We study several problems in Bose-Einstein condensates with internal degrees of freedom, and we find that this kind of condensates, which are usually referred to as spinor condensates, exhibit several phenomena that are qualitatively different from scalar (i.e. spinless) condensates. We analyze the ground state of a condensate with the constraint of maintaining a constant value of the total spin, and we find a number of different structures depending on the value of the total spin and the applied external magnetic field. We also study a certain type of measurement on spinor condensates in an attempt to distinguish between the so-called coherent and singlet states. We find that this kind of measurement cannot distinguish between the two states in question. We then consider a different experiment based on the interference between spinor condensate. It turns out that interference experiments cannot be used to distinguish between coherent and singlet states either. One of the interesting results regarding interference between two spinor condensates is that both the offset and visibility of the interference fringes vary from shot to shot, even if the initial conditions are identical in all the runs of the experiment. We then turn to the problem of condensing a gas of effectively spin 1/2 atoms. We argue that if spin relaxation mechanisms are slow enough, the condensate displays the phenomenon of fragmentation. The main difference of the fragmented state that we study and other fragmented states discussed in the literature is that this one is not caused by interatomic interactions, but rather by the constraint on the total spin of the system. We investigate the consequences of performing the experiment in a toroidal trap, and we find that, under certain conditions, the system spontaneously builds up a macroscopic value of orbital angular momentum. We finally discuss several problems related to the external Josephson effect. We derive simple equations of motion for the case of a two-component condensate that are identical to the extensively analyzed Bloch equations. We also find equilibrium points of the motion that are unstable in the spinless case.
We study several problems in Bose-Einstein condensates with internal degrees of freedom, and we find that this kind of condensates, which are usually referred to as spinor condensates, exhibit several phenomena that are qualitatively different from scalar (i.e. spinless) condensates. We analyze the ground state of a condensate with the constraint of maintaining a constant value of the total spin, and we find a number of different structures depending on the value of the total spin and the applied external magnetic field. We also study a certain type of measurement on spinor condensates in an attempt to distinguish between the so-called coherent and singlet states. We find that this kind of measurement cannot distinguish between the two states in question. We then consider a different experiment based on the interference between spinor condensate. It turns out that interference experiments cannot be used to distinguish between coherent and singlet states either. One of the interesting results regarding interference between two spinor condensates is that both the offset and visibility of the interference fringes vary from shot to shot, even if the initial conditions are identical in all the runs of the experiment. We then turn to the problem of condensing a gas of effectively spin 1/2 atoms. We argue that if spin relaxation mechanisms are slow enough, the condensate displays the phenomenon of fragmentation. The main difference of the fragmented state that we study and other fragmented states discussed in the literature is that this one is not caused by interatomic interactions, but rather by the constraint on the total spin of the system. We investigate the consequences of performing the experiment in a toroidal trap, and we find that, under certain conditions, the system spontaneously builds up a macroscopic value of orbital angular momentum. We finally discuss several problems related to the external Josephson effect. We derive simple equations of motion for the case of a two-component condensate that are identical to the extensively analyzed Bloch equations. We also find equilibrium points of the motion that are unstable in the spinless case.
In this thesis, we present some experiments realized with ultracold gases of sodium atoms, trapped at the intersect between two laser beams. At very low temperature, the discretization of energy and the indistinguishability of particles, lead to a new state of matter, a Bose-Einstein condensate. This remarkable phenomenon was initially introduced to describe an ideal gas, that is to say with no interactions between its constituents. Here, we are interested in the effects of the interactions between the atoms. More precisely, our atoms carry a spin 1, and we focus on the collective spin state, in a regime where the spatial degrees of freedom are frozen. Two important results that we present were obtained by embedding the condensate in a nearly vanishing magnetic field. In that regime, interactions dominate and favor the emergence of strongly correlated states. In a first series of experiment, the magnetic field is suddenly decreased to bring the system out-of-equilibrium. The ensuing relaxation dynamics leads to a stationnary state that can be well described by a Gibbs ensemble. In a second experiment, the field is slowly reduced, in order to follow the ground state of the system. We thereby produce a fragmented condensate, which possesses the remarkable feature of being invariant upon spin rotations. The restoration of this symmetry, always broken by single (i.e. nonfragmented) condensates, is driven by the pairing of atoms in singlet states.
Bose-Einstein condensation (BEC) is a phenomenon in which identical bosons occupy the same quantum state below a certain critical temperature. A hallmark of BEC is the coherence between particles every particle shares the same quantum wavefunction and phase. This coherence has been demonstrated for the external (motional) degrees of freedom of the atomic condensates by interfering two condensates. In this thesis, the coherence is shown to extend to the internal spin degrees of freedom of a spin-1 Bose gas evidenced by the observed coherent and reversible spin-changing collisions. The observed coherent dynamics are analogous to Josephson oscillations in weakly connected superconductors and represent a type of matter-wave four-wave mixing. Control of the coherent evolution of the system using magnetic fields is also demonstrated. The studies on spinor condensates begin by creating spinor condensates directly using all-optical approaches that were first developed in our laboratory. All-optical formation of Bose-Einstein condensates (BEC) in 1D optical lattice and single focus trap geometries are developed and presented. These techniques offer considerable flexibility and speed compared to magnetic trap approaches, and the trapping potential can be essentially spin-independent and are ideally suited for studying spinor condensates. Using condensates with well-defined initial non-equilibrium spin configuration, spin mixing of F = 1 and F = 2 spinor condensates of rubidium-87 atoms confined in an optical trap is observed. The equilibrium spin configuration in the F = 1 manifold confirms that 87Rb is ferromagnetic. The coherent spinor dynamics are demonstrated by initiating spin mixing deterministically with a non-stationary spin population configuration. Finally, the interplay between the coherent spin mixing and spatial dynamics in spin-1 condensates with ferromagnetic interactions is investigated.
We study two aspects of measurement theory in spinor Bose-Einstein condensates of F=1 atoms: the probability of obtaining a certain outcome of the measurement and the evolution of the state of the condensate due to the measurement. We also study the interference patterns arising from the spatial overlap of two spinor condensates. We show that neither a measurement on a small number of escaping atoms nor an interference experiment can distinguish between an antiferromagnetic coherent state condensate, i.e., a condensate in which all the atoms have Sz=0 along an a priori unknown direction, and a spin-singlet condensate, i.e., a condensate with Stotal=0. We also show that a singlet-state condensate evolves into a coherent state as a result of the measurement.
This thesis contains theoretical studies of weakly interacting, trapped Bose-Einstein condensed gases. The main emphasis is on the rotational properties of these systems. A typical Bose-Einstein condensate reacts to external rotation by forming singly quantized vortices. By the word ”typical” we refer to a condensate with repulsive interparticle interactions and with a frozen spin degree of freedom. However, there are some atomic species for which the low-energy interactions are attractive. Moreover, the tuning of different condensate properties is relatively easy. For example, there are ways to experimentally change the effective interaction from repulsive to attractive. For an attractively interacting condensate the vortex is not the only possible rotational state but the sample may also experience rotation through its center of mass. In the first part of the thesis, we analyze some properties of a rotating attractive Bose gas at the zero temperature limit. First, we note that in order to maintain energetical stability, the gas has to be rotated in an external trap which is steeper than a harmonic trap. We study the system in an anharmonic quadratic + quartic potential. The rotating ground state phase-space is determined with analytical and numerical methods. If the interactions are strong enough, the rotating ground state appears to be a state with the rotating center of mass. On the other hand, at the limit of weak interactions the system experiences rotation by forming a multiply quantized vortex. We also determine the spectrum of elementary excitations for these quantum many-particle states. We find that the broken symmetry of the center of mass rotating state induces an additional zero-energy (Goldstone) mode and that the small oscillations of the ground state exhibit the decoupling between the center of mass and relative motions. If the spin of the atoms is allowed to change freely, a rich variety of topological excitations in condensates can be studied. External rotation is one of the tools for examining the excitations in spinor condensates. In a spinless scalar condensate the appearance of a quantized vortex is manifested by the vortex line in which the condensate density vanishes. In the plane perpendicular to the vortex line, one speaks of the vortex core for the density minimum. We study the properties of slowly rotated F = 1 spinor condensates and show that for ferromagnetic interactions the ground state is a coreless vortex. While the individual spin components may carry ordinary vortices the overall density of the system is coreless. We also study a method to create a point-like monopole structure in a ferromagnetic condensate by suitably imprinting vortices and solitons for different spin components of the condensate.
In this thesis, we study theoretically and in experimentally the properties of spin-1 Bose-Einstein condensates with antiferromagnetic interactions realized in the ultra-cold sodium gases confined in optical dipole traps. We present in detail how to realize, diagnose and control the spinor Bose-Einstein condensates in our experiment. In order to describe the condensate, a mean-field theory is first adopted. This theory predicts a phase transition when changing the magnetic field B. The predictions of the mean-field theory agree very well with most of our experimental results, including the values of the critical magnetic field Bc, asymptotic values of n0 (relative atom number in mF=0 state) at large B and the phase diagram of n0. However, for small magnetization and small magnetic fields, we find abnormally large fluctuations (super-Poissonian) of n0. In order to describe these large fluctuations, we develop a full quantum statistical description for the spinor condensate at finite temperature. To describe uncondensed thermal atoms (also present in the same trap), we use the ``semi-ideal" Hartree-Fock approximation to deal with the interactions between the condensate atoms and the thermal ones. The experimental results lead us to introduce two kinds of temperatures, the ``spin temperature" Ts and the ``kinetic temperature" Tk with Ts≪Tk, characterizing respectively the fluctuaitons of the condensate spin and the thermal gas. We conclude that the system is reaching a quasi-equilibrium states, where different degrees of freedom reach equilibrium by separate mechanisms but where the mutual thermalization does not occur over the lifetime of the cloud.
Recently it has been predicted that if a gas of spin-1/2 bosonic atoms is cooled down while conserving its total spin, it can form a Bose-Einstein condensate in a new type of fragmented state. In that fragmented state two orbital wave functions are macroscopically occupied. We derive a set of Gross-Pitaevskii equations that describe the two occupied wave functions, taking into account the effects of interatomic interactions. We then analyze the solutions of those equations in some special cases. In particular, we find that if the fragmented state is realized in a toroidal trap, under certain conditions the system will spontaneously acquire macroscopic orbital angular momentum. Finally, we discuss the nature of the phase transition from an uncondensed gas to a fragmented-state condensate.