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Advanced Optical Materials

Programmable Polarization of 2D Anisotropic Rare Earth Material for Images Transmission and Encryption

Ping Chen, Xinliang Feng, Dongyan Li, Lejing Pi, Zexin Li, Xiang Xu, Haoyun Wang, Xing Zhou, Tianyou Zhai

Published Dec 23, 2021• 23 citations
Publisher

Abstract

Abstract Light manipulation has promoted applications in all‐optical processing. 2D anisotropic rare earth (RE) materials are promising for light modulation to realize information transmission and encryption due to the unique optical behaviors of RE ions. Here, image transmission and encryption have been realized by using 2D anisotropic RE material Eu2O3. The polarized photoluminescence (PL) of Eu2O3 has been innovatively applied for information transmission by switching the on/off states. The opposite two modes of polarization‐dependent PL have been applied to grayscale‐resolved image transmission and encryption with high security. This novel approach, polarization manipulation on the PL of 2D anisotropic RE materials, will shed light on the development of information processing, all‐optical switch, and all‐optical computation.

DOI
10.1002/adom.202102512

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Abstract Light manipulation has promoted applications in all‐optical processing. 2D anisotropic rare earth (RE) materials are promising for light modulation to realize information transmission and encryption due to the unique optical behaviors of RE ions. Here, image transmission and encryption have been realized by using 2D anisotropic RE material Eu2O3. The polarized photoluminescence (PL) of Eu2O3 has been innovatively applied for information transmission by switching the on/off states. The opposite two modes of polarization‐dependent PL have been applied to grayscale‐resolved image transmission and encryption with high security. This novel approach, polarization manipulation on the PL of 2D anisotropic RE materials, will shed light on the development of information processing, all‐optical switch, and all‐optical computation.
Abstract All‐optical responsive nanomaterials, which can rapidly switch between two stable states, have been regarded as the next‐generation memories due to their potential to realize binary information storage and implement on‐chip, integrated photonic neuromorphic systems. Rare earth oxides are preeminent candidates owing to their extraordinary luminescent stability and narrow optical transitions. However, due to the lack of simple and effective optical switches, it is difficult to realize all‐optical data storage, encoding, and retrieval by pure rare earth‐doped luminescent nanoparticles. Here, a rapid and high‐contrast of 104 luminescent switching of Y2O3:Eu3+ nanoparticle between the enhancement and quenching states is achieved by employing the strong light confinement and ultrafast thermal response of localized surface plasmon resonance. A self‐encrypted all‐optical memory is presented with optical information writing, encryption, reading, and re‐writing, and a high‐sensitivity synaptic response of emitters to frequency and light intensity flux, which can be harnessed to encrypt information flows and promote convenient and high‐security information encryption. Such a convenient and secure plasmonic thermally assisted self‐encrypting luminescent switch paves the way for constructing high‐performance stimuli‐responsive rare earth oxide crystals on demand and expanding their applications in various data encryption, anti‐counterfeiting, and rewritable colouration devices.
Abstract Optical encryption techniques in over the last 10 years have become more important in the area of optical information processing. Several applications, including online payments, medical or biometric image storage or transmission, private military applications, police identification techniques, online banking platforms, governmental services, identity (ID) cards, etc., are only a few examples. Require special and reliable security in the transmission and storage of images. Since digital picture information may be readily accessed by hackers via transmission over the Internet or other communication channels, the issue of photos with unlawful usage is becoming more and more severe. A more effective and secure means of communicating images may be offered via optical encryption. The encryption mechanism and keys are needed at the receiver side in order to decrypt the original optical data. Picture security becomes a highly important subject in communication science as a result of network growth and rising need for image transmission. There are several security issues with picture data, including forgery detection and illegal access. The most straightforward method of picture protection is to encrypt it as text. The traditional text encryption algorithms are inappropriate for picture encryption because of the high correlation present in image data. Over the last two decades, a number of optical approaches have been proposed for photo encryption, with the specific advantage of processing two-dimensional (2D) image data in parallel conduction mode. Therefore, we are doing an extensive investigation on optical image encryption in this work.
Since quantum information technologies are expected to offer communication security and high computational capacities, research in the field is currently attracting a lot of attention. Among the materials studied so far, rare earth doped inorganic insulators are one of the most promising. With the different available trivalent rare earth ions, the visible and the IR range including the telecom wavelength at 1.5 μm can be covered. Transitions are usually narrow, and at low temperatures, long optical and spin coherence times can often be observed. Investigations using bulk single crystals have already led to many promising results. Recently, spectroscopic studies have been extended to other forms of inorganic materials, such as transparent ceramics, thin films, and nanoparticles for single rare‐earth qubits. Progress in these areas is expected to offer many new possibilities for the design of quantum light‐matter interfaces and scalable quantum memories and processors.
Abstract Optical encryption is a potential scheme for information security that exploits abundant degrees of freedom of light to encode information. However, conventional encryption based on fluorescent materials faces challenges in handling complex secret information. Alternatively, single‐pixel imaging (SPI) provides a computational modality to solve these problems. In this study, a high‐capacity fluorescence encryption scheme, achieved by introducing lanthanide materials and steganography into the encoding and decoding processes of SPI is proposed. Two types of well‐designed lanthanide luminescent materials are utilized and excited to generate fluorescence images (fluo‐images), which are crucial in this scheme. Various practical experiments using fluo‐images as secret keys demonstrate the robustness, effectiveness, and repeatability of this scheme. Furthermore, multi‐image experiments indicate the potential of this method to increase secret information capacity. Thus, the proposed fluorescence encryption scheme does provide an efficient computational encryption strategy based on lanthanide luminescent materials for information security, which can improve the security of traditional optical encryption and simultaneously enhance the flexibility of SPI computational decryption.