloads for geomagnetic remote sensing. Among them, the spin-exchange relaxation-free (SERF) OPM with aT-level ultimate sensitivity stands as mainstream. While enlarging the alkali-metal vapor cell of the SERF OPM enhances sensitivity, it triggers complex atomic spin relaxation, notably intensified magnetic field gradient relaxation. To address the dilemma of atomic spin relaxation regulation and the engineering requirements of ultra-high-sensitivity SERF magnetometers, this paper constructs an analytical model of the total relaxation rate that comprehensively considers wall-collision relaxation, spin-destruction collision relaxation, and longitudinal/transverse magnetic field gradient relaxation, etc. The analytical relationship between buffer gas pressure and total relaxation rate for a commonly used spherical vapor cell is derived, revealing the intrinsic correlation among cell size, atomic spin relaxation, and optimal pressure. Based on the theoretical model, the filling parameters of the vapor cell are optimized, and experimental measurements are carried out. The theoretical relaxation results are highly consistent with the experimental ones, realizing the precise optimization of buffer gas pressure. The optimization method proposed in this paper provides a theoretical basis and parameter guidance for the engineering preparation of alkali-metal vapor cells for high-sensitivity SERF magnetometers in remote sensing applications.
In the spin-exchange relaxation-free (SERF) magnetometer of a perpendicular pump-probe configuration, the pump and probe beam characteristics significantly affect the performance. In this paper, an efficient evaluation of optical parameters to improve the sensitivity of a miniature magnetometer has been presented. We have determined the pump light’s optimal intensity and wavelength through theoretical analysis and the zero-field resonance experiments. Chirp signals are applied to measure the optical rotations at different probe intensities and frequencies. Through theoretical and experimental analysis of noise source characterization under different beam intensities and wavelengths, we demonstrate that dual-beam magnetometer performance is mainly limited by photon shot noise. Based on the optimum pump and probe beam parameters, we demonstrate magnetic field sensitivity of 6.3 fT/ Hz in an 87Rb vapor cell filled with nitrogen gas, with an active measurement volume of 3 × 3 × 3 mm3.
Abstract The hybrid optical pumping spin exchange relaxation free (SERF) atomic magnetometers can realize ultrahigh sensitivity measurement of magnetic field and inertia. We have studied the 85 Rb polarization of two types of hybrid optical pumping SERF magnetometers based on 39 K- 85 Rb- 4 He and 133 Cs- 85 Rb- 4 He respectively. Then we found that 85 Rb polarization varies with the number density of buffer gas 4 He and quench gas N 2 , pumping rate of pump beam and cell temperature respectively, which will provide an experimental guide for the design of the magnetometer. We obtain a general formula on the fundamental sensitivity of the hybrid optical pumping SERF magnetometer due to shot-noise. The formula describes that the fundamental sensitivity of the magnetometer varies with the number density of buffer gas and quench gas, the pumping rate of pump beam, external magnetic field, cell effective radius, measurement volume, cell temperature and measurement time. We obtain a highest fundamental sensitivity of 1.5073 aT / Hz 1/2 (1 aT = 10 −18 T ) with 39 K- 85 Rb- 4 He magnetometer between above two types of magnetometers when 85 Rb polarization is 0.1116. We estimate the fundamental sensitivity limit of the hybrid optical pumping SERF magnetometer to be superior to 1.8359 × 10 −2 aT / Hz 1/2 , which is higher than the shot-noise-limited sensitivity of 1 aT / Hz 1/2 of K SERF atomic magnetometer.
We describe a Cs atomic magnetometer operating in the spin-exchange-relaxation-free (SERF) regime. With a vapor cell temperature of $103\text{ }\ifmmode^\circ\else\textdegree\fi{}\text{C}$ we achieve intrinsic magnetic resonance widths $\ensuremath{\Delta}B=17\text{ }\ensuremath{\mu}\text{G}$ corresponding to an electron spin-relaxation rate of $300\text{ }{\text{s}}^{\ensuremath{-}1}$ when the spin-exchange rate is ${\ensuremath{\Gamma}}_{\text{SE}}=14\text{ }000\text{ }{\text{s}}^{\ensuremath{-}1}$. We also observe an interesting narrowing effect due to diffusion. Signal-to-noise measurements yield a sensitivity of about 400 pG/Hz400\text{ }\text{pG}/\sqrt{\text{Hz}}400 pG/Hz​. Based on photon shot noise, we project a sensitivity of 40 pG/Hz40\text{ }\text{pG}/\sqrt{\text{Hz}}40 pG/Hz​. A theoretical optimization of the magnetometer indicates sensitivities on the order of 2 pG/Hz2\text{ }\text{pG}/\sqrt{\text{Hz}}2 pG/Hz​ should be achievable in a 1 cm31\text{ }{\text{cm}}^{3}1 cm3 volume. Because Cs has a higher saturated vapor pressure than other alkali metals, SERF magnetometers using Cs atoms are particularly attractive in applications requiring lower temperatures.
Spin-exchange-relaxation-free (SERF) optical atomic magnetometers are facing the challenges of dramatic decrease of sensitivity when the alkali vapor cells become small. This paper focuses on the sensitivity improvement of the chip-scale atomic magnetometer (CSAM) by changing buffer-gas pressures inside the microfabricated vapor cells. The rubidium vapor cells with three different buffer-gas pressures were tested in the SERF magnetometer. The influences of vapor cell temperature and pumping laser power on the device sensitivity are also characterized for further optimization. Results show that the three atomic vapor cells, with N2buffer-gas pressure of 0.20, 0.88, and 2.35 amg, have sensitivities of 900, 500, and 150 fT/Hz1/2, respectively. Results indicated that when the alkali vapor cells continue to be smaller, high buffer-gas pressure would provide an effective way to reduce the wall collision and improve the performance of CSAMs.
A new magnetometer with Cs vapor in the spin exchange relaxation free(SERF) regime is described.Cs has a higher saturated vapor pressure than other alkali metals;so cesium SERF magnetometer is particularly attractive in applications that require lower power dissipation.Four factors affect atomic transverse relaxations in the SERF magnetometer,including collisions and diffusions among Cs,N2 and He,laser pumping and detecting processes;the buffer gas pressure of He that affects the relaxation is calculated and discussed emphatically in theory at 105 ℃,the result shows that the optimum buffer gas pressure is 350×133.3 Pa.Under the optimum pressure,the polarized spectrum linewidth as the function of the cell temperature is discussed briefly.It is found the least linewidth is only 3.7 Hz corresponding to the electric spin relaxation rate of 278 s-1 at 105 ℃.The result provides a help to increase the sensitivity of the magnetometer with Cs vapor.